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The evolution of porous structure and mechanical properties of binary glasses under tensile loading were examined using molecular dynamics simulations. We consider vitreous systems obtained in the process of phase separation after a rapid…

Soft Condensed Matter · Physics 2018-07-19 Nikolai V. Priezjev , Maxim A. Makeev

We report the first large scale molecular dynamics simulations of the effect of the photoisomerization of probe molecules on the dynamics of a glassy molecular material. We show that the photoisomerization of the probe molecules induces the…

Soft Condensed Matter · Physics 2009-12-22 V. Teboul , M. Saiddine , J-M. Nunzi

Experimentally resolving atomic-scale structural changes of a deformed glass remains challenging owing to the disordered nature of glass structure. Here, we show that the structural anisotropy emerges as a general hallmark for different…

We use molecular dynamics computer simulations to study the equilibrium properties of the surface of amorphous silica. Two types of geometries are investigated: i) clusters with different diameters (13.5\AA, 19\AA, and 26.5\AA) and ii) a…

Statistical Mechanics · Physics 2009-10-31 Alexandra Roder , Walter Kob , Kurt Binder

In $e$-beam evaporated amorphous silicon ($a$-Si), the densities of two-level systems (TLS), $n_{0}$ and $\overline{P}$, determined from specific heat $C$ and internal friction $Q^{-1}$ measurements, respectively, have been shown to vary by…

Disordered Systems and Neural Networks · Physics 2020-11-17 D. R. Queen , X. Liu , J. Karel , H. C. Jacks , T. H. Metcalf , F. Hellman

The application of amorphous chalcogenide alloys as data-storage media relies on their ability to undergo an extremely fast (10-100 ns) crystallisation once heated at sufficiently high temperature. However, the peculiar features that make…

Disordered Systems and Neural Networks · Physics 2015-06-05 Gabriele C. Sosso , Joerg Behler , Marco Bernasconi

The results of RHEED, FTIR and Raman spectroscopy study of silicon and germanium films with the thickness up to 200 nm grown from molecular beams on dielectric Si$_3$N$_4$/SiO$_2$/Si(001) substrates are presented. Noticeable changes of the…

Indentation has been widely used for investigating the mechanical behavior of glasses. However, how the various microscopic properties (such as atomic structure and mechanics) of glass evolve from the immediate contact with the indenter to…

Disordered Systems and Neural Networks · Physics 2023-05-09 Linfeng Ding , Ranran Lu , Lianjun Wang , Qiuju Zheng , John C. Mauro , Zhen Zhang

Molecular dynamics computer simulations are used to investigate a silica melt confined between walls at equilibrium and in a steady-state Poisseuille flow. The walls consist of point particles forming a rigid face-centered cubic lattice and…

Statistical Mechanics · Physics 2009-11-07 Juergen Horbach , Kurt Binder

The time evolution of the pore size distributions and mechanical properties of amorphous solids at constant pressure is studied using molecular dynamics simulations. The porous glasses were initially prepared at constant volume conditions…

Soft Condensed Matter · Physics 2018-10-22 Nikolai V. Priezjev , Maxim A. Makeev

The optical properties of inhomogeneous cerium dioxide (CeO2) films on aluminum (Al) sublayer are investigated. The dependencies of the reflection, scattering, and absorption of coherent electromagnetic radiation as functions of the…

We study a calcium aluminosilicate glass of composition (SiO$_2$)$_{0.67}$-(Al$_2$O$_3$)$_{0.12}$-(CaO)$_{0.21}$ by means of molecular-dynamics (MD) simulations, using a potential made of two-body and three-body interactions. In order to…

Disordered Systems and Neural Networks · Physics 2009-11-10 Patrick Ganster , Magali Benoit , Walter Kob , Jean-Marc Delaye

X-ray photon correlation is used to probe the slow dynamics of the glass-former B2O3 across the glass transition. In the undercooled liquid phase the decay times of the measured correlation functions are consistent with visible light…

Disordered Systems and Neural Networks · Physics 2019-07-03 Giovanna Pintori , Giacomo Baldi , Beatrice Ruta , Giulio Monaco

The structure-property relation of nanostructured Al-doped ZnO thin films has been investigated in detail through a systematic variation of structure and morphology, with particular emphasis on how they affect optical and electrical…

Materials Science · Physics 2013-11-28 P. Gondoni , M. Ghidelli , F. Di Fonzo , M. Carminati , V. Russo , A. Li Bassi , C. S. Casari

As-deposited and unencapsulated GeSe$_{1-x}$Te$_x$ ($x = 0, 0.25$) 3-$\mu$m-thick amorphous films on Si(001) were obtained via the co-evaporation technique to study the effect of selenium (Se) substitution for tellurium (Te) on the GeSe…

Materials Science · Physics 2025-01-22 P. Armand , R. Escalier , G. Silly , J. Lizion , A. Piarristeguy

The evolution of the atomic structures of the combinatorial library of Sm-substituted thin film BiFeO3 along the phase transition boundary from the ferroelectric rhombohedral phase to the non-ferroelectric orthorhombic phase is explored…

Data Analysis, Statistics and Probability · Physics 2021-03-03 Chris Nelson , Anna N. Morozovska , Maxim A. Ziatdinov , Eugene A. Eliseev , Xiaohang Zhang , Ichiro Takeuchi , Sergei V. Kalinin

We deposit intrinsic hydrogenated amorphous silicon (a-Si:H) thin films by reactive pulsed laser deposition, for various hydrogen pressures in the 0-20 Pa range, at a low deposition temperature of 120C, and investigate the hydrogen…

Materials Science · Physics 2017-04-17 A. Mellos , M. Kandyla , D. Palles , M. Kompitsas

We study the statistical mechanics of a closed random manifold of fixed area and fluctuating volume, encapsulating a fixed number of noninteracting particles. Scaling analysis yields a unified description of such swollen manifolds,…

Soft Condensed Matter · Physics 2008-08-24 Emir Haleva , Haim Diamant

Atomistic simulations are used to explore the effect of interfacial structure on residual radiation damage. Specifically, an ordered grain boundary is compared to a disordered amorphous intergranular film, to investigate how interface…

Materials Science · Physics 2015-07-31 Joseph E. Ludy , Timothy J. Rupert

A structure of germanium selenide glasses is simulated by the featured clusters built from the tetrahedral GeSe4 units up to the clusters with six germanium atoms (Ge6Se16H4 and Ge6Se16H8). Quantum chemical calculations at the DFT level…

Materials Science · Physics 2017-08-23 V. Gurin , O. Shpotyuk , V. Boyko