Related papers: Quantum Chessboards in the Deuterium Molecular Ion
We report on a search for Interstellar CH2D+. Four transitions occur in easily accessible portions of the spectrum; we report on emission at the frequencies of these transitions toward high column density star-forming regions. While the…
We propose a mechanism to produce a superposition of atomic and molecular states by a train of ultrashort laser pulses combined with weak control fields. By adjusting the repetition rate of the pump pulses and the intensity of the coupling…
We propose an optical control scheme for driving a polar molecule from a high-lying vibrational level to a target low-lying one, within the same electronic state. The scheme utilizes an infrared chirped laser pulse with an analytical shape,…
Ultrafast laser excitation can trigger multiplex coherent dynamics in molecules. Here, we report attosecond transient absorption experiments addressing simultaneous probing of electronic and vibrational dynamics in a prototype molecule,…
There are several important solid-state systems, such as defects in solids, superconducting circuits and molecular qubits, for attractive candidates of quantum computations. Molecular qubits, which benefit from the power of chemistry for…
Quantum phenomena have remained largely inaccessible to the general public. This can be attributed to the fact that we do not experience quantum mechanics on a tangible level in our daily lives. Games can provide an environment in which…
We propose a methodology to design optimal pulses for achieving quantum optimal control on molecular systems. Our approach constrains pulse shapes to linear combinations of a fixed number of experimentally relevant pulse functions. Quantum…
We develop and demonstrate a technique to engineer universal unitary baths in quantum systems. Using the correspondence between unitary decoherence due to ambient environmental noise and errors in a control system for quantum bits, we show…
Molecular vibrations underpin important phenomena such as spectral properties, energy transfer, and molecular bonding. However, obtaining a detailed understanding of the vibrational structure of even small molecules is computationally…
The presence of decoherence in quantum computers necessitates the suppression of noise. Dynamically corrected gates via specially designed control pulses offer a path forward, but hardware-specific experimental constraints can cause…
We propose to use a new platform - ultracold polar molecules - for quantum computing with switchable interactions. The on/off switch is accomplished by selective excitation of one of the "0" or "1" qubits - long-lived molecular states - to…
We introduce a quantum control technique using polychromatic pulse sequences (PPS), consisting of pulses with different carrier frequencies, i.e. different detunings with respect to the qubit transition frequency. We derive numerous PPS,…
Tunnel ionization of room-temperature D$_2$ in an ultrashort (12 femtosecond) near infra-red (800 nm) pump laser pulse excites a vibrational wavepacket in the D2+ ions; a rotational wavepacket is also excited in residual D2 molecules. Both…
Understanding and controlling the electronic as well as ro-vibrational motion and, thus, the entire chemical dynamics in molecules is the ultimate goal of ultrafast laser and imaging science. In photochemistry, laser-induced dissociation…
Quantum process tomography is used to fully characterize the evolution of the quantum vibrational state of atoms. Rubidium atoms are trapped in a shallow optical lattice supporting only two vibrational states, which we charcterize by…
A particular superconducting quantum interference device (SQUID)qubit, indicated as double SQUID qubit, can be manipulated by rapidly modifying its potential with the application of fast flux pulses. In this system we observe coherent…
Quantum systems are powerful detectors with wide-ranging applications from scanning probe microscopy of materials to biomedical imaging. Nitrogen vacancy (NV) centers in diamond, for instance, can be operated as qubits for sensing of…
Classical algorithms for predicting the equilibrium geometry of strongly correlated molecules require expensive wave function methods that become impractical already for few-atom systems. In this work, we introduce a variational quantum…
A theoretical study of the intense-field single ionization of molecular hydrogen or deuterium oriented either parallel or perpendicular to a linear polarized laser pulse (400 nm) is performed for different internuclear separations and pulse…
We describe a method for improving coherent control through the use of detailed knowledge of the system's Hamiltonian. Precise unitary transformations were obtained by strongly modulating the system's dynamics to average out unwanted…