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Light-matter interaction at the nanoscale in magnetic alloys and heterostructures is a topic of intense research in view of potential applications in high-density magnetic recording. While the element-specific dynamics of electron spins is…

The ultrafast time-dependence of the energy absorption of covalent solids upon excitation with femtosecond laser pulses is theoretically analyzed. We use a microscopic theory to describe laser induced structural changes and their influence…

Materials Science · Physics 2007-05-23 H. O. Jeschke , M. E. Garcia , K. H. Bennemann

The ultrafast structure dynamics and surface transient electric field, which are concurrently induced by laser excited electrons of an aluminum nanofilm, have been investigated simultaneously by the same transmission electron diffraction…

Materials Science · Physics 2014-07-17 Run-Ze Li , Pengfei Zhu , Long Chen , Jie Chen , Jianming Cao , Zheng-Ming Sheng , Jie Zhang

We report on ultrafast optical experiments in which femtosecond mid-infrared radiation is used to excite the lattice of complex oxide heterostructures. By tuning the excitation energy to a vibrational mode of the substrate, a long-lived…

We report the lattice dynamics of transition metal thin films by using the ultrafast electron diffraction. We observe a suppression of the diffraction intensity in a few picosecond after the photoexcitation, which is directly interpreted as…

Materials Science · Physics 2016-01-19 A. Nakamura , T. Shimojima , M. Nakano , Y. Iwasa , K. Ishizaka

Resonant optical excitation of apical oxygen vibrational modes in the normal state of underdoped YBa2Cu3O6+x induces a transient state with optical properties similar to those of the equilibrium superconducting state. Amongst these, a…

The complex interaction dynamics of intense femtosecond (fs) pulses and their picosecond (ps)-long leading edge with nanostructured solids occur at both the nanometer and the femtosecond scales, making them extremely difficult to measure…

Plasma Physics · Physics 2024-03-19 Ankit Dulat , Sagar Dam , Sk Rakeeb , Amit D. Lad , Yash M. Ved , G. Ravindra Kumar

We use femtosecond x-ray diffraction to study the structural response of charge and orbitally ordered Pr$_{1-x}$Ca$_x$MnO$_3$ thin films across a phase transition induced by 800 nm laser pulses. By investigating the dynamics of both…

Optically induced ultrafast electronic excitations with sufficiently long lifetimes may cause strong effects on phase transitions like structural and nonmetal to metal ones. Examples are transitions diamond to graphite, graphite to…

Materials Science · Physics 2010-09-21 K. H. Bennemann

Hot electrons formed in a graphene crystal by high-intensity short-duration laser pulses can exist for a time that is less than an electron-phonon energy relaxation time. During that time, electron-electron collisions cause the electrons to…

Mesoscale and Nanoscale Physics · Physics 2024-02-21 E. G. Mishchenko

Melting is an everyday phase transition that is determined by thermodynamic parameters like temperature and pressure. In contrast, ultrafast melting is governed by the microscopic response to a rapid energy input and, thus, can reveal the…

We present an electron projection imaging method to study the ultrafast evolution of photoelectron density distribution and transient fields near the surface. The dynamical profile of the photoelectrons from graphite reveals an origin of a…

Materials Science · Physics 2015-05-14 Ramani K. Raman , Zhensheng Tao , Tzong-Ru Han , Chong-Yu Ruan

We present an experimental observation of non-linear up- and down-converted optical luminescence of graphene and thin graphite subject to picosecond infrared laser pulses. We show that the excitation yields to a high density electron-hole…

Materials Science · Physics 2010-10-01 Rainer J. Stoehr , Roman Kolesov , Jens Pflaum , Joerg Wrachtrup

Direct visualization of ultrafast coupling between charge carriers and lattice degrees of freedom in photo-excited semiconductors has remained a long-standing challenge and is critical for understanding the light-induced physical behavior…

We propose a kinetic model of transient nonequilibrium phenomena in metals exposed to ultrashort laser pulses when heated electrons affect the lattice through direct electron-phonon interaction. This model describes the destruction of a…

Statistical Mechanics · Physics 2009-10-31 L. A. Falkovsky , E. G. Mishchenko

We utilize coherent femtosecond extreme ultraviolet (EUV) pulses derived from a free electron laser (FEL) to generate transient periodic magnetization patterns with periods as short as 44 nm. Combining spatially periodic excitation with…

Superlattices are artificial periodic nanostructures which can control the flow of electrons. Their operation typically relies on the periodic modulation of the electric potential in the direction of electron wave propagation. Here we…

Mesoscale and Nanoscale Physics · Physics 2012-04-26 Hugen Yan , Xuesong Li , Bhupesh Chandra , George Tulevski , Yanqing Wu , Marcus Freitag , Wenjuan Zhu , Phaedon Avouris , Fengnian Xia

The use of femtosecond laser pulses to impulsively excite thermal and mechanical transients in matter has led, in the last years, to the development of picosecond acoustics. Recently, the pump-probe approach has been applied to…

Mesoscale and Nanoscale Physics · Physics 2010-04-02 C. Giannetti , F. Banfi , D. Nardi , G. Ferrini , F. Parmigiani

The formation of permanent laser-induced periodic surface structures (LIPSS) on solid surfaces under impulsive laser irradiation above the damage threshold has been subject of extensive research. We demonstrate the formation of transient…

We theoretically investigate the generation of ultrafast currents in insulators induced by strong few-cycle laser pulses. Ab initio simulations based on time-dependent density functional theory give insight into the atomic-scale properties…