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The tunability and spatial precision of paramagnetic molecules makes them attractive for quantum sensing. However, usual microwave-based detection methods have poor temporal and spatial resolution, and optical methods compatible with…

Quantum Physics · Physics 2024-07-30 Erica Sutcliffe , Nathanael P. Kazmierczak , Ryan G. Hadt

Electron spin qubits in molecular systems offer high reproducibility and the ability to self assemble into larger architectures. However, interactions between neighbouring qubits are 'always-on' and although the electron spin coherence…

Single molecule magnets straddle the classical and quantum mechanical worlds, displaying many fascinating phenomena. They may have important technological applications in information storage and quantum computation. We review the physical…

Mesoscale and Nanoscale Physics · Physics 2010-08-06 Jonathan R. Friedman , Myriam P. Sarachik

Magnetic hysteresis has become a crucial aspect for characterizing single-molecule magnets, but the comprehension of the coercivity mechanism is still a challenge. By using analytical derivation and quantum dynamical simulations, we reveal…

Materials Science · Physics 2023-09-08 Lei Gu , Qiancheng Luo , Guoping Zhao , Yan-Zhen Zheng , Ruqian Wu

Precise control of the resonant frequency of a spin qubit is of fundamental importance to quantum sensing protocols. We demonstrate a control technique on a single nitrogen-vacancy (NV) centre in diamond where the applied magnetic field is…

Engineered spin-electric coupling enables spin qubits in semiconductor nanostructures to be manipulated efficiently and addressed individually. While synthetic spin-orbit coupling using a micromagnet is widely used for driving qubits based…

Single molecule magnets and single spin centers can be individually addressed when coupled to contacts forming an electrical junction. In order to control and engineer the magnetism of quantum devices, it is necessary to quantify how the…

Mesoscale and Nanoscale Physics · Physics 2015-11-20 Peter Jacobson , Tobias Herden , Matthias Muenks , Gennadii Laskin , Oleg Brovko , Valeri Stepanyuk , Markus Ternes , Klaus Kern

We provide the first evidence for coherence and Rabi oscillations of spin-solitons pinned by the local breaking of translational symmetry in isotropic Heisenberg chains (simple antiferromagnetic-N\'{e}el or spin-Peierls).We show that these…

Strongly Correlated Electrons · Physics 2015-06-18 Sylvain Bertaina , Charles-Emmanuel Dutoit , Johan Van Tol , Martin Dressel , Bernard Barbara , Anatoli Stepanov

In this paper, we investigate the thermal quantum correlations in a semiconductor double quantum dot system. The device comprises a single electron in a double quantum dot subjected to a longitudinal magnetic field and a transverse magnetic…

Quantum Physics · Physics 2024-12-30 Vinicius Leitão , Onofre Rojas , Moises Rojas

Cold molecules provide an excellent platform for quantum information, cold chemistry, and precision measurement. Certain molecules have enhanced sensitivity to beyond Standard Model physics, such as the electron's electric dipole moment…

We study the decay of multiple quantum (MQ) NMR coherences in systems with the large number of equivalent spins. As being created on the preparation period of MQ NMR experiment, they decay due to the dipole-dipole interactions (DDI) on the…

Quantum Physics · Physics 2011-01-25 S. I. Doronin , E. B. Fel'dman , A. I. Zenchuk

A lateral quantum dot design for coherent electrical manipulation of a two-level spin-charge system is presented. Two micron-size permanent magnets integrated to high-frequency electrodes produce a static slanting magnetic field suitable…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 M. Pioro-Ladriere , Y. Tokura , T. Obata , T. Kubo , S. Tarucha

We investigate theoretically the coherent longitudinal and transversal spin relaxation of photoexcited electrons in quantum wells in quantized magnetic fields. We find the relaxation time for typical quantum well parameters between 100 and…

Disordered Systems and Neural Networks · Physics 2009-11-11 E. Ya. Sherman , J. E. Sipe

We analyze quantum coherence generated by non-interacting magnons in a ferromagnetic spin chain described by the isotropic Heisenberg model. The exact expression derived for the reduced density operator of an arbitrary subsystem reveals…

Quantum Physics · Physics 2025-09-23 V. C. Vieira , F. M. de Paula

We demonstrate fluorescence thermometry techniques with sensitivities approaching 10 mK Hz^(-1/2) based on the spin-dependent photoluminescence of nitrogen vacancy (NV) centers in diamond. These techniques use dynamical decoupling protocols…

Mesoscale and Nanoscale Physics · Physics 2013-05-24 David M. Toyli , Charles F. de las Casas , David J. Christle , Viatcheslav V. Dobrovitski , David D. Awschalom

Quantum information, encoded within the states of quantum systems, represents a novel and rich form of information which has inspired new types of computers and communications systems. Many diverse electron spin systems have been studied…

Quantum Physics · Physics 2019-06-06 John J. L. Morton , Patrice Bertet

For the realisation of scalable solid-state quantum-bit systems, spins in semiconductor quantum dots are promising candidates. A key requirement for quantum logic operations is a sufficiently long coherence time of the spin system.…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 T. Korn , M. Kugler , M. Griesbeck , R. Schulz , A. Wagner , M. Kubová , C. Gerl , D. Schuh , W. Wegscheider , C. Schüller

How many magnetic moments periodically arranged on a metallic surface are needed to generate a coherent Kondo lattice behavior? We investigate this fundamental issue within the particle-hole symmetric Kondo lattice model using quantum Monte…

Strongly Correlated Electrons · Physics 2019-03-12 Marcin Raczkowski , Fakher F. Assaad

Erbium ions doped into crystals have unique properties for quantum information processing, because of their optical transition at 1.5 $\mu$m and of the large magnetic moment of their effective spin-1/2 electronic ground state. Most…

Controlling nanocircuits at the single electron spin level is a possible route for large-scale quantum information processing. In this context, individual electron spins have been identified as versatile quantum information carriers to…

Mesoscale and Nanoscale Physics · Physics 2017-11-01 H. Flentje , P-A. Mortemousque , R. Thalineau , A. Ludwig , A. D. Wieck , C. Bäuerle , T. Meunier