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We employ collisions of individual atomic cesium (Cs) impurities with an ultracold rubidium (Rb) gas to probe atomic interaction with hyperfine- and Zeeman-state sensitivity. Controlling the Rb bath's internal state yields access to novel…

We explore the rich internal structure of Cs_2 Feshbach molecules. Pure ultracold molecular samples are prepared in a CO_2-laser trap, and a multitude of weakly bound states is populated by elaborate magnetic-field ramping techniques. Our…

Other Condensed Matter · Physics 2009-09-29 M. Mark , F. Ferlaino , S. Knoop , J. G. Danzl , T. Kraemer , C. Chin , H. -C. Naegerl , R. Grimm

We present a new, mathematically rigorous, method suitable for bound state and scattering processes calculations for various three atomic or molecular systems where the underlying forces are of a hard-core nature. We employed this method to…

Chemical Physics · Physics 2007-05-23 E. A. Kolganova , A. K. Motovilov , S. A. Sofianos

We show that the interaction of polar alkali dimers in the quintet spin state leads to the formation of a deeply bound reaction complex. The reaction complex can decompose adiabatically into homonuclear alkali dimers (for all molecules…

Atomic Physics · Physics 2013-11-22 Michał Tomza , Kirk W. Madison , Robert Moszynski , Roman V. Krems

The ground electronic, vibrational and rotational state of the OH molecule is currently of interest as it can be manipulated by electric and magnetic fields for experimental studies in ultracold chemistry and quantum degeneracy. Based on…

Quantum Physics · Physics 2015-06-17 N. Cawley , Z. Howard , M. Kleinert , M. Bhattacharya

We investigate theoretically the combination of first-order quadrupole-quadrupole and second-order dipole-dipole effects on the long-range electrostatic interactions between a ground-state homonuclear alkali-metal dimer and an excited…

Quantum Physics · Physics 2017-04-19 Maxence Lepers , Olivier Dulieu

We report the observation of cold Cs Rydberg atom molecules bound at internuclear separations of R~3-9 um. The bound states result from avoided crossings between Rydberg atom pair interaction potentials in an applied electric field. The…

Ab initio quantum chemistry calculations are performed for the mixed alkali triatomic system. Global minima of the ground and first excited doublet states of the trimer are found and Born-Oppenheimer potential energy surfaces of the Li atom…

Chemical Physics · Physics 2018-03-14 Patryk Jasik , Tymon Kilich , Jan Kozicki , Józef E. Sienkiewicz

We have observed and located more than 60 magnetic field-induced Feshbach resonances in ultracold collisions of ground-state $^{133}$Cs atoms. These resonances are associated with molecular states with up to four units of rotational angular…

Soft Condensed Matter · Physics 2007-05-23 Cheng Chin , Vladan Vuletic , Andrew J. Kerman , Steven Chu , Eite Tiesinga , Paul J. Leo , Carl J. Williams

The non-crossing rule for the energy levels of a parameter-dependent Hamiltonian is revisited and a flaw in a commonly accepted proof is revealed. Some aspects of avoided crossings are illustrated by means of simple models. One of them…

Quantum Physics · Physics 2015-04-22 Francisco M. Fernández

In weakly bound diatomic molecules, energy levels are closely spaced and thus more susceptible to mixing by magnetic fields than in the constituent atoms. We use this effect to control the strengths of forbidden optical transitions in…

Atomic Physics · Physics 2015-12-22 B. H. McGuyer , M. McDonald , G. Z. Iwata , W. Skomorowski , R. Moszynski , T. Zelevinsky

We investigate the energy levels of heteronuclear alkali metal dimers in levels correlating with the lowest rotational level of the ground electronic state, which are important in efforts to produce ground-state ultracold molecules. We use…

Atomic Physics · Physics 2009-11-13 J. Aldegunde , Ben A. Rivington , Piotr S. Żuchowski , Jeremy M. Hutson

We report our experimental results on the collisional physics between non-S-state atoms (ytterbium (Yb), effectively a two-electron system, in the metastable ${}^3\mathrm{P}_2$ state) and S-state atoms (lithium (Li), an alkali metal, in the…

Ultracold temperatures in dilute quantum gases opened the way to an exquisite control of matter at the quantum level. Here we focus on the control of ultracold atomic collisions using a laser to engineer their interactions at large…

Quantum Gases · Physics 2022-02-23 T. Xie , A. Orbán , X. Xing , E. Luc-Koenig , R. Vexiau , O. Dulieu , N. Bouloufa-Maafa

We consider bound states in the continuum (BICs) in low-contrast dielectric gratings (DGs). It is demonstrated that the BICs originate from the reduced guided modes on the effective dielectric slab with the permittivity equal to the average…

Optics · Physics 2018-11-28 Evgeny N. Bulgakov , Dmitrii N. Maksimov

We show theoretically that it is possible to create and manipulate a pair of bound states in continuum in ultracold atoms by two lasers in the presence of a magnetically tunable Feshbach resonance. These bound states are formed due to…

Atomic and Molecular Clusters · Physics 2016-09-15 Bimalendu Deb , G. S. Agarwal

We show that the integral cross sections for state-to-state quantum scattering of cold molecules in a magnetic field can be efficiently computed using the total angular momentum representation despite the presence of unphysical Zeeman…

Chemical Physics · Physics 2022-02-02 Suyesh Koyu , Rebekah Hermsmeier , Timur V. Tscherbul

Using a non-selective broadband detection scheme we discovered an efficient mechanism of formation of ultracold Cs$_2$ molecules in deeply bound levels ($v=1-9$) of their electronic ground state X$^1 \Sigma_g^+$. They are formed by a…

We report on the realization of a time-domain `St\"uckelberg interferometer', which is based on the internal state structure of ultracold Feshbach molecules. Two subsequent passages through a weak avoided crossing between two different…

Other Condensed Matter · Physics 2007-09-24 M. Mark , T. Kraemer , P. Waldburger , J. Herbig , C. Chin , H. -C. Naegerl , R. Grimm

This work presents a perturbative calculation methodology for evaluating the energy shifts and broadening of vibrational energy levels, caused by interactions between bound and unbound dissociative electronic states. The method is validated…

Atomic Physics · Physics 2025-04-16 Laiz R. Ventura , Ramon S. da Silva , Sergio R. Souza , Jayr Amorim , Carlos E. Fellows
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