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The present work reports the preparation of polycrystalline multiferroic $GdFeO_3$ (GdFO) and characterization with x-ray diffraction (XRD), magnetization, temperature dependent Raman spectroscopy, temperature and magnetic field dependent…

Materials Science · Physics 2021-12-06 Anjali Panchwanee , V. Raghavendra Reddy , Ajay Gupta , V. G. Sathe

In many multiferroics, rare-earth and transition-metal orders exist side by side. For analyzing their interaction and its consequences for the multiferroic state, the associated domain patterns and their spatial correlation can give…

Inelastic neutron scattering experiments combining time-of-flight and polarized techniques yield a comprehensive picture of the magnon dispersion in multiferroic TbMnO3 including the dynamic chirality. Taking into account only Mn3+ moments,…

Strongly Correlated Electrons · Physics 2024-02-27 S. Holbein , P. Steffens , S. Biesenkamp , J. Ollivier , A. C. Komarek , M. Baum , M. Braden

We model changes of magnetic ordering in Mn-antiperovskite nitrides driven by biaxial lattice strain at zero and at finite temperature. We employ a non-collinear spin-polarised density functional theory to compare the response of the…

Strongly Correlated Electrons · Physics 2017-06-07 J. Zemen , E. Mendive Tapia , Z. Gercsi , R. Banerjee , C. E. Patrick , J. B. Staunton , K. G. Sandeman

We study the electronic and magnetic structures of multiferroic CaMn$_7$O$_{12}$ by first-principle calculations, based on the experimentally determined modulated crystal structure. We confirm the presence of a 3$d$ orbital modulation of…

Materials Science · Physics 2015-06-23 Kun Cao , Roger D. Johnson , Natasha Perks , Feliciano Giustino , Paolo G. Radaelli

We shall discuss magnetization and transport measurements in materials exhibiting a broad first-order transition. The phase transitions would be caused by varying magnetic field as well as by varying temperature, and we concentrate on…

Strongly Correlated Electrons · Physics 2009-11-11 P. Chaddah

X-ray magnetic circular and linear dichroism (XMCD and XMLD) have been used to investigate the Fe magnetic response during the spin reorientation transition (SRT) in TmFeO3. These experiments are complemented with resonant magnetic…

The electric-field dependence of the magnetic structure of multiferroic MnWO4 has been investigated using spherical neutron polarimetry as a function of temperature. The application of an electric field drives the magnetic structure to a…

Materials Science · Physics 2009-07-10 A Poole , A S Wills , P J Brown

The multiferroic properties of EuTiO3 are greatly enhanced when a sample is strained, signifying that coupling between strain and structural, magnetic or ferroelectric order parameters is extremely important. Here resonant ultrasound…

Materials Science · Physics 2015-03-19 J. Schiemer , L. J. Spalek , S. S. Saxena , C. Panagopoulos , T. Katsufuji , M. A. Carpenter

To sum up, we show in the present paper that magnetic response in Nb$_2$O$_2$F$_3$ at the high-temperatures ($T>$90 K) is related to the orbital selective regime, when part of the electrons form molecular orbitals while other electrons have…

Materials Science · Physics 2017-05-24 V. V. Gapontsev , D. I. Khomskii , S. V. Streltsov

Magnetic and magnetoelectric excitations in the multiferroic TbMnO_3 have been investigated at terahertz frequencies. Using different experimental geometries we can clearly separate the electro-active excitations (electromagnons) from the…

Strongly Correlated Electrons · Physics 2009-03-16 A. Pimenov , A. Shuvaev , A. Loidl , F. Schrettle , A. A. Mukhin , V. D. Travkin , V. Yu. Ivanov , A. M. Balbashov

We use ab initio electronic structure calculations within the generalized gradient approximation (GGA+U) to density functional theory (DFT) to determine the microscopic exchange interactions in the series of orthorhombic rare-earth…

Materials Science · Physics 2015-04-22 Natalya S. Fedorova , Claude Ederer , Nicola A. Spaldin , Andrea Scaramucci

We have investigated the dielectric anomalies associated with spin ordering transitions in the tetragonal spinel Mn$_3$O$_4$, using thermodynamic, magnetic, and dielectric measurements. We find that two of the three magnetic ordering…

Materials Science · Physics 2007-10-16 R. Tackett , G. Lawes , B. C. Melot , M. Grossman , E. S. Toberer , R. Seshadri

We present a detailed study of magnetization, resistivity, heat capacity, and X-ray and neutron powder diffraction measurements performed on single crystals of non-stoichiometric CeAuBi$_2$, Au deficiency 18$\%$, a strongly correlated…

The orthovanadate DyVO3 crystal, known to exhibit multiple structural, spin and orbital ordering transitions, is presently investigated on the basis of magnetization, heat capacity, resistivity, dielectric and polarization measurements. Our…

Strongly Correlated Electrons · Physics 2014-07-24 Q. Zhang , K. Singh , C. Simon , L. D. Tung , G. Balakrishnan , V. Hardy

In the effective Ising spin-1/2 antiferromagnetic chain system BaCo$_2$V$_2$O$_8, the magnetic-field influence is highly anisotropic. For magnetic fields along the easy axis $c$, the N\'{e}el order is strongly suppressed already for low…

Strongly Correlated Electrons · Physics 2015-06-15 S. K. Niesen , G. Kolland , M. Seher , O. Breunig , M. Valldor , M. Braden , B. Grenier , T. Lorenz

We discuss a simple phenomenological Landau theory of phase transitions with two coupled single-component order parameters and compare the results with available experimental data. The model corresponds to the case of a ferroic system, in…

Strongly Correlated Electrons · Physics 2011-03-30 Olga Howczak , Jozef Spalek

Our measured dielectric constant and mechanical response of multiferroic BiFeO3 indicate four phase transitions below room temperature. Features correlate with those reported at 50K (from a peak in the zero-field-cooled magnetic…

Materials Science · Physics 2008-06-23 S. A. T. Redfern , C. Wang , J. W. Hong , G. Catalan , J. F. Scott

The complete irreducible co-representations of the paramagnetic space group provide a simple and direct path to explore the symmetry restrictions of magnetically driven ferroelectricity. The method consists of a straightforward…

Materials Science · Physics 2015-05-14 J. L. Ribeiro

We report an unusual canted magnetism due to 3d and 4f electrons, occupying two different crystallographic sites, with its consequence to electric dipole order. This is based on neutron powder diffraction measurements on Tb2BaNiO5…