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We report molecular dynamics simulation studies addressing the effects of pore connectivity on the dynamics of two representative fluids CO$_2$ and ethane in silicalite by systematically varying the degree of pore connectivity through…

Soft Condensed Matter · Physics 2023-04-28 Siddharth Gautam , David R. Cole

Equilibrium molecular dynamics simulations are used to investigate the effect of phase transitions on the transport properties of highly-confined water between parallel graphene sheets. An abrupt reduction by several orders of magnitude in…

Computational Physics · Physics 2019-01-23 Frederike Jaeger , Omar K. Matar , Erich A. Müller

When two binary solutions are separated by a permeable barrier, the individual species typically diffuse and mix, dissipating their chemical potential gradients. However, we use model lattice simulations to show that single-file…

Statistical Mechanics · Physics 2009-10-31 Tom Chou , Detlef Lohse

Superconductivity is inevitably suppressed in reduced dimensionality. Questions of how thin superconducting wires or films can be before they lose their superconducting properties have important technological ramifications and go to the…

Superconductivity · Physics 2015-06-25 Mustafa M. Ozer , James R. Thompson , Hanno H. Weitering

Using first-principles variable-composition evolutionary methodology, we explored the high-pressure structures of beryllium hydrides between 0 and 400 GPa. We found that BeH$_2$ remains the only stable compound in this pressure range. The…

Materials Science · Physics 2014-07-15 Shuyin Yu , Qingfeng Zeng , Artem R. Oganov , Chaohao Hu , Gilles Frapper , Litong Zhang

Mechanosensitive ion nanochannels regulate transport by undergoing conformational changes within nanopores. However, achieving precise control over these conformational states remains a major challenge for both artificial soft or solid…

Chemical Physics · Physics 2026-01-06 Ke Zhou

The effect of quantum confinement in the optical absorption spectra of atomically thin {\alpha}-In2Se3 crystals is studied, observing a huge thickness-dependent shift in the optical band gap of exfoliated {\alpha}-In2Se3 flakes. The band…

Mesoscale and Nanoscale Physics · Physics 2016-10-19 Jorge Quereda , Robert Biele , Gabino Rubio-Bollinger , Nicolás Agraït , Roberto D'Agosta , Andres Castellanos-Gomez

The apparently intractable shape of a fold in a compressed elastic film lying on a fluid substrate is found to have an exact solution. Such systems buckle at a nonzero wavevector set by the bending stiffness of the film and the weight of…

Soft Condensed Matter · Physics 2011-10-12 Haim Diamant , Thomas A. Witten

Band gap modification for small-diameter (1 nm) silicon nanowires resulting from the use of different species for surface termination is investigated by density functional theory calculations. Because of quantum confinement, small-diameter…

Materials Science · Physics 2010-02-03 Michael Nolan , Sean O'Callaghan , Giorgos Fagas , James C. Greer , Thomas Frauenheim

Since the discovery of high-temperature superconductivity in the thin-film FeSe/SrTiO$_3$ system, iron selenide and its derivates have been intensively scrutinized. Using ab initio density functional theory calculations we review the…

Superconductivity · Physics 2017-09-07 Daniel Guterding , Harald O. Jeschke , Roser Valenti

Unique optical properties of semiconductor nanoparticles (SN) make them very promising in the multitude of applications including lasing, light emission and photovoltaics. In many of these applications it is imperative to understand the…

Mesoscale and Nanoscale Physics · Physics 2017-01-04 Kirill A. Velizhanin

Despite decades of research in spatially confined superconducting systems to understand the modification of superconductivity from reduced length scales, the investigation of the quantum confinement effect on high-temperature…

Superconductivity · Physics 2024-07-08 Guanyang He , Yu Li , Yuxuan Lei , Andreas Kreisel , Brian M. Andersen , Jian Wang

The role of image charges in nanoporous semiconductor materials is investigated within the framework of the effective mass and envelope function approximations. We show that nanometric air bubbles in these materials can act as…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 J. Planelles , J. L. Movilla

We consider ion transport through protein ion channels in lipid membranes and water-filled nanopores in silicon films. It is known that, due to the large ratio of dielectric constants of water and the surrounding material, an ion placed…

Soft Condensed Matter · Physics 2009-11-11 J. Zhang , A. Kamenev , B. I. Shklovskii

A systematic study of the electronic properties of single layer Sb (antimonene) nanoribbons is presented. By using a 6-orbital tight-binding Hamiltonian, we study the electronic band structure of finite ribbons with zigzag or armchair…

Mesoscale and Nanoscale Physics · Physics 2018-12-05 Edo van Veen , Jin Yu , Mikhail I. Katsnelson , Rafael Roldan , Shengjun Yuan

For semimetal nanowires with diameters smaller than a few tens of nanometers, a semimetal-to-semiconductor transition is observed as the emergence of an energy band gap resulting from quantum confinement. Quantum confinement in a semimetal…

Mesoscale and Nanoscale Physics · Physics 2016-12-02 Alfonso Sanchez-Soares , James C. Greer

Motivated by recent advances in fabricating graphene nanostructures, we find that an electron can be trapped in Z-shaped graphene nanoconstriction with zigzag edges. The central section of the constriction operates as a single-level quantum…

Mesoscale and Nanoscale Physics · Physics 2010-09-23 Adam Rycerz

Hydrogenation has proven to be an effective tool to open the bandgap of graphene. In the present density functional study we demonstrate that single-side-hydrogenated graphene is a semiconductor with an indirect bandgap of 1.89 eV, in…

Materials Science · Physics 2011-03-01 Bhalchandra S. Pujari , Sergey Gusarov , Michael Brett , Andriy Kovalenko

By substituting S into single-layer FeSe/SrTiO3, chemical pressure is applied to tune its paramagnetic state that is modeled as an incoherent superposition of spin-spiral states. The resulting electronic bands resemble an ordered…

Superconductivity · Physics 2023-10-10 Qiang Zou , Basu Dev Oli , Huimin Zhang , Tatsuya Shishidou , Daniel Agterberg , Michael Weinert , Lian Li

We show that the negative electronic compressibility of two-dimensional electronic systems at sufficiently low density enables the generation of charge density waves through the application of a uniform force field, provided no current is…

Mesoscale and Nanoscale Physics · Physics 2017-08-23 Erica E. Hroblak , Alessandro Principi , Hui Zhao , Giovanni Vignale