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We formulate a general mean-field theory of a flat electric double layer in ionic liquids and electrolyte solutions with ions possessing static polarizability and a permanent dipole moment on a charged electrode. We establish a new…

Statistical Mechanics · Physics 2021-08-17 Yu. A. Budkov , S. V. Zavarzin , A. L. Kolesnikov

We study $N$-electron atoms with nuclear charge $Z$. It is well known that, in the cationic ($Z > N$) high-$Z$ region, the atom behaves as a weakly interacting system. The anionic ($Z < N$) regime, on the other hand, is characterized by an…

Atomic Physics · Physics 2017-10-20 G. Gil , A. Gonzalez

The reduced 1D Poisson-Nernst-Planck (PNP) model of artificial nanopores in the presence of a permanent charge on the channel wall is studied. More specifically, we consider the limit where the channel length exceed much the Debye screening…

Chemical Physics · Physics 2008-11-23 I. D. Kosińska , I. Goychuk , M. Kostur , G. Schmid , P. Hänggi

We study the large-time asymptotic behavior of solutions to the one-dimensional damped pressureless Euler-Poisson system with variable background states, subject to a neutrality condition. In the case where the background density converges…

Analysis of PDEs · Mathematics 2025-06-10 Young-Pil Choi , Dong-ha Kim , Dowan Koo , Eitan Tadmor

We consider the limit of vanishing Debye length for ionic diffusion in fluids, described by the Nernst-Planck-Navier-Stokes system. In the asymptotically stable cases of blocking (vanishing normal flux) and uniform selective (special…

Analysis of PDEs · Mathematics 2021-09-01 Peter Constantin , Mihaela Ignatova , Fizay-Noah Lee

Understanding how electrolyte-filled porous electrodes respond to an applied potential is important to many electrochemical technologies. Here, we consider a model supercapacitor of two blocking cylindrical pores on either side of a…

Soft Condensed Matter · Physics 2022-04-05 Jie Yang , Mathijs Janssen , Cheng Lian , René van Roij

We consider the Poisson-Boltzmann equation in a periodic cell, representative of a porous medium. It is a model for the electrostatic distribution of $N$ chemical species diluted in a liquid at rest, occupying the pore space with charged…

Analysis of PDEs · Mathematics 2015-04-24 Gregoire Allaire , Jean-Francois Dufreche , Andro Mikelic , Andrey Piatnitski

We study the propagation of surface plasmon polaritons (SPPs) on a metal surface which hosts a thin film of a liquid dielectric. The ohmic losses, that are inherently present due to the coupling of SPPs to conductors' electron plasma,…

Optics · Physics 2018-06-20 Shimon Rubin , Yeshaiahu Fainman

In graphene, where the electron-electron scattering is dominant, electrons collectively act as a fluid. This hydrodynamic behaviour of charge carriers leads to exciting nonlinear phenomena such as solitary waves and shocks, among others. In…

Mesoscale and Nanoscale Physics · Physics 2024-04-12 Pedro Cosme , Hugo Terças

The concept of the partial osmotic pressure of ions in an electrolyte solution is critically examined. In principle these can be defined by introducing a solvent-permeable wall and measuring the force per unit area which can certainly be…

Soft Condensed Matter · Physics 2022-12-09 Patrick B. Warren

We studied ion concentration profiles and the charge density gradient caused by electrode reactions in weak electrolytes by using the Poisson--Nernst--Planck equations without assuming charge neutrality. In weak electrolytes, only a small…

Soft Condensed Matter · Physics 2018-02-08 Yohichi Suzuki , Kazuhiko Seki

The catalytic performance of multimetallic electrodes is often attributed to a beneficial combination of ligand, strain, and ensemble effects. Understanding the influence of the electrochemical environment on the stability of the alloy…

Chemical Physics · Physics 2021-12-08 Stephen E. Weitzner , Ismaila Dabo

We derive high-order terms in the asymptotic expansions of the steady-state voltage potentials in the presence of a finite number of diametrically small inhomogeneities with conductivities different from the background conductivity. Our…

Mathematical Physics · Physics 2007-05-23 Habib Ammari , Hyeonbae Kang

We present a generalized theory for studying static monomer density-density correlation function (structure factor) in concentrated solutions and melts of dipolar as well as ionic polymers. The theory captures effects of electrostatic…

Soft Condensed Matter · Physics 2018-11-14 Rajeev Kumar , Bradley Lokitz , Timothy E. Long , Bobby G. Sumpter

We consider the Poisson-Nernst-Planck system which is well-accepted for describing dilute electrolytes as well as transport of charged species in homogeneous environments. Here, we study these equations in porous media whose electric…

Mathematical Physics · Physics 2013-02-26 Markus Schmuck

This work presents a finite element method for a modified Poisson-Nernst-Planck/Navier-Stokes (PNP/NS) model under the mechanical equilibrium, developed for compressible electrolytes. Another key contribution of this work is the reduction…

Numerical Analysis · Mathematics 2026-01-27 Ankur , Ram Jiwari , Satyvir Singh

The kinetic behavior of a phase field model of electrochemistry is explored for advancing (electrodeposition) and receding (electrodissolution) conditions in one dimension. We described the equilibrium behavior of this model in [J. E.…

Materials Science · Physics 2007-05-23 J. E. Guyer , W. J. Boettinger , J. A. Warren , G. B. McFadden

Solid polymer electrolytes exhibit ion conduction and high mechanical properties, thus are promising materials for future energy storage devices. The ion conductivity in an SPE is intricately connected to salt ion distribution in the…

Soft Condensed Matter · Physics 2024-06-04 Ganesh K Rajahmundry , Tarak K Patra

Metal nanoparticles are receiving increased scientific attention owing to their unique physical and chemical properties that make them suitable for a wide range of applications in diverse fields, such as electrochemistry, biochemistry, and…

Chemical Physics · Physics 2020-10-09 Bendix Petersen , Rafael Roa , Joachim Dzubiella , Matej Kanduc

Poisson-Nernst-Planck equations are widely used to describe the electrodiffusion of ions in a solvated biomolecular system. Two kinds of two-grid finite element algorithms are proposed to decouple the steady-state Poisson-Nernst-Planck…

Numerical Analysis · Mathematics 2016-09-09 Ying Yang , Benzhuo Lu , Yan Xie