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A "supercooled" liquid develops when a fluid does not crystallize upon cooling below its ordering temperature. Instead, the microscopic relaxation times diverge so rapidly that, upon further cooling, equilibration eventually becomes…

We show theoretically that spin and orbital degrees of freedom in the pyrochlore oxide Y2Mo2O7, which is free of quenched disorder, can exhibit a simultaneous glass transition, working as dynamical randomness to each other. The interplay of…

Disordered Systems and Neural Networks · Physics 2020-03-04 Kota Mitsumoto , Chisa Hotta , Hajime Yoshino

The pyrochlore antiferromagnet Tb2Ti2O7 has proven to be an enigma to experimentalists and theorists working on frustrated magnetic systems. The experimentally determined energy level structure suggests a local <111> Ising antiferromagnet…

Statistical Mechanics · Physics 2009-11-10 M. Enjalran , M. J. P. Gingras , Y. -J. Kao , A. Del Maestro , H. R. Molavian

The low-temperature thermodynamic properties of the frustrated pyrochlore Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$ have been studied using the single crystal of $x=0.005$ sitting in a long range ordered phase in the $x$-$T$ phase diagram. We observed…

Strongly Correlated Electrons · Physics 2017-04-25 H. Takatsu , T. Taniguchi , S. Kittaka , T. Sakakibara , H. Kadowaki

We report the discovery of a spin one diamond lattice in NiRh2O4. This spinel undergoes a cubic to tetragonal phase transition at T = 440 K that leaves all nearest neighbor interactions equivalent. In the tetragonal phase, magnetization…

Strongly Correlated Electrons · Physics 2018-03-30 J. R. Chamorro , L. Ge , J. Flynn , M. Subramanian , M. Mourigal , T. M. McQueen

We report the characterisation of natural samples of the cubic pyrite mineral MnS2 using very high resolution synchrotron X-ray diffraction techniques. At low temperatures we find a new low temperature polymorph, which results from coupling…

Strongly Correlated Electrons · Physics 2015-05-21 Simon A. J. Kimber , Tapan Chatterji

We present a model which accounts for the high field magnetisation at very low temperature in two pyrochlore frustrated systems, Er2Ti2O7 and Tb2Ti2O7. The two compounds present very different ground states: Er2Ti2O7, which has a planar…

Strongly Correlated Electrons · Physics 2015-06-15 Pierre Bonville , Sylvain Petit , Isabelle Mirebeau , Julien Robert , Elsa Lhotel , Carley Paulsen

Gd2GaSbO7 and Gd2InSbO7 pyrochlore compounds exhibit quantum fluctuations in a spin ice-like state. These compounds have not been adequately studied based on the concept of magnetic frustration. Here, we have synthesised and characterised…

Strongly Correlated Electrons · Physics 2024-08-06 S. Nallamuthu , Andrea Dzubinska , K. Arun , Vimaljith A. R , Marian Reiffers , R. Nagalakshmi , Ivan Curlik , Sergej Ilkovic

Ho2Ti2O7 and Dy2Ti2O7 spin ices exhibit elementary excitations akin to magnetic monopoles. Here we focus on Tb2Ti2O7 spin liquid, where correlated magnetic moments keep fluctuating down to very low temperatures. Using a monopole picture, we…

Strongly Correlated Electrons · Physics 2015-06-05 A. P. Sazonov , A. Gukasov , I. Mirebeau , P. Bonville

Geometrical frustration, as in pyrochlore lattices made of corner-sharing tetrahedra, precludes the onset of conventional magnetic ordering, enabling the stabilization of fluctuating spin states at low temperature. Disorder is a subtle…

Neutron scattering and magnetization measurements have been performed on the stuffed pyrochlore system Tb2+xTi2-2xNbxO7. We find that despite the introduction of chemical disorder and increasingly antiferromagnetic interactions, a spin…

Strongly Correlated Electrons · Physics 2010-02-25 B. G. Ueland , J. S. Gardner , A. J. Williams , M. L. Dahlberg , J. G. Kim , Y. Qiu , J. R. D. Copley , P. Schiffer , R. J. Cava

We present results of $^{23}$Na and $^{19}$F nuclear magnetic resonance (NMR) measurements on NaCaCo$_2$F$_7$, a frustrated pyrochlore magnet with a Curie-Weiss temperature, $T_{cw}$ ~-140 K, and intrinsic bond disorder. Below 3.6 K both…

Strongly Correlated Electrons · Physics 2017-12-20 R. Sarkar , J. W. Krizan , F. Brückner , E. C. Andrade , S. Rachel , M. Vojta , R. J. Cava , H. -H. Klauss

We investigated the nature of the freezing in the geometrically frustrated Heisenberg spin-glass Y2Mo2O7 by measuring the temperature dependence of the static internal magnetic field distribution above the spin-glass temperature, Tg, using…

Strongly Correlated Electrons · Physics 2009-11-11 Eva Sagi , Oren Ofer , Amit Keren , Jason S. Gardner

High resolution time-of-flight neutron scattering measurements on Tb2Ti2O7 reveal a rich low temperature phase diagram in the presence of a magnetic field applied along [110]. In zero field at T=0.4 K, terbium titanate is a highly…

Frustrated systems are ubiquitous and interesting because their behavior is difficult to predict. Magnetism offers extreme examples in the form of spin lattices where all interactions between spins cannot be simultaneously satisfied. Such…

Strongly Correlated Electrons · Physics 2009-11-07 S. -H. Lee , C. Broholm , W. Ratcliff , G. Gasparovic , Q. Huang , T. H. Kim , S. -W. Cheong

In the ground state of Ho2Ti2O7 spin ice, the disorder of the magnetic moments follows the same rules as the proton disorder in water ice. Excitations take the form of magnetic monopoles that interact via a magnetic Coulomb interaction.…

Strongly Correlated Electrons · Physics 2013-05-24 L. J. Chang , M. R. Lees , G. Balakrishnan , Y. -J. Kao , A. D. Hillier

Dy$_{2}$Zr$_{2}$O$_{7}$ a disordered pyrochlore system, exhibits the spin ice freezing under the application of magnetic field. Our studies suggest the stabilization of pyrochlore phase in Dy$_{2-x}$La$_{x}$Zr$_{2}$O$_{7}$ with the…

Strongly Correlated Electrons · Physics 2021-10-12 Sheetal , C. S. Yadav

Despite a Curie-Weiss temperature $\theta_{\rm CW} \sim -14$ K, the Tb2Ti2O7 pyrochlore magnetic material lacks long range magnetic order down to at least $T^*\approx 50$ mK. It has recently been proposed that the low temperature collective…

Statistical Mechanics · Physics 2009-05-07 Hamid R. Molavian , Michel J. P. Gingras

We report the low temperature magnetic properties of the pyrochlore Pr$_2$Hf$_2$O$_7$. Polycrystalline and single-crystal samples are investigated using time-of-flight neutron spectroscopy and macroscopic measurements, respectively. The…

The ferrimagnetic spinels MnB2O4 (B = Mn,V) exhibit a similar series of closely spaced magnetic and structural phase transitions at low temperatures, reflecting both magnetic frustration and a strong coupling between the spin and lattice…

Strongly Correlated Electrons · Physics 2015-01-28 S. L. Gleason , T. Byrum , Y. Gim , A. Thaler , P. Abbamonte , G. J. MacDougall , L. W. Martin , H. D. Zhou , S. L. Cooper
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