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Environmental molecular beam experiments are used to examine water interactions with liquid methanol films at temperatures from 170 K to 190 K. We find that water molecules with 0.32 eV incident kinetic energy are efficiently trapped by the…

Monolayer 2D semiconductors, such as WS2, exhibit uniquely strong light-matter interactions due to exciton resonances that enable atomically-thin optical elements. Similar to geometry-dependent plasmon and Mie resonances, these intrinsic…

Methanol-water liquid mixtures have been investigated by high-energy synchrotron X-ray and neutron diffraction at low temperatures. We are thus able to report the first complete sets of both X-ray and neutron weighted total scattering…

A description of phase separation kinetics for solid binary (A,B) mixtures in thin film geometry based on the Kawasaki spin-exchange kinetic Ising model is presented in a discrete lattice molecular field formulation. It is shown that the…

Statistical Mechanics · Physics 2009-11-13 Subir K. Das , Jürgen Horbach , Kurt Binder

The molecular dynamics in the ambient-pressure solid phase of (1,1,2)-trichloroethane is studied by means of broadband dielectric spectroscopy and molecular dynamics simulations. The dielectric spectra of polycrystalline samples obtained by…

The relaxation dynamics of many disordered systems, such as structural glasses, proteins, granular materials or spin glasses, is not completely frozen even at very low temperatures. This residual motion leads to a change of the properties…

Soft Condensed Matter · Physics 2009-10-31 Walter Kob , Francesco Sciortino , Piero Tartaglia

We report on an inelastic (Raman) light scattering study of the local structure of amorphous GeTe films. A detailed analysis of the temperature-reduced Raman spectra has shown that appreciable structural changes occur as a function of…

Materials Science · Physics 2009-11-11 K. S. Andrikopoulos , S. N. Yannopoulos , G. A. Voyiatzis , A. V. Kolobov , M. Ribes , J. Tominaga

In the past, light-assisted cold collisions between laser cooled atoms have been widely studied in magneto-optical atom traps (MOTs). We describe here theoretical studies of dynamical interactions, specifically cold collisions, between…

Atomic Physics · Physics 2009-11-10 J. Piilo , K. -A. Suominen

Using molecular dynamics computer simulations we investigate how the glass transition and the properties of the resulting glass depend on the cooling rate with which the sample has been quenched. This is done by studying a two component…

Condensed Matter · Physics 2009-10-28 Katharina Vollmayr , Walter Kob , Kurt Binder

We present the results of a Molecular Dynamics computer simulation of a binary Lennard-Jones liquid confined in a narrow pore. The surface of the pore has an amorphous structure similar to that of the confined liquid. We find that the…

Statistical Mechanics · Physics 2007-05-23 Peter Scheidler , Walter Kob , Kurt Binder

To support a new interpretation of the origin of the dynamic heterogeneity observed pervasively in fragile liquids as they approach their glass transition temperatures Tg, we demonstrate that the introduction of ~2 nm structural…

Disordered Systems and Neural Networks · Physics 2010-12-14 Kazuhide Ueno , C. Austen Angell

Quantifying temperature variations at the micron scale can provide new opportunities in optical sensing. In this paper, we present a novel approach using the temperature-dependent variations in fluorescence of rare-earth doped tellurite…

The scattering of light impacts sensing and communication technologies throughout the electromagnetic spectrum. Overcoming the effects of time-varying scattering media is particularly challenging. In this article we introduce a new way to…

The understanding of dynamics and functioning of biological membranes and in particular of membrane embedded proteins is one of the most fundamental problems and challenges in modern biology and biophysics. In particular the impact of…

Biological Physics · Physics 2009-12-27 Maikel C. Rheinstadter

We describe an optical method to directly measure position-dependent thermal diffusivity of reflective single crystal samples across a broad range of temperatures for condensed matter physics research. Two laser beams are used, one as a…

Point defects in real crystals at finite temperatures are inevitable. Their dynamics severely influence the mechanical properties of crystals under shear giving rise to nonlinear effects such as ductility. Therefore, it is crucial to…

Soft Condensed Matter · Physics 2021-02-02 Gaurav P. Shrivastav , Gerhard Kahl

Employing wide-angle neutron spin echo spectroscopy, we measured the Q-dependent coherent intermediate scattering function of the prototypical ionic glass former Ca0.4K0.6(NO3)1.4, in the equilibrium and supercooled liquid states beyond the…

The viscosity of glass-forming liquids increases by many orders of magnitude if their temperature is lowered by a mere factor of 2-3 [1,2]. Recent studies suggest that this widespread phenomenon is accompanied by spatially heterogeneous…

Disordered Systems and Neural Networks · Physics 2015-05-28 Walter Kob , Sandalo Roldan-Vargas , Ludovic Berthier

We summarize the different puzzles raised by aging experiments of spin-glasses and their various interpretations. We try to reconcile the `real space', droplet like pictures with the hierarchical pictures that have been proposed in the…

Condensed Matter · Physics 2009-11-07 Jean-Philippe Bouchaud , Vincent Dupuis , Jacques Hammannn , Eric Vincent

In this work we give a consistent picture of the thermodynamic properties of bosons in the Mott insulating phase when loaded adiabatically into one-dimensional optical lattices. We find a crucial dependence of the temperature in the optical…

Statistical Mechanics · Physics 2009-11-11 K. P. Schmidt , A. Reischl , G. S. Uhrig