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Related papers: Dissecting the hydrogen bond: a Quantum Monte Carl…

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Geometric configuration and energy of a hydrogen molecule centered between two point-shaped tips of equal charge are calculated with the variational quantum Monte-Carlo (QMC) method without the restriction of the Born-Oppenheimer (BO)…

Mesoscale and Nanoscale Physics · Physics 2020-05-29 W. Schattke , T. Frederiksen , M. A. Van Hove , R. Díez Muiño

An antiferromagnetic Heisenberg model on a 1/5-depleted two-dimensional square-lattice, a model of CaV$_4$O$_9$, is investigated by variational Monte Carlo simulation. A prototype of a trial wave function is made by projecting out the…

Condensed Matter · Physics 2009-10-28 T. Miyazaki , D. Yoshioka

The variational Monte Carlo method is used to evaluate the ground-state energy of the confined hydrogen molecule, H_2. Accordingly, we considered the case of hydrogen molecule confined by a hard prolate spheroidal cavity when the nuclear…

Atomic and Molecular Clusters · Physics 2015-09-10 S. B. Doma , F. N. El-Gammal , A. A. Amer

The physical nature of a frequency shift of hydrogen valence vibrations in a water molecule due to its interaction with neighbor molecules has been studied. Electrostatic forces connected with the multipole moments of molecules are supposed…

Chemical Physics · Physics 2017-05-02 I. V. Zhyganiuk , M. P. Malomuzh

Although liquid water has been studied for many decades by (X-ray and neutron) diffraction measurements, new experimental results keep appearing, virtually every year. The reason for this is that neither X-ray, nor neutron diffraction data…

Soft Condensed Matter · Physics 2016-02-25 Ildikó Pethes , László Pusztai

The work presents the detailed analysis of the water dimer properties. Their parameters are investigated on the basis of a multipole interaction potential extended up to the quadrupole--quadrupole and dipole--octupole terms. All main…

Chemical Physics · Physics 2013-05-02 P. V. Makhlaichuk , M. P. Malomuzh , I. V. Zhyganiuk

We revisit the accuracy of the variational Monte Carlo (VMC) method by taking an example of ground state properties for the one-dimensional Hubbard model. We start from the variational wave functions with the Gutzwiller and long-range…

Strongly Correlated Electrons · Physics 2013-08-13 Ryui Kaneko , Satoshi Morita , Masatoshi Imada

The molecular dissociation energy has often been explained and discussed in terms of singlet bonds, formed by bounded pairs of valence electrons. In this work we use a highly correlated resonating valence bond ansatz, providing a consistent…

Chemical Physics · Physics 2020-09-28 Claudio Genovese , Sandro Sorella

Neural network parametrizations have increasingly been used to represent the ground and excited states in variational Monte Carlo (VMC) with promising results. However, traditional VMC methods only optimize the wave function in regions of…

Computational Physics · Physics 2025-07-03 Huan Zhang , Robert J. Webber , Michael Lindsey , Timothy C. Berkelbach , Jonathan Weare

A theoretical study is reported of the molecular-to-atomic transition in solid hydrogen at high pressure. We use the diffusion quantum Monte Carlo method to calculate the static lattice energies of the competing phases and a…

Materials Science · Physics 2014-04-23 Sam Azadi , Bartomeu Monserrat , W. M. C. Foulkes , R. J. Needs

Square water takes into account the directionality of hydrogen bonds. The model is reviewed and its properties as a solvent for apolar particles are studied through Monte Carlo simulations. Specific heat measurements are used to identify…

Statistical Mechanics · Physics 2007-05-23 Nara Guisoni , Vera Bohomoletz Henriques

We explore the application of Monte Carlo transport methods to solving coupled radiation-hydrodynamics problems. We use a time-dependent, frequency-dependent, 3-dimensional radiation transport code, that is special relativistic and includes…

Instrumentation and Methods for Astrophysics · Physics 2015-06-19 Nathaniel Roth , Daniel Kasen

We present an investigation of vibrational features in water clusters performed by means of our recently established divide-and-conquer semiclassical approach [M. Ceotto, G. Di Liberto, and R. Conte, Phys. Rev. Lett. 119, 010401 (2017)].…

Chemical Physics · Physics 2018-04-05 Giovanni Di Liberto , Riccardo Conte , Michele Ceotto

We extend our low-scaling variational Monte Carlo (VMC) algorithm to optimize the symmetry projected Jastrow mean field (SJMF) wavefunctions. These wavefunctions consist of a symmetry-projected product of a Jastrow and a general…

Strongly Correlated Electrons · Physics 2019-06-19 Ankit Mahajan , Sandeep Sharma

The accuracy and efficiency of ab-initio quantum Monte Carlo (QMC) algorithms benefits greatly from compact variational trial wave functions that accurately reproduce ground state properties of a system. We investigate the possibility of…

Materials Science · Physics 2019-01-30 Shivesh Pathak , Lucas K. Wagner

We review a recent approach for the simulation of many-body interacting systems based on an efficient generalization of the Lanczos method for Quantum Monte Carlo simulations. This technique allows to perform systematic corrections to a…

Strongly Correlated Electrons · Physics 2007-05-23 Sandro Sorella

The three-band \emph{d-p} model is investigated by means of Variational Monte-Carlo (VMC) method with the BCS-like wave-function supplemented by the Gutzwiller and Jastrow correlators. The VMC optimization leads to $d$-$wave$…

Superconductivity · Physics 2020-06-08 A. Biborski , M. Zegrodnik , J. Spalek

Fixed node diffusion Monte Carlo (DMC) has been performed on a test set of forward and reverse barrier heights for 19 non-hydrogen-transfer reactions, and the nodal error has been assessed. The DMC results are robust to changes in the nodal…

Chemical Physics · Physics 2017-04-26 Kittithat Krongchon , Brian Busemeyer , Lucas K. Wagner

Fermionic cold atoms in optical traps provide viable quantum simulators of correlation effects in electronic systems. For dressed Rydberg atoms in two-dimensional traps with out-of-plane dipole moments, a realistic model of the pairwise…

Quantum Gases · Physics 2026-01-13 Clio Johnson , Neil D. Drummond , James P. Hague , Calum MacCormick

A discrete multistate kinetic model for water-wire proton transport is constructed and analyzed using Monte-Carlo simulations. The model allows for each water molecule to be in one of three states: oxygen lone pairs pointing leftward,…

Soft Condensed Matter · Physics 2009-11-10 Tom Chou