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Single crystals of EuPd$_3$Si$_2$ were grown using a high-temperature EuPd-flux method. The material was structurally and chemically characterized by single-crystal x-ray diffraction, powder x-ray diffraction, Laue method and…

Strongly Correlated Electrons · Physics 2026-02-19 Michelle Ocker , Franziska Walther , Nour Maraytta , Matthieu Le Tacon , Michael Merz , Cornelius Krellner , Kristin Kliemt

Magnetic structures and the relationship between spin and charge-orbital orderings of an A-site ordered double-perovskite manganite SmBaMn2O6, an anticipated multiferroic material, were investigated by means of neutron diffraction. The spin…

Strongly Correlated Electrons · Physics 2021-07-14 Ryoji Kiyanagi , Shigeki Yamada , Hiroshi Aoki , Hajime Sagayama , Taketo Moyoshi , Akiko Nakao , Takahisa Arima

We report inelastic neutron scattering studies of magnetic excitations in antiferromagnetically ordered SrFe$_{2}$As$_{2}$ ($T_{N}=220$ K), the parent compound of the FeAs-based superconductors. At low temperatures (T=7 K), the spectrum of…

We investigated the magnetic phase diagram of single crystals of SrNdFeO$_{4}$ by measuring the magnetic properties, the specific heat and the dielectric permittivity. The system has two magnetically active ions, Fe$^{3+}$ and Nd$^{3+}$.…

Materials Science · Physics 2015-06-05 J. M. Hwang , E. S. Choi , H. D. Zhou , Y. Xin , J. Lu , P. Schlottmann

We report measurements of magnetization, specific heat, and thermal expansion performed on As-deficient MnAs single crystals (MnAs$_{0.968}$). Ferromagnetic order is observed near $T_C \simeq$ 306 K on warming and $T_C \simeq$ 302 K on…

Strongly Correlated Electrons · Physics 2024-08-16 B. D. White , K. Huang , I. L. Fipps , J. J. Hamlin , S. Jang , G. J. Smith , B. Xia , J. W. Simonson , C. S. Nelson , M. C. Aronson , M. B. Maple

The transition temperature Tc~26 K of the recently discovered superconductor LaFeAs(O,F) has been demonstrated to be extremely sensitive to the lanthanide ion, reaching 55 K for the Sm containing oxypnictides. Therefore, it is important to…

Superconductivity · Physics 2008-12-17 Y. Qiu , Wei Bao , Q. Huang , T. Yildirim , J. Simmons , J. W. Lynn , Y. C. Gasparovic , J. Li , M. Green , T. Wu , G. Wu , X. H. Chen

Nematic orders emerge nearly universally in iron-based superconductors, but elucidating their origins is challenging because of intimate couplings between orbital and magnetic fluctuations. The iron-based ladder material BaFe2S3, which…

Spinel compounds AB$_{2}$X$_{4}$ consist of both tetrahedral (AX$_{4}$) and octahedral (BX$_{6}$) environments with the former forming a diamond lattice and the latter a geometrically frustrated pyrochlore lattice. Exploring the fascinating…

Chemical Physics · Physics 2023-03-29 Qiang Zhang , Wei Tian , Roshan K. Nepal , Ashfia Huq , Stephen Nagler , J. F. DiTusa , Rongying Jin

We investigate the temperature evolution of the structural parameters of potential ferrotoroidic LiFeSi2O6 compound across structural and magnetic phase transitions. The structural transition (TS)is around 220K and the paramagnetic to…

Strongly Correlated Electrons · Physics 2019-09-04 R. K. Maurya , Priyamedha Sharma , R. Rawat , R. S. Singh , R. Bindu

Neutron diffraction measurements have been carried out to investigate the magnetic form factor of the parent SrFe2As2 system of the iron-based superconductors. The general feature is that the form factor is approximately isotropic in wave…

Superconductivity · Physics 2010-04-20 W. Ratcliff , P. A. Kienzle , Jeffrey W. Lynn , Shiliang Li , Pengcheng Dai , G. F. Chen , N. L. Wang

Neutron diffraction and magnetic susceptibility studies of a polycrystalline SrCr$_2$As$_2$ sample reveal that this compound is an itinerant G-type antiferromagnet below the N${\rm \acute{e}}$el temperature $T_{\textrm N}$ = 590(5) K with…

Cooperative Jahn-Teller ordering is well-known to drive the cubic $Fd\overline{3}m$ to tetragonal $I$4$_1$/$amd$ structural distortion in Mn$_3$O$_4$ at 1170 $^{\circ}$C. Further structural distortion occurs in Mn$_3$O$_4$ upon magnetic…

Materials Science · Physics 2014-08-26 Moureen C. Kemei , Jaye K. Harada , Ram Seshadri , Matthew R. Suchomel

We set forth the structural and magnetic properties of the frustrated spin-$5/2$ triangle lattice antiferromagnet Na$_3$Fe(PO$_4$)$_2$ examined via x-ray diffraction, magnetization, heat capacity, and neutron diffraction measurements on the…

Materials Science · Physics 2022-01-26 Sebin J. Sebastian , A. Jain , S. M. Yusuf , M. Uhlarz , R. Nath

We review neutron scattering investigations of the crystal structures, magnetic structures, and spin dynamics of the iron-based RFe(As,P)O (R=La, Ce, Pr, Nd), (Ba,Sr,Ca)Fe2As2, and Fe1+x(Te-Se) systems. On cooling from room temperature all…

Superconductivity · Physics 2009-05-20 Jeffrey W. Lynn , Pengcheng Dai

Er2Ti2O7 is believed to be a realization of an XY antiferromagnet on a frustrated lattice of corner-sharing regular tetrahedra. It is presented as an example of the order-by-disorder mechanism in which fluctuations lift the degeneracy of…

Strongly Correlated Electrons · Physics 2012-09-28 P. Dalmas de Reotier , A. Yaouanc , Y. Chapuis , S. H. Curnoe , B. Grenier , E. Ressouche , C. Marin , J. Lago , C. Baines , S. R. Giblin

Neutron and x-ray diffraction studies of Ba(Fe{1-x}Mn{x})2As2 for low doping concentrations (x <= 0.176) reveal that at a critical concentration, 0.102 < x < 0.118, the tetragonal-to-orthorhombic transition abruptly disappears whereas…

Using x-ray powder diffraction technique at various temperatures and applied magnetic fields, we have studied the magnetostructural properties of Ce(Fe0.95Si0.05)2. The x-ray diffraction data establish quantitative relationships between…

Strongly Correlated Electrons · Physics 2010-05-21 Arabinda Haldar , Niraj K. Singh , Ya. Mudryk , K. G. Suresh , A. K. Nigam , V. K. Pecharsky

Magnetic ordering in the geometrically frustrated magnetic oxide spinels MgCr_2O_4 and ZnCr_2O_4 is accompanied by a structural change that helps relieve the frustration. Analysis of high-resolution synchrotron X-ray scattering reveals that…

This study investigates the changes of magnetic ordering temperature via nano- and mesoscale structural features in an iron arsenide. Although magnetic ground states in quantum materials can be theoretically predicted from known crystal…

By performing high-pressure single-crystal neutron diffraction measurements, the evolution of structure and magnetic ordering in EuFe2As2 under hydrostatic pressure were investigated. Both the tetragonal-toorthorhombic structural transition…

Superconductivity · Physics 2019-07-24 W. T. Jin , Y. Xiao , S. Nandi , S. Price , Y. Su , K. Schmalzl , W. Schmidt , T. Chatterji , A. Thamizhavel , Th. Brueckel