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X-ray scattering measurements on single crystals of TiOCl reveal the presence of commensurate dimerization peaks within both the incommensurate spin-Peierls phase and the so-called pseudogap phase above T_c2. This scattering is relatively…

Strongly Correlated Electrons · Physics 2016-08-05 J. P. Clancy , B. D. Gaulin , K. C. Rule , J. P. Castellan , F. C. Chou

We have studied the S=1/2 quasi-one-dimensional antiferromagnet TiOCl using single crystal x-ray diffraction and inelastic x-ray scattering techniques. The Ti ions form staggered spin chains which dimerize below Tc1 = 66 K and have an…

Strongly Correlated Electrons · Physics 2009-11-13 E. T. Abel , K. Matan , F. C. Chou , E. D. Isaacs , D. E. Moncton , H. Sinn , A. Alatas , Y. S. Lee

The ground state of the spin-Peierls system TiOCl was probed using synchrotron x-ray diffraction on a single-crystal sample at T = 6 K. We tracked the evolution of the structural superlattice peaks associated with the dimerized ground state…

Strongly Correlated Electrons · Physics 2012-08-23 A. Prodi , J. S. Helton , Yejun Feng , Y. S. Lee

We report on a detailed single crystal x-ray diffraction study of the unconventional spin-Peierls compound TiOCl. The intermediate phase of TiOCl is characterized by an incommensurate modulation which is virtually identical to that recently…

Strongly Correlated Electrons · Physics 2007-05-23 A. Krimmel , J. Strempfer , B. Bohnenbuck , B. Keimer , M. Hoinkis , M. Klemm , S. Horn , A. Loidl , M. Sing , R. Claessen , M. v. Zimmermann

Impurity-induced magnetic order has been observed in many quasi-1D systems including doped variants of the spin-Peierls system CuGeO3. TiOCl is another quasi-1D quantum magnet with a spin-Peierls ground state, and the magnetic Ti sites of…

Strongly Correlated Electrons · Physics 2015-05-27 A. A. Aczel , G. J. MacDougall , F. L. Ning , J. A. Rodriguez , S. R. Saha , F. C. Chou , T. Imai , G. M. Luke

In doped CuGeO3 systems, such as (Cu1-xZnx)GeO3 and Cu(Ge1-xSix)O3, the spin-Peierls (SP) ordering (T<Tsp) coexists with the antiferromagnetic (AF) phase (T<TN<Tsp). Tsp decreases while TN increases with increasing x in low doping region.…

Materials Science · Physics 2009-10-31 H. Nakao , M. Nishi , Y. Fujii , T. Masuda , I. Tsukada , K. Uchinokura , K. Hirota , G. Shirane

We report comprehensive synchrotron x-ray scattering and magnetic susceptibility studies of the doped spin-Peierls materials Cu_{1-x}Zn_xGeO_3 and CuGe_{1-y}Si_yO_3. Temperature versus dopant concentration phase diagrams are mapped out for…

Strongly Correlated Electrons · Physics 2007-05-23 Y. J. Wang , Y. J. Kim , R. J. Christianson , S. C. LaMarra , F. C. Chou , T. Masuda , I. Tsukada , K. Uchinokura , R. J. Birgeneau

The $S=1/2$ antiferromagnetic Heisenberg spin chain compound Sr$_2$CuO$_3$ doped with $1 \%$ and $2 \%$ of Ni impurities has been studied by means of $^{63}$Cu nuclear magnetic resonance. A strong decrease of the spin-lattice relaxation…

The energy spectrum of incommensurate spin fluctuations in superconducting Sr-doped La2CuO4 has been studied by inelastic neutron scattering experiments. An energy gap in the spin excitation spectrum is observed in the superconducting state…

Superconductivity · Physics 2009-10-31 Chul-Ho Lee , Kazuyoshi Yamada , Yasuo Endoh , Gen Shirane , R. J. Birgeneau , M. A. Kastner , M. Greven , Y-J. Kim

We have performed detailed x-ray scattering measurements on single crystals of the spin-Peierls compound TiOBr in order to study the critical properties of the transition between the incommensurate spin-Peierls state and the paramagnetic…

Strongly Correlated Electrons · Physics 2016-08-05 J. P. Clancy , B. D. Gaulin , F. C. Chou

We study the effect of disorder induced by doping on the transition temperature in high $T_c$ cuprates. Since the impurity lies between the CuO$_2$ planes, the momentum transfer is restricted by small angle with a range of order of $1/(d…

Superconductivity · Physics 2009-10-31 Hae-Young Kee

Using neutron scattering techniques, we have studied incommensurate spin ordering as well as low energy spin dynamics in single crystal underdoped \LBCO with x$\sim$0.095 and 0.08; high temperature superconductors with T$_C \sim$ 27 K and…

Superconductivity · Physics 2009-11-13 S. R. Dunsiger , Y. Zhao , Z. Yamani , W. J. L. Buyers , H. Dabkowska , B. D. Gaulin

Temperature-dependent x-ray diffraction of the low-dimensional spin 1/2 quantum magnet TiOBr shows that the phase transition at T_{c2} = 47.1 (4) K corresponds to the development of an incommensurate superstructure. Below T_{c1} = 26.8 \pm…

Other Condensed Matter · Physics 2007-05-23 Sander van Smaalen , Lukas Palatinus , Andreas Schonleber

We report a synchrotron x-ray scattering study of the diluted spin-Peierls (SP) material Cu_{1-x}Mg_xGeO_3. In a recent paper we have shown that the SP dimerization attains long-range order only for x < x_c = 0.022(0.001). Here we report…

Strongly Correlated Electrons · Physics 2009-10-31 V. Kiryukhin , Y. J. Wang , S. C. LaMarra , R. J. Birgeneau , T. Masuda , I. Tsukada , K. Uchinokura

We report neutron scattering studies on single crystals of the electron-doped (n-type) superconducting cuprate Nd2-xCexCuO4 (x=0.15) with Tc = 18 K and 25 K. Unlike the hole-doped (p-type) superconducting cuprates where incommensurate…

Strongly Correlated Electrons · Physics 2009-11-07 K. Yamada , K. Kurahashi , T. Uefuji , M. Fujita , S. Park , S. -H. Lee , Y. Endoh

The sequence of phase transitions and the symmetry of in particular the low temperature incommensurate and spin-Peierls phases of the quasi one-dimensional inorganic spin-Peierls system TiOX (TiOBr and TiOCl) have been studied using…

Incommensurate (IC) charge-order (CO) and spin density wave (SDW) order in electron doped SrMn1-xWxO3-{\delta} (x= 0.08 to 0.1875) have been studied using neutron diffraction.The study highlights the drastic effect of electron doping on the…

Materials Science · Physics 2019-07-04 Poonam Yadav , Shivani Sharma , Aga Shahee , Ivan da Silva , Vaclav Petricek , N P Lalla

The spin dynamics of an optimally doped YBa2Cu3O7 (Tc = 93 K) crystal array have been investigated in a wide range of momentum and energy (Q - E) space using the time-of-flight neutron scattering method. Incommensurate spin modulation in Q…

Superconductivity · Physics 2007-05-23 M. Arai , T. Nishijima , Y. Endoh , A. W. Garrett , S. Tajima , K. Tomimoto , Y. Shiohara , C. D. Frost , S. M. Bennington

Dramatic evolution of properties with minute change in the doping level is a hallmark of the complex chemistry which governs cuprate superconductivity as manifested in the celebrated superconducting domes as well as quantum criticality…

The application of pressure can induce transitions between unconventional quantum phases in correlated materials. The inorganic compound TiOCl, composed of chains of S=1/2 Ti ions, is an ideal realization of a spin-Peierls system with a…

Strongly Correlated Electrons · Physics 2018-02-21 Costel R. Rotundu , Jiajia Wen , Wei He , Yongseong Choi , Daniel Haskel , Young S. Lee
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