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Using pulsed optically detected magnetic resonance techniques, we directly probe electron-spin resonance transitions in the excited-state of single Nitrogen-Vacancy color centers in diamond. Unambiguous assignment of excited state fine…

Optical and microwave double resonance techniques are used to obtain the excited state structure of single nitrogen-vacancy centers in diamond. The excited state is an orbital doublet and it is shown that it can be split and associated…

The ground state spin of the negatively charged nitrogen-vacancy center in diamond has been the platform for the recent rapid expansion of new frontiers in quantum metrology and solid state quantum information processing. In ambient…

Materials Science · Physics 2012-06-05 M. W. Doherty , F. Dolde , H. Fedder , F. Jelezko , J. Wrachtrup , N. B. Manson , L. C. L. Hollenberg

The emission intensity of diamond samples containing nitrogen-vacancy centres are measured as a function of magnetic field along a <111> direction for various temperatures. At low temperatures the responses are sample and stress dependent…

Materials Science · Physics 2009-06-04 L J Rogers , R L McMurtrie , S Armstrong , M J Sellars , N B Manson

We discuss the side resonances of optically detected magnetic resonance in diamond crystal and propose the new approach to the calculation of hyperfine interaction in composed system, consisted of negatively charged nitrogen-vacancy NV-…

Mesoscale and Nanoscale Physics · Physics 2017-01-17 Alexander Ivanov , Alexei Ivanov

Precise knowledge of a quantum system's Hamiltonian is a critical pre-requisite for its use in many quantum information technologies. Here, we report a method for the precise characterization of the non-secular part of the excited-state…

Quantum Physics · Physics 2017-06-20 F. Poggiali , P. Cappellaro , N. Fabbri

Colour centres in diamond have emerged as versatile tools for solid-state quantum technologies ranging from quantum information to metrology, where the nitrogen-vacancy centre is the most studied to-date. Recently, this toolbox has expanded…

Elucidation of the mechanism for optical spin initialization of point defects in solids in the context of quantum applications requires an accurate description of the excited electronic states involved. While variational density functional…

Materials Science · Physics 2023-07-14 Aleksei V. Ivanov , Yorick L. A. Schmerwitz , Gianluca Levi , Hannes Jónsson

The interaction of solid-state electronic spins with deformations of their host crystal is an important ingredient in many experiments realizing quantum information processing schemes. Here, we theoretically characterize that interaction…

Mesoscale and Nanoscale Physics · Physics 2018-08-08 Péter Udvarhelyi , Vladyslav O. Shkolnikov , Adam Gali , Guido Burkard , András Pályi

We propose a high efficiency high fidelity measurement of the ground state spin of a single NV center in diamond, using the effects of cavity quantum electrodynamics. The scheme we propose is based in the one dimensional atom or Purcell…

Quantum Physics · Physics 2015-03-13 A. Young , C. Y. Hu , L. Marseglia , J. P. Harrison , J. L. O'Brien , J. G. Rarity

We investigate phonon induced electronic dynamics in the ground and excited states of the negatively charged silicon-vacancy ($\mathrm{SiV}^-$) centre in diamond. Optical transition line widths, transition wavelength and excited state…

The nitrogen-vacancy (NV) center in diamond is well known in quantum metrology and quantum information for its favorable spin and optical properties, which span a wide temperature range from near zero to over 600 K. Despite its prominence,…

Mesoscale and Nanoscale Physics · Physics 2023-09-01 Stefan Ernst , Patrick J. Scheidegger , Simon Diesch , Christian L. Degen

We examine the quantum spin state of a single nitrogen-vacancy (NV) center in diamond at room temperature as it makes a transition from the orbital ground-state (GS) to the orbital excited-state (ES) during non-resonant optical excitation.…

Quantum Physics · Physics 2015-06-03 G. D. Fuchs , A. L. Falk , V. V. Dobrovitski , D. D. Awschalom

Magnetic resonance techniques provide a powerful tool for controlling spin systems, with applications ranging from quantum information processing to medical imaging. Nevertheless, the behavior of a spin system under strong excitation…

Quantum Physics · Physics 2015-05-19 Lilian Childress , Jean McIntyre

We report on measurements of the photoluminescence (PL) properties of single nitrogen-vacancy (NV) centers in diamond at temperatures between 4-300 K. We observe a strong reduction of the PL intensity and spin contrast between ca. 10-100 K…

Mesoscale and Nanoscale Physics · Physics 2023-09-01 Stefan Ernst , Patrick J. Scheidegger , Simon Diesch , Luca Lorenzelli , Christian L. Degen

We used optically detected magnetic resonance (ODMR) technique to directly probe electron-spin resonance transitions in the excited state of negatively-charged boron vacancy (VB-) defects in hexagonal boron nitride (hBN) at room…

We report a study of the 3E excited-state structure of single nitrogen-vacancy (NV) defects in diamond, combining resonant excitation at cryogenic temperatures and optically detected magnetic resonance. A theoretical model of the…

We report a study of high-resolution microwave spectroscopy of nitrogen-vacancy centers in diamond crystals at and around zero magnetic field. We observe characteristic splitting and transition imbalance of the hyperfine transitions, which…

The excited electronic states involved in the optical cycle preparation of a pure spin state of the negatively charged NV-defect in diamond are calculated using the HSE06 hybrid density functional and variational optimization of the…

Materials Science · Physics 2025-10-29 Lei Sun , Elvar Örn Jónsson , Aleksei Ivanov , Ji Chen , Hannes Jónsson

The ground state spin of the negatively charged nitrogen-vacancy center in diamond has many exciting applications in quantum metrology and solid state quantum information processing, including magnetometry, electrometry, quantum memory and…

Materials Science · Physics 2012-06-05 M. W. Doherty , F. Dolde , H. Fedder , F. Jelezko , J. Wrachtrup , N. B. Manson , L. C. L. Hollenberg
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