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The heterogeneous oxidation reaction of single aqueous ascorbic acid (AH$_2$) aerosol particles with gas-phase ozone was investigated in this study utilizing aerosol optical tweezers with Raman spectroscopy. The measured liquid-phase…

Chemical Physics · Physics 2021-05-12 Yuan-Pin Chang , Shan-Jung Wu , Min-Sian Lin , Che-Yu Chiang , Genin Gary Huang

Surfaces are able to control physical-chemical processes in multi-component solution systems and, as such, find application in a wide range of technological devices. Understanding the structure, dynamics and thermodynamics of non-ideal…

Soft Condensed Matter · Physics 2023-09-29 Aaron R. Finney , Matteo Salvalaglio

We consider the interactions between two uncharged planar macroscopic surfaces immersed in an electrolyte solution which are induced by interfacial selectivity. These forces are taken into account by introducing a depletion free-energy…

Soft Condensed Matter · Physics 2009-10-31 M. N. Tamashiro , P. Pincus

We argue that the kosmotropes remain strongly hydrated in the vicinity of a hydrophobic surface, while the chaotropes lose their hydration shell and can become adsorbed to the interface. The mechanism of adsorption is still a subject of…

Soft Condensed Matter · Physics 2018-02-14 Alexandre P. dos Santos , Yan Levin

Deformations of horizontal liquid interfaces by optical radiation pressure are generally expected to display similar behaviors whatever the direction of propagation of the exciting laser beam is. In the present experiment we find this…

Optics · Physics 2009-11-07 Alexis Casner , Jean-Pierre Delville , Iver Brevik

Thin liquid films on surfaces are part of our everyday life, they serve e.g. as coatings or lubricants. The stability of a thin layer is governed by interfacial forces, described by the effective interface potential, and has been subject of…

Soft Condensed Matter · Physics 2015-06-04 Oliver Bäumchen , Renate Fetzer , Mischa Klos , Matthias Lessel , Ludovic Marquant , Hendrik Hähl , Karin Jacobs

Starch solutions, which are strongly non-Newtonian, show a surface instability, when subjected to a load. A droplet of the fluid is sandwiched between two glass plates and a weight varying from 1 to 5 kgs. is placed on the top plate. The…

Soft Condensed Matter · Physics 2010-12-13 Moutushi Dutta Choudhury , Subrata Chandra , Soma Nag , Shantanu Das , Sujata Tarafdar

An accurate description of electron-ion interactions in materials is crucial for our understanding of their equilibrium and non-equilibrium properties. Here, we assess the properties of frictional forces experienced by ions in…

Disordered Systems and Neural Networks · Physics 2020-07-15 Jacopo Simoni , Jerome Daligault

The presence of even small amount of surfactant at the particle-laden fluid interface subjected to shear makes surface flow incompressible if the shear rate is small enough [T. M. Fischer et al, J. Fluid Mech. 558, 451 (2006)]. In the…

Soft Condensed Matter · Physics 2014-04-07 S. V. Lishchuk

The electrostatic interaction between two non-identical, moderately charged colloids situated in close proximity of each other at a fluid interface is studied. By resorting to a well-justified model system, this problem is analytically…

Soft Condensed Matter · Physics 2018-04-30 Arghya Majee , Timo Schmetzer , Markus Bier

Understanding the force between charged surfaces immersed in an electrolyte solution is a classic problem in soft matter and liquid-state theory. Recent experiments showed that the force decays exponentially but the characteristic decay…

Soft Condensed Matter · Physics 2018-09-26 Alpha A. Lee , Jean-Pierre Hansen , Olivier Bernard , Benjamin Rotenberg

We study the breakup of a liquid thread inside another liquid at different surface tensions. In general, the pinch-off of a liquid thread is governed by the dynamics of fluid flow. However, when the interfacial tension is ultralow (2 to 3…

Soft Condensed Matter · Physics 2022-11-29 Jack Hau Yung Lo , Yuan Liu , Sze Yi Mak , Zhuo Xu , Youchuang Chao , Kaye Jiale Li , Ho Cheung Shum , Lei Xu

In the supercooled regime at elevated pressure two forms of liquid water, high-density (HDL) and low-density (LDL), have been proposed to be separated by a coexistence line ending at a critical point, but a connection to ambient conditions…

Soft Condensed Matter · Physics 2011-06-27 K. T. Wikfeldt , A. Nilsson , L. G. M. Pettersson

Interfacial behaviours in multiphase systems containing H2 are crucial to underground H2 storage but are not well understood. Molecular dynamics simulations were conducted to study interfacial properties of the H2O+H2 and…

Chemical Physics · Physics 2022-12-29 Yafan Yang , Arun Kumar Narayanan Nair , Weiwei Zhu , Shuxun Sang , Shuyu Sun

The linear stability analysis of an optically thin plasma where a general reaction proceeds, including chemical relaxation time effects, is carried out . A fifth order dispersion equation (instead of the fourth order one resulting when such…

Astrophysics · Physics 2007-05-23 Miguel H. Iba~nez S.

We consider a model fluid with long-ranged, dispersion interparticle potentials confined between competing parallel walls. One wall is solvophilic and would be completely wet at bulk liquid-gas coexistence while the other is solvophobic and…

Soft Condensed Matter · Physics 2015-06-05 M. C. Stewart , R. Evans

The fragilities (Tg-normalized temperature dependence of alpha-relaxation times) of 33 glass-forming liquids and polymers are compared for isobaric, mP, and isochoric, mV, conditions. We find that the two quantities are linearly correlated,…

Soft Condensed Matter · Physics 2009-11-11 R. Casalini , C. M. Roland

Universal properties of the Coulomb interaction energy apply to all many-electron systems. Bounds on the exchange-correlation energy, inparticular, are important for the construction of improved density functionals. Here we investigate one…

Chemical Physics · Physics 2015-05-13 Mariana M. Odashima , K. Capelle

Microgels are soft colloidal particles constituted by cross-linked polymer networks with a high potential for applications. In particular, after adsorption at a fluid interface, interfacial tension provides two-dimensional (2D) confinement…

Soft Condensed Matter · Physics 2021-09-03 Jacopo Vialetto , Natalie Nussbaum , Jotam Bergfreund , Peter Fischer , Lucio Isa

We revisit the role of the local solvent structure on the activity coefficient of electrolytes with a general non-local dielectric function approach. We treat the concentrated electrolyte as a dielectric medium and suggest an interpolated…

Chemical Physics · Physics 2020-01-08 Amir Levy , Martin Z. Bazant , Alexei A. Kornyshev
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