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We predict that it is possible to cool rotational, vibrational and translational degrees of freedom of molecules by coupling a molecular dipole transition to an optical cavity. The dynamics is numerically simulated for a realistic set of…

Quantum Physics · Physics 2007-08-13 Giovanna Morigi , Pepijn W. H. Pinkse , Markus Kowalewski , Regina de Vivie-Riedle

We study the origin of the cold molecular clumps in quasar outflows, recently detected in CO and HCN emission. We first describe the physical properties of such radiation-driven outflows and show that a transition from a momentum- to an…

Astrophysics of Galaxies · Physics 2016-12-14 Andrea Ferrara , Evan Scannapieco

We report the creation and characterization of a near quantum-degenerate gas of polar $^{40}$K-$^{87}$Rb molecules in their absolute rovibrational ground state. Starting from weakly bound heteronuclear KRb Feshbach molecules, we implement…

We use two-dimensional transverse laser cooling to produce an ultracold beam of YbF molecules. Through experiments and numerical simulations, we study how the cooling is influenced by the polarization configuration, laser intensity, laser…

We present a novel cooling method that uses the phase separation and evaporative cooling of 3He to reach and continuously maintain sub-kelvin temperatures. While less complex than a dilution refrigerator, the system performs similarly to a…

Other Condensed Matter · Physics 2025-03-17 P. H. Kim , M. Hirschel , J. Suranyi , J. P. Davis

We demonstrate significantly improved magneto-optical trapping of molecules using a very slow cryogenic beam source and RF modulated and DC magnetic fields. The RF MOT confines $1.1(3) \times 10^5$ CaF molecules at a density of $4(1) \times…

We discuss the possibility of trapping polar molecules in the standing-wave electromagnetic field of a microwave resonant cavity. Such a trap has several novel features that make it very attractive for the development of ultracold molecule…

Atomic Physics · Physics 2009-11-10 D. DeMille , D. R. Glenn , J. Petricka

Nitric oxide (NO) molecules initially traveling at 795 m/s in pulsed supersonic beams have been photoexcited to long-lived hydrogenic Rydberg-Stark states, decelerated and electrostatically trapped in a cryogenically cooled, chip-based…

Chemical Physics · Physics 2020-09-21 A. Deller , M. H. Rayment , S. D. Hogan

We show that a large class of helium-containing cold polar molecules form readily in a cryogenic buffer gas, achieving densities as high as 10^12 cm^-3. We explore the spin relaxation of these molecules in buffer gas loaded magnetic traps,…

Atomic Physics · Physics 2011-04-29 N. Brahms , T. V. Tscherbul , P. Zhang , J. K los , H. R. Sadeghpour , A. Dalgarno , J. M. Doyle , T. G. Walker

We present the first experimental observation of cold collisions between two different species of neutral polar molecules, each prepared in a single internal quantum state. Combining for the first time the techniques of Stark deceleration,…

Complex Organic Molecules (COMs) are believed to form in the ice mantle of dust grains and are released to the gas by thermal sublimation when grain mantles are heated to temperatures of $T_{\rm d}\gtrsim 100\,\rm K$. However, some COMs are…

Molecular laser cooling and trapping requires addressing all spontaneous decays to excited vibrational states that occur at the $\gtrsim 10^{-4} - 10^{-5}$ level, which is accomplished by driving repumping transitions out of these states.…

Atomic Physics · Physics 2023-06-06 Nickolas H. Pilgram , Arian Jadbabaie , Chandler J. Conn , Nicholas R. Hutzler

We propose an improved photoassociation scheme to produce ultracold molecules in their vibronic ground state for the generic case where non-adiabatic effects facilitating transfer to deeply bound levels are absent. Formation of molecules is…

Atomic Physics · Physics 2008-10-28 Christiane P. Koch , Robert Moszynski

We employ laser cooling to intensify and cool an atomic beam of metastable Ne(3s) atoms. Using several collimators, a slower and a compressor we achieve a ^{20}Ne^* flux of 6 10^{10} atoms/s in an 0.7 mm diameter beam traveling at 100 m/s,…

We present a large sample of H- and K-band spectra of 32 optically line luminous central cluster galaxies. We find significant rovibrational H_2 emission in 23 of these galaxies as well as H recombination and/or [FeII] emission in another…

Astrophysics · Physics 2009-09-17 A. C. Edge , R. J. Wilman , R. M. Johnstone , C. S. Crawford , A. C. Fabian , S. W. Allen

We propose a cooling scheme based on depolarisation of a polarised cloud of trapped atoms. Similar to adiabatic demagnetisation, we suggest to use the coupling between the internal spin reservoir of the cloud and the external kinetic…

Quantum Physics · Physics 2009-11-11 S. Hensler , A. Greiner , J. Stuhler , T. Pfau

The helium dimer in its metastable triplet state is a promising candidate to be the first laser-cooled homonuclear molecule. An ultracold gas of He$_2^*$ would enable a new generation of precision measurements to test quantum…

Atomic Physics · Physics 2025-05-22 Lucía Verdegay , Bingcheng Zeng , Daniel Y. Knapp , Jack C. Roth , Maximilian Beyer

The rich internal structure and long-range dipole-dipole interactions establish polar molecules as unique instruments for quantum-controlled applications and fundamental investigations. Their potential fully unfolds at ultracold…

There is substantial interest in producing samples of ultracold molecules for possible applications in quantum computation, quantum simulation of condensed matter systems, precision measurements, controlled chemistry, and high precision…

Atomic Physics · Physics 2013-05-30 J. F. Barry , E. S. Shuman , E. B. Norrgard , D. DeMille
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