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The thermodynamic stability of structural isomers of $\mathrm{C}_{24}$, $\mathrm{C}_{26}$, $\mathrm{C}_{28}$ and $\mathrm{C}_{32}$, including fullerenes, is studied using density functional and quantum Monte Carlo methods. The energetic…

Atomic and Molecular Clusters · Physics 2009-10-31 P. R. C. Kent , M. D. Towler , R. J. Needs , G. Rajagopal

We study a new hypothetical form of solid carbon \csc, with a unit cell which is composed of the \cs \ fullerene cluster and an additional single carbon atom arranged in the zincblende structure. Using {\it ab initio} calculations, we show…

Condensed Matter · Physics 2016-08-31 Linda M. Zeger , Yu-Min Juan , Efthimios Kaxiras , A. Antonelli

The lowest energy configurations of Cn(n =< 55) clusters are obtained using the energy mini- mization technique with the conjugate gradient (CG) method where a modified Brenner potential is invoked to describe the carbon and hydrocarbon…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 D. P. Kosimov , A. A. Dzhurakhalov , F. M. Peeters

A class of highly symmetric silicon carbide fullerene-like cage nanoclusters with carbon atoms inside the Si_20 cage and with high stability are presented. The Generalized Gradient Approximation of Density Functional Theory (GGA-DFT) is…

Condensed Matter · Physics 2007-05-23 M. N. Huda , A. K. Ray

The four most stable structures of Ni$_N$ clusters with $N$ from 2 to 150 have been determined using a combination of the embedded-atom method in the version of Daw, Baskes and Foiles, the {\it variable metric/quasi-Newton} method, and our…

Atomic and Molecular Clusters · Physics 2016-09-08 V. G. Grigoryan , M. Springborg

Based on the third allotropic form of carbon (Fullerenes) through theoretical study have been predicted structures described as non-classical fullerenes. We have studied novel allotropic carbon structures with a closed cage configuration…

Materials Science · Physics 2017-05-24 Christian A. Celaya , Jesús Muñiz , Luis Enrique Sansores

The ground state structures of small silicon clusters are determined through exhaustive tight-binding molecular dynamics simulation studies. These simulations revealed that \Si{11} is an icosahedron with one missing cap, \Si{12} is a…

chem-ph · Physics 2016-08-31 Jun Pan , Atul Bahel , Mushti V. Ramakrishna

The morphology of Bucky onions is investigated by {\it ab initio} calculations using Yang's new $O(N)$ method. It is found that for large single shell fullerenes with $I_h$ symmetry, the spherical morphology has the lower energy than that…

Condensed Matter · Physics 2007-05-23 Jian Ping Lu

In this paper we propose a tight-binding molecular dynamics with parameters fitted to first-principles calculations on the smaller clusters and with an environment correction, to be a powerful technique for studying large transition/noble…

Atomic and Molecular Clusters · Physics 2009-11-10 Mukul Kabir , Abhijit Mookerjee , A. K. Bhattacharya

Motivated by contradicting reports in the literature, we have investigated the structural stability of tungsten nanoparticles using density functional theory calculations. The comparison of BCC, FCC, A15, disordered, and icosahedral…

Materials Science · Physics 2024-04-08 Laurent Pizzagalli , Sandrine Brochard , Julien Godet , Julien Durinck

The theoretical formalism of the local density approximation (LDA) to density functional theory (DFT) has been used to study the electronic and geometric structures of SimCn (1<=m, n<=4;n<=m) clusters. An all electron 6-311++G** basis set…

Atomic and Molecular Clusters · Physics 2007-05-23 Prachi Pradhan , Asok K. Ray

We present the first ab initio study of the geometry, electronic structure, charged states, bonding and vibrational modes of the recently synthesized fullerene-like As@Ni12@As20 cluster which has icosahedral point symmetry [Science, 300,…

Materials Science · Physics 2009-11-10 Tunna Baruah , Rajendra R. Zope , Steven L. Richardson , Mark R. Pederson , ;

A family of unusually stable boron cages was identified and examined using first-principles local density functional method. The structure of the fullerenes is similar to that of the B12 icosahedron and consists of six crossing…

Materials Science · Physics 2021-09-21 Nevill Gonzalez Szwacki

We report the first principle theory-based study of stability, electronic structure and optical properties of cluster assembled materials in various 1D, 2D and 3D nanostructures using a cage-like Cd9Te9 cluster as the super-atom. The bulk…

Mesoscale and Nanoscale Physics · Physics 2022-05-27 Kashinath T Chavan , Sharat Chandra

A class of silicon carbide cage clusters with two carbon atoms inside the silicon cage and with high stabilities are presented. The theoretical formalism used is Hartree-Fock theory followed by second order many body perturbation theory to…

Atomic and Molecular Clusters · Physics 2009-11-10 M. N. Huda , A. K. Ray

We have performed molecular dynamics simulations on the formation of mixed molecular clusters of buckminsterfullerene and coronene, $(\mathrm{C}_{24}\mathrm{H}_{12})_n(\mathrm{C}_{60})_{N-n}$. We report on our findings on the structures and…

Chemical Physics · Physics 2024-02-01 Naemi Florin , Henning Zettergren , Michael Gatchell

Using first-principles density functional theory based calculations, we analyze the structural stability of small clusters of 3$d$ late transition metals. We consider the relative stability of the two structures - layer-like structure with…

Mesoscale and Nanoscale Physics · Physics 2011-08-15 Soumendu Datta , Mukul Kabir , Tanusri Saha-Dasgupta

In this study, based on density functional theory (DFT), we propose a new branch of pseudo-fullerenes which contain triple bonds with sp hybridization. We should call these new nanostructures fullerynes, according to IUPAC. We present four…

Materials Science · Physics 2020-03-24 Mohammad Qasemnazhand , Farhad Khoeini , Farah Marsusi

Using density functional theory calculations, we study doping of a Cr, Mo, and W atom in boron clusters in the size range of 18-24 atoms and report the finding of metal atom encapsulated fullerene-like cage structures with 20 to 24 boron…

Atomic and Molecular Clusters · Physics 2019-07-31 Amol B. Rahane , Pinaki Saha , N. Sukumar , Vijay Kumar

Both even- and odd-numbered neutral carbon clusters Cn (n = 2-10) are systematically studied using the energy minimization method and the modified Brenner potential for the carbon-carbon interactions. Many stable configurations were found…

Materials Science · Physics 2009-11-13 D. P. Kosimov , A. A. Dzhurakhalov , F. M. Peeters
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