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The strongly correlated material FeSi exhibits several unusual thermal, magnetic, and structural properties under varying pressure-temperature (P-T) conditions. It is a potential thermoelectric alloy and a materials of several geological…

We have performed powder inelastic neutron scattering measurements on the unconventional superconductor $\beta$-FeSe ($T_{\rm c} \simeq 8\,\mathrm{K}$). The spectra reveal highly dispersive paramagnetic fluctuations emerging from the…

Superconductivity · Physics 2015-05-11 M. C. Rahn , R. A. Ewings , S. J. Sedlmaier , S. J. Clarke , A. T. Boothroyd

We present neutron scattering measurements on low-energy phonons from a superconducting ($T_{c} = 2.7$~K) Sn$_{0.8}$In$_{0.2}$Te single crystal sample. The longitudinal acoustic phonon mode and one transverse acoustic branch have been…

We report a comprehensive investigation of the lattice dynamics of URu$_2$Si$_2$ as a function of temperature using Raman scattering, optical conductivity and inelastic neutron scattering measurements as well as theoretical {\it ab initio}…

Inelastic and elastic neutron scattering have been used to study a single crystal of the Ni$_{54}$Mn$_{23}$Al$_{23}$ Heusler alloy over a broad temperature range. The paper reports the first experimental determination of the low-lying…

We use inelastic neutron scattering to study magnetic excitations of the FeAs-based superconductor BaFe$_{1.9}$Ni$_{0.1}$As$_2$ above and below its superconducting transition temperature $T_c=20$ K. In addition to gradually open a spin gap…

We use variable-temperature x-ray thermal diffuse scattering and inelastic scattering to investigate the lattice dynamics in single crystals of multiferroic CaMn7O12 which undergo a series of orbital and magnetic transitions at low…

Strongly Correlated Electrons · Physics 2016-11-24 S. M. Souliou , Y. Li , X. Du , M. Le Tacon , A. Bosak

We report a phonon density of states measurement of $\alpha$-ZnCl$_{2}$ using the coherent inelastic neutron scattering technique and a lattice dynamical calculation in four crystalline phases of ZnCl$_{2}$ using a transferable interatomic…

Materials Science · Physics 2007-05-23 A. Sen , Mala N. Rao , R Mittal , S. L. Chaplot

Inelastic neutron scattering measurements on the molecular dimer-Mott insulator $\kappa$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]Cl reveal a phonon anomaly in a wide temperature range. Starting from $T_{\rm ins}\sim50$-$60$ K where the charge gap…

The study of phonon coupling in doped semiconductors via electrical transport measurements is challenging due to unwanted temperature-induced effects such as dopant ionisation and parallel conduction. Here, we study phonon scattering in 2D…

Mesoscale and Nanoscale Physics · Physics 2025-03-03 Y. Ashlea Alava , K. Kumar , C. Harsas , P. Mehta , P. Hathi , C. Chen , D. A. Ritchie , A. R. Hamilton

Lithium transition metal phospho-olivines are useful electrode materials, owing to their stability, high safety, low cost and cyclability. We report phonon studies using neutron inelastic scattering experiments, ab-initio density functional…

Materials Science · Physics 2014-08-19 Prabhatasree Goel , M. K. Gupta , R. Mittal , S. Rols , S. J. Patwe , S. N. Achary , A. K. Tyagi , S. L. Chaplot

Phonon densities of states (DOS) for the high performing thermoelectric material, AgPbmSbTe2+m (LAST-m, m = 16, 18, and 20), were extracted from time-of-flight inelastic neutron scattering measurements. The phonon DOS of LAST-18 differs…

Materials Science · Physics 2011-06-13 M. E. Manley , S. Shapiro , Q. Li , A. Llobet , M. E. Hagen

Beta eucryptite (LiAlSiO4) shows one-dimensional super-ionic conductivity as well as anisotropic thermal expansion behavior. We have performed inelastic neutron scattering measurements in beta eucryptite over 300 to 900 K and calculated the…

Phonons in single crystals of PrFeAsO_{1-y} are investigated using high-resolution inelastic x-ray scattering and ab initio pseudopotential calculations. Extensive measurements of several samples at temperatures spanning the magnetic…

Strongly Correlated Electrons · Physics 2011-08-12 T. Fukuda , A. Q. R. Baron , H. Nakamura , S. Shamoto , M. Ishikado , M. Machida , H. Uchiyama , A. Iyo , H. Kito , J. Mizuki , M. Arai , H. Eisaki

Based on ab-initio calculated parameters, we apply a theoretical model on the iron-based BaFe2As2 superconductor that takes into account dramatic enhancements of the electron-phonon coupling of soft transverse phonons in the FeAs layers and…

Superconductivity · Physics 2019-06-14 Chi Ho Wong , Rolf Lortz

The dynamics of solid deuterium (sD2) is studied by means of inelastic scattering (coherent and incoherent) of thermal and cold neutrons at different temperatures and para-ortho ratios. In this paper, the results for the generalized density…

Materials Science · Physics 2009-05-26 A. Frei , E. Gutsmiedl , C. Morkel , A. R. Müller , S. Paul , M. Urban , H. Schober , S. Rols , T. Unruh M. Hölzel

The ferropnictide superconductors exhibit a sensitive interplay between the lattice and magnetic degrees of freedom, including a number of phonon modes that are much softer than predicted by nonmagnetic calculations using density functional…

Superconductivity · Physics 2014-03-13 D. Parshall , R. Heid , J. L. Niedziela , Th. Wolf , M. B. Stone , D. L. Abernathy , D. Reznik

We report inelastic neutron scattering measurements aimed at investigating the origin of the temperature-induced paramagnetism in the narrow-gap semiconductor FeSb2. We find that inelastic response for energies up to 60 meV and at…

Strongly Correlated Electrons · Physics 2011-12-05 I. A. Zaliznyak , A. T. Savici , V. O. Garlea , Rongwei Hu , C. Petrovic

Although the rutile structure of TiO$_2$ is stable at high temperatures, the conventional quasiharmonic approximation predicts that several acoustic phonons decrease anomalously to zero frequency with thermal expansion, incorrectly…

Materials Science · Physics 2015-08-19 Tian Lan , C. W. Li , O. Hellman , D. Kim , J. A. Muñoz , H. Smith , D. L. Abernathy , B. Fultz

One of the key requirements for good thermoelectric materials is a low lattice thermal conductivity. Here we present a combined neutron scattering and theoretical investigation of the lattice dynamics in the type I clathrate system…