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This paper presents a proposal of a rather new type of effective interatomic interaction for molecular dynamics and similar applications. The model consists of atoms with prescribed geometric arrangement of active orbitals, represented by…

Chemical Physics · Physics 2009-10-19 Ladislav Kocbach , Suhail Lubbad

We first argue that the covalent bond and the various closed-shell interactions can be thought of as symmetry broken versions of one and the same interaction, viz., the multi-center bond. We use specially chosen molecular units to show that…

Strongly Correlated Electrons · Physics 2017-06-16 Jon C. Golden , Vinh Ho , Vassiliy Lubchenko

The approximate atomic self-interaction corrections (ASIC) method to density functional theory is put to the test by calculating the exchange interaction for a number of prototypical materials, critical to local exchange and correlation…

Materials Science · Physics 2009-11-13 A. Akande , S. Sanvito

Giant atoms -- quantum emitters that couple to light at multiple discrete points -- are emerging as a new paradigm in quantum optics thanks to their many promising properties, such as decoherence-free interaction. While most previous work…

Quantum Physics · Physics 2023-01-18 Ariadna Soro , Carlos Sánchez Muñoz , Anton Frisk Kockum

We investigate theoretically the long-range electrostatic interactions between a ground-state homonuclear alkali-metal dimer and an excited alkali-metal atom taking into account its fine-structure. The interaction involves the combination…

Chemical Physics · Physics 2017-09-13 Maxence Lepers , Olivier Dulieu

Even something as conceptually simple as adsorption of electronegative adatoms on metal surfaces, where repulsive lateral interactions are expected for obvious reasons, can lead to unanticipated behavior. In this context, we explain the…

Materials Science · Physics 2020-05-01 Matic Poberžnik , Anton Kokalj

We study the two-body problem of the ultracold fermionic alkaline-earth (like) atoms in the electronic $^1$S$_0$ state ($g$-state) and $^3$P$_0$ state ($e$-state), which are confined in a quasi-one-dimensional (quasi-1D) tube. In addition,…

Quantum Gases · Physics 2020-02-05 Ren Zhang , Peng Zhang

The way atoms attach to each other defines the function(s), e.g., mechanical, optical, electronic, of a given material. The nature of the chemical bond is, therefore, one of the most fundamental issues in materials. Both ionic interactions,…

Materials Science · Physics 2019-07-10 Yevgeny Rakita , Thomas Kirchartz , Gary Hodes , David Cahen

In the field of noncovalent interactions a new paradigm has recently become popular. It stems from the analysis of molecular electrostatic potentials and introduces a label, which has recently attracted enormous attention. The label is…

Chemical Physics · Physics 2017-08-31 Michal H. Kolář , Pavel Hobza

We review two different theoretical approaches to the strong interaction dynamics at the early times immediately following heavy ion collisions. One approach is based on small-coupling physics of the Color Glass Condensate (CGC). The other…

High Energy Physics - Phenomenology · Physics 2009-11-18 Yuri V. Kovchegov

We present a tight-binding potential for transition metals, carbon, and transition metal carbides, which has been optimized through a systematic fitting procedure. A minimal basis, including the s, p electrons of carbon and the d electrons…

We find a geometric description of interacting $\beta\gamma$-systems as a null Kac-Moody quotient of a nonlinear sigma-model for systems with varying amounts of supersymmetry.

High Energy Physics - Theory · Physics 2020-07-15 Ulf Lindström , Martin Roček

A method for generating angular forces around $\sigma$-bonded transition metal ions is generalized to treat $\pi$-bonded configurations. The theoretical approach is based on an analysis of a ligand-field Hamiltonian based on the moments of…

Soft Condensed Matter · Physics 2009-10-31 A. E. Carlsson , S. Zapata

We describe the collisional interaction between two different atoms that are trapped in a harmonic potential. The atoms are exposed to a magnetic field, which is modulated in the vicinity of an s-wave Feshbach resonance, and we study the…

Other Condensed Matter · Physics 2007-06-29 Jesper Fevre Bertelsen , Klaus Molmer

To understand the recently observed mysterious non-adiabatic energy transfer for hyperthermal H atom scattering from a semiconductor surface, Ge(111)c(2*8), we present a mixed quantum-classical non-adiabatic molecular dynamics model based…

The theory of correlated electron systems is formulated in a form which allows to use as a reference point an ab initio band structure theory (AIBST). The theory is constructed in two steps. As a first step the total Hamiltonian is…

Strongly Correlated Electrons · Physics 2007-05-23 Igor Sandalov , Borje Johansson , Olle Eriksson

We investigate an effective model for organometallic complexes (with potential uses in optoelectronic devices) via both exact diagonalisation and the configuration interaction singles (CIS) approximation. This model captures a number of…

Strongly Correlated Electrons · Physics 2011-10-17 A. C. Jacko , B. J. Powell

In this paper we continue our analysis of the interplay between the pairing and the non-Fermi liquid behavior in a metal for a set of quantum-critical (QC) systems with an effective dynamical electron-electron interaction $V(\Omega_m)…

Superconductivity · Physics 2021-01-27 Yi-Ming Wu , Shang-Shun Zhang , Artem Abanov , Andrey V. Chubukov

Metal-semiconductor contacts are a pillar of modern semiconductor technology. Historically, their microscopic understanding has been hampered by the inability of traditional analytical and numerical methods to fully capture the complex…

Materials Science · Physics 2016-04-13 Daniele Stradi , Umberto Martinez , Anders Blom , Mads Brandbyge , Kurt Stokbro

The nature of metal silane sigma-bond interaction has been investigated in several key systems by a range of experimental and computational techniques. The structure of [Cp'Mn(CO)2(eta2-HSiHPh2)] 1 has been determined by single crystal…

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