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Relaxation dynamics of embedded metal nanoparticles after ultrafast laser pulse excitation is driven by thermal phenomena of different origins the accurate description of which is crucial for interpreting experimental results: hot electron…

Materials Science · Physics 2009-11-13 Majid Rashidi-Huyeh , Sebastian Volz , Bruno Palpant

The femtosecond evolution of the electronic temperature of laser-excited gold nanoparticles is measured, by means of ultrafast time-resolved photoemission spectroscopy induced by extreme-ultraviolet radiation pulses. The temperature of the…

We explore the influence of the nanoporous structure on the thermal relaxation of electrons and holes excited by ultrashort laser pulses ($\sim 7$ fs) in thin gold films. Plasmon decay into hot electron-hole pairs results in the generation…

Ultrafast laser material processing has received significant attention due to a growing need for the fabrication of miniaturized devices at micro- and nanoscales. The traditional phenomenological laws, such as Fourier's law of heat…

Computational Physics · Physics 2015-11-12 Yuwen Zhang , D. Y. Tzou , J. K. Chen

Core-shell nanoparticles, particularly those having a gold core, have emerged as a highly promising class of materials due to their unique optical and thermal properties, which underpin a wide range of applications in photothermal therapy,…

Computational Physics · Physics 2025-06-06 Julien El Hajj , Gilles Ledoux , Samy Merabia

A method is proposed for determining the temperature of hot electrons in a metallic nanoparticle embedded in a dielectric matrix under ultrashort laser pulses irradiation. The amplitude and power of the longitudinal spherical acoustic…

Mesoscale and Nanoscale Physics · Physics 2017-12-15 N. I. Grigorchuk

Transient absorption spectroscopy is routinely used to study the electron dynamics in plasmonic gold nanoparticles. Typically, the transient absorption bleach is analyzed as measure for the electron temperature. However, the implicitly…

Mesoscale and Nanoscale Physics · Physics 2026-03-30 Nour E. H. Chetoui , Jonas Grumm , Robert Lemke , Andreas Knorr , Holger Lange

Efficient mixing and pumping of liquids at the microscale is a technology that is still to be optimized. The combination of an AC electric field with a small temperature gradient leads to a strong electro-thermal flow that can be used for…

Fluid Dynamics · Physics 2024-03-18 Carlos David González Gómez , Raúl A. Rica , Emilio Ruiz-Reina

The structural evolution of laser-excited systems of gold has previously been measured through ultrafast MeV electron diffraction. However, there has been a long-standing inability of atomistic simulations to provide a consistent picture of…

Materials Science · Physics 2024-06-19 J. M. Molina , T. G. White

We investigate melting and undercooling in nanoscale (radius ~100 nm) gold particles that are levitated in a quadrupole ion (Paul) trap in a high vacuum environment. The particle is heated via laser illumination and probed using two main…

Mesoscale and Nanoscale Physics · Physics 2022-01-27 Joyce Coppock , Quinn Waxter , Robert Wolle , B. E. Kane

We propose a new approach to understand the time-dependent temperature increasing process of gold-silica core-shell nanoparticles injected into chicken tissues under near-infrared laser irradiation. Gold nanoshells strongly absorb…

Mesoscale and Nanoscale Physics · Physics 2018-04-04 Vu T. T. Duong , Anh D. Phan , Nghiem T. H. Lien , Do T. Hue , Do Q. Hoa , Do T. Nga , Tran H. Nhung , Nguyen A. Viet

In this paper, we present a simple and robust numerical method able to predict, with high accuracy, the photo-thermal effects occurring for a gold nanoparticles arrangement under externally applied strain. The physical system is numerically…

Applied Physics · Physics 2020-09-08 Giuseppe E. Lio , Giovanna Palermo , Antonio De Luca , Roberto Caputo

Photoexcitation of metallic nanostructures with short optical pulses can drive non-thermal electronic states, which, upon decay, lead to elevated electronic temperatures ($T_e \gtrapprox 1000\,\mathrm{K}$) eventually equilibrating with the…

Mesoscale and Nanoscale Physics · Physics 2025-01-07 Qian Ye , Stephen K. Sanders , Andrea Schirato , Alessandro Alabastri

A sample-based stochastic model is presented to investigate the effects of uncertainties of various input parameters, including laser fluence, laser pulse duration, thermal conductivity constants for electron, and electron-lattice coupling…

Computational Physics · Physics 2016-04-28 Nazia Afrin , Yuwen Zhang , J. K. Chen

The ultrafast laser-induced solid-liquid phase transition in metals is still not clearly understood and its accurate quantitative description remains a challenge. Here we systematically investigated, both experimentally and theoretically,…

The work is dedicated to the development of the electron-lattice energy exchange theory in metal particles and it dependence of on particle size and electron temperature. We obtained the expressions for the constants of the electron-lattice…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Petro Tomchuk , Yevgen Bilotsky

The thermal dynamics induced by ultrashort laser pulses in nanoscale systems, i.e. all-optical time-resolved nanocalorimetry is theoretically investigated from 300 to 1.5 K. We report ab-initio calculations describing the temperature…

Mesoscale and Nanoscale Physics · Physics 2015-03-13 F. Banfi , F. Pressacco , B. Revaz , C. Giannetti , D. Nardi , G. Ferrini , F. Parmigiani

The electrons and phonons in metal films after ultra-short pulse laser heating are in highly non-equilibrium states not only between the electron sub-system and the phonon sub-system but also within the electron sub-system. An…

Materials Science · Physics 2014-08-05 Jun Zhou , Nianbei Li , Ronggui Yang

The simulation and analysis of the thermal stability of nanoparticles, a stepping stone towards their application in technological devices, require fast and accurate force fields, in conjunction with effective characterisation methods. In…

The radiative heat transfer between gold nanoparticle layers is presented using the coupled dipole method. Gold nanoparticles are modelled as effective electric and magnetic dipoles interacting via electromagnetic fluctuations. The effect…

Mesoscale and Nanoscale Physics · Physics 2013-12-05 Anh D. Phan , The-Long Phan , Lilia M. Woods
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