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Nuclear polarization dynamics are measured in the nuclear spin bi-stability regime in a single optically pumped InGaAs/GaAs quantum dot. The controlling role of nuclear spin diffusion from the dot into the surrounding material is revealed…

We present a detailed experimental and theoretical analysis of the optical orientation of electron spins in GaAs/AlAs quantum wells. Using time and polarization resolved photoluminescence excitation spectroscopy, the initial degree of…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 S. Pfalz , R. Winkler , T. Nowitzki , D. Reuter , A. D. Wieck , D. Haegele , M. Oestreich

We report the optical spectroscopic results of a single self-assembled InAlAs/Al GaAs quantum dot. The polarization-dependent shift of the Zeeman splitting in a single InAlAs QD has been observed. The induced Overhauser field is estimated…

Other Condensed Matter · Physics 2009-11-10 T. Yokoi , S. Adachi , H. Sasakura , S. Muto , H. Z. Song , T. Usuki , S. Hirose

We demonstrate that bistability of the nuclear spin polarization in optically pumped semiconductor quantum dots is a general phenomenon possible in dots with a wide range of parameters. In experiment, this bistability manifests itself via…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 A. Russell , Vladimir I. Fal'ko , A. I. Tartakovskii , M. S. Skolnick

Optical and electrical control of the nuclear spin system allows enhancing the sensitivity of NMR applications and spin-based information storage and processing. Dynamic nuclear polarization in semiconductors is commonly achieved in the…

Mesoscale and Nanoscale Physics · Physics 2014-09-09 G. Sallen , S. Kunz , T. Amand , L. Bouet , T. Kuroda , T. Mano , D. Paget , O. Krebs , X. Marie , K. Sakoda , B. Urbaszek

We present an experimental study of the dynamics underlying the buildup and decay of dynamical nuclear spin polarization in a single semiconductor quantum dot. Our experiment shows that the nuclei can be polarized on a time scale of a few…

Optics · Physics 2007-08-02 P. Maletinsky , A. Badolato , A. Imamoglu

We investigate the dynamic nuclear polarization process by frequently injecting polarized electron spins into a quantum dot. Due to the suppression of the direct dipolar and indirect electron-mediated nuclear spin interactions, by the…

Mesoscale and Nanoscale Physics · Physics 2016-07-26 Na Wu , Wenkui Ding , Anqi Shi , Wenxian Zhang

We study the dynamics of optically-induced nuclear spin polarization in a fluorine-doped ZnSe epilayer via time-resolved Kerr rotation. The nuclear polarization in the vicinity of a fluorine donor is induced by interaction with coherently…

Mesoscale and Nanoscale Physics · Physics 2016-02-24 F. Heisterkamp , E. Kirstein , A. Greilich , E. A. Zhukov , T. Kazimierczuk , D. R. Yakovlev , A. Pawlis , M. Bayer

Sizable nuclear spin polarization is pumped in individual InP/GaInP dots in a wide range of external magnetic fields B_ext=0-5T by circularly polarized optical excitation. We observe nuclear polarization of up to ~40% at Bext=1.5T and…

We employ optical pump-probe spectroscopy to investigate the voltage dependence of spontaneous electron and nuclear spin polarizations in hybrid MnAs/n-GaAs and Fe/n-GaAs Schottky diodes. Through the hyperfine interaction, nuclear spin…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 R. J. Epstein , J. Stephens , M. Hanson , Y. Chye , A. C. Gossard , P. M. Petroff , D. D. Awschalom

We demonstrate all optical electron spin initialization, storage and readout in a single self-assembled InGaAs quantum dot. Using a single dot charge storage device we monitor the relaxation of a single electron over long timescales…

Mesoscale and Nanoscale Physics · Physics 2016-11-25 D. Heiss , V. Jovanov , F. Klotz , D. Rudolph , M. Bichler , G. Abstreiter , M. S. Brandt , J. J. Finley

Photoluminescence polarization is experimentally studied for samples with (In,Ga)As/GaAs selfassembled quantum dots in transverse magnetic field (Hanle effect) under slow modulation of the excitation light polarization from fractions of Hz…

Mesoscale and Nanoscale Physics · Physics 2017-04-26 M. S. Kuznetsova , R. V. Cherbunin , I. Ya. Gerlovin , I. V. Ignatiev , S. Yu. Verbin , D. R. Yakovlev , D. Reuter , A. D. Wieck , M. Bayer

Hyperfine coupling of electron spins to nuclear spins is studied for a GaAs-based double quantum dot in the spin blockade regime where the electron conduction is mostly blocked by Pauli effect unless the electron spin state in the double…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Keiji Ono , Seigo Tarucha

We report the hysteresis of optically-pumped nuclear spin polarization and the degree of circular polarization of photoluminescence on the excitation power and electron spin polarization in single InAlAs quantum dots. By increasing (or…

Materials Science · Physics 2009-11-13 R Kaji , S Adachi , H Sasakura , S Muto

The spin dynamics of positively (X$^{+}$) and negatively (X$^{-}$) charged excitons in InP/In$_{0.48}$Ga$_{0.52}$P quantum dots subject to a magnetic field is studied. We find that a characteristic feature of the system under study is the…

Mesoscale and Nanoscale Physics · Physics 2019-12-18 S. V. Nekrasov , I. A. Akimov , Yu. G. Kusrayev , D. R. Yakovlev , M. Bayer

The interplay of optical driving and hyperfine interaction between an electron confined in a quantum dot and its surrounding nuclear spin environment produces a range of interesting physics such as mode-locking. In this work, we go beyond…

Mesoscale and Nanoscale Physics · Physics 2024-03-12 Arian Vezvaee , Gargee Sharma , Sophia E. Economou , Edwin Barnes

We report optical pumping of neutral quantum dots leading to nuclear spin alignment with direction insensitive to polarization and wavelength of light. Measurements of photoluminescence of both "dark" and "bright" excitons in single dots…

Mesoscale and Nanoscale Physics · Physics 2011-04-05 E. A. Chekhovich , A. B. Krysa , M. S. Skolnick , A. I. Tartakovskii

We demonstrate optical control of the polarization eigenstates of a neutral quantum dot exciton without any external fields. By varying the excitation power of a circularly polarized laser in micro-photoluminescence experiments on…

We fabricated GaAs/AlGaAs quantum dots by droplet epitaxy method, and obtained the geometries of the dots from scanning transmission electron microscopy data. Post-thermal annealing is essential for the optical activation of quantum dots…

Materials Science · Physics 2012-11-15 Pilkyung Moon , J. D. Lee , S. K. Ha , E. H. Lee , W. J. Choi , J. D. Song , J. S. Kim , L. S. Dang

We find that detuning an optical pulse train from electronic transitions in quantum dots controls the direction of nuclear spin flips. The optical pulse train generates electron spins that precess about an applied magnetic field, with a…

Quantum Physics · Physics 2015-05-13 S. G. Carter , A. Shabaev , Sophia E. Economou , T. A. Kennedy , A. S. Bracker , T. L. Reinecke