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We have developed and demonstrated a scheme to achieve rotationally-closed photon cycling in polyatomic molecules with complex hyperfine structure and sensitivity to hadronic symmetry violation, specifically $^{171}$YbOH and $^{173}$YbOH.…

While the implementation of single particle coherent diffraction imaging for non-crystalline particles is complicated by current limitations in photon flux, hit rate, and sample delivery a concept of many-particle coherent diffraction…

Disordered Systems and Neural Networks · Physics 2013-02-22 R. P. Kurta , R. Dronyak , M. Altarelli , E. Weckert , I. A. Vartanyants

Optically levitated nanospheres are highly sensitive to the motion of their center of mass even under small momentum transfer. We propose detecting exotic particles via nucleon scattering in such spheres in the context of an ongoing…

High Energy Physics - Phenomenology · Physics 2025-02-04 Bhaskar Dutta , Dilip Kumar Ghosh , Sk Jeesun

Single molecule rotational correlation functions are analyzed for several reorientation geometries. Even for the simplest model of isotropic rotational diffusion our findings predict non-exponential correlation functions to be observed by…

Other Condensed Matter · Physics 2016-08-16 G. Hinze , G. Diezemann , Th. Basché

Scattering can rapidly degrade our ability to form an optical image, to the point where only speckle-like patterns can be measured. Truly non-invasive imaging through a strongly scattering obstacle is difficult, and usually reliant on a…

Optics · Physics 2022-10-26 Y. Jauregui-Sánchez , Harry Penketh , Jacopo Bertolotti

Illumination of colloid sphere monolayers by circularly polarized beams enables the fabrication of concave patterns consisting of circular nanohole miniarrays that can be transferred into convex metal nanoparticle patterns via a lift-off…

Optics · Physics 2020-05-21 Aron Sipos , Emese Toth , Oliver A. Fekete , Maria Csete

Proposals to determine biomolecular structures from diffraction experiments using femtosecond X-ray free-electron laser (XFEL) pulses involve a conflict between the incident brightness required to achieve diffraction-limited atomic…

Optics · Physics 2015-05-19 Harry M. Quiney , Keith A. Nugent

A sparsity-exploiting algorithm intended for few-view Single Photon Emission Computed Tomography (SPECT) reconstruction is proposed and characterized. The algorithm models the object as piecewise constant subject to a blurring operation. To…

Medical Physics · Physics 2012-12-05 Paul A Wolf , Jakob H Jørgensen , Taly G Schmidt , Emil Y Sidky

On the basis of general theoretical results developed previously in [JETP 112, 246 (2011)], we analyze the reflection of quasiresonant light from a plane surface of dense and disordered ensemble of motionless point scatters. Angle…

Atomic Physics · Physics 2016-01-15 A. S. Kuraptsev , I. M. Sokolov

Conventional approaches to control and shape the scattering patterns of light generated by different nanostructures are mostly based on engineering of their electric response due to the fact that most metallic nanostructures support…

Optics · Physics 2014-05-05 Wei Liu , Andrey E. Miroshnichenko , Yuri S. Kivshar

The relative roles of multiple electron scattering and in-molecule free-space propagation in transmission electron microscopy of small molecules are discussed. It is argued that while multiple scattering tends to have only a moderate effect…

Image and Video Processing · Electrical Eng. & Systems 2019-12-02 T. E. Gureyev , H. M. Quiney , A. Kozlov , L. J. Allen

Nanobeam electron diffraction can probe local structural properties of complex crystalline materials including phase, orientation, tilt, strain, and polarization. Ideally, each diffraction pattern from a projected area of a few unit cells…

We numerically study light scattering and absorption in self-similar aggregates of dielectric nanoparticles, as generated by simulated ballistic deposition upon a surface starting from a single seed particle. The resulting structure…

Materials Science · Physics 2015-06-15 Matteo Gerosa , Carlo Enrico Bottani

The current state of the art in structural biology is led by NMR, X-ray crystallography and TEM investigations. These powerful tools however all rely on averaging over a large ensemble of molecules. Here, we present an alternative concept…

Atomic and Molecular Clusters · Physics 2015-12-15 Tatiana Latychevskaia , Jean-Nicolas Longchamp , Conrad Escher , Hans-Werner Fink

The wavefront is scrambled when coherent light propagates through a random scattering medium and which makes direct use of the conventional optical methods ineffective. In this paper, we propose and demonstrate a structured light…

The pathway toward the tailored synthesis of materials starts with precise characterization of the conformational properties and dynamics of individual molecules. Electron spin resonance based scanning tunneling microscopy can potentially…

Modelling the scattering of focused, coherent light by nano-scale structures is oftentimes used to reconstruct or infer geometrical or material properties of structures under investigation in optical scatterometry. This comprises both…

The theoretical formulation of x-ray resonant magnetic scattering from rough surfaces and interfaces is given for specular reflectivity. A general expression is derived for both structurally and magnetically rough interfaces in the…

Materials Science · Physics 2009-11-10 D. R. Lee , D. Haskel , Y. Choi , J. C. Lang , S. A. Stepanov , G. Srajer , S. K. Sinha

We develop the analysis of x-ray intensity correlations from dilute ensembles of identical particles in a number of ways. First, we show that the 3D particle structure can be determined if the particles can be aligned with respect to a…

Data Analysis, Statistics and Probability · Physics 2015-05-28 Veit Elser

We analyze multi-bounce propagation of light in an unknown hidden volume and demonstrate that the reflected light contains sufficient information to recover the 3D structure of the hidden scene. We formulate the forward and inverse theory…

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