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We have studied the magnetic properties of clinoatacamite Cu$_2$Cl(OH)$_3$, the parent compound of the quantum spin liquid candidate herbertsmithite and a longstanding puzzle among frustrated quantum magnets. As we reveal using…

Kagome metals have established a new arena for correlated electron physics. To date, the predominant experimental evidence centers around unconventional charge order, nematicity, and superconductivity, while magnetic fluctuations due to…

We report through 17O NMR, an unambiguous local determination of the intrinsic kagome lattice spin susceptibility as well as that created around non-magnetic defects issued from natural Zn/ Cu exchange in the S=1/2 (Cu2+) herbertsmithite…

Strongly Correlated Electrons · Physics 2009-11-13 A. Olariu , P. Mendels , F. Bert , F. Duc , J. C. Trombe , M. A. de Vries , A. Harrisson

The recent NMR experiments on ZnCu3(OH)6Cl2 motivate our study of the effect of non- magnetic defects on the antiferromagnetic spin-1/2 kagome lattice. We use exact diagonalization methods to study the effect of two such defects on finite…

Strongly Correlated Electrons · Physics 2009-11-13 M. J. Rozenberg , R. Chitra

Two-dimensional (2D) kagome metals offer a unique platform for exploring electron correlation phenomena derived from quantum many-body effects. Here, we report a combined study of electrical magnetotransport and neutron scattering on…

The spin-1/2 kagome antiferromagnets are key prototype materials for studying frustrated magnetism. Three isostructural kagome antiferromagnets LnCu$_3$(OH)$_6$Cl$_3$ (Ln = Gd, Tb, Dy) have been successfully synthesized by the hydrothermal…

Strongly Correlated Electrons · Physics 2021-08-27 Ying Fu , Lianglong Huang , Xuefeng Zhou , Jian Chen , Xinyuan Zhang , Pengyun Chen , Shanmin Wang , Cai Liu , Dapeng Yu , Hai-Feng Li , Le Wang , Jia-Wei Mei

Experimental studies of high-purity kagome-lattice antiferromagnets (KAFM) are of great importance in attempting to better understand the predicted enigmatic quantum spin-liquid ground state of the KAFM model. However, realizations of this…

Strongly Correlated Electrons · Physics 2021-06-02 W. Sun , T. Arh , M. Gomilšek , P. Koželj , S. Vrtnik , M. Herak , J. -X. Mi , A. Zorko

The magnetic properties of Cs$_2$Cu$_3$CeF$_{12}$ were investigated through magnetization and specific heat measurements. Cs$_2$Cu$_3$CeF$_{12}$ is composed of a buckled kagome lattice of Cu$^{2+}$, which is stacked along the b axis. The…

Strongly Correlated Electrons · Physics 2015-06-04 Taiki Amemiya , Izumi Umegaki , Hidekazu Tanaka , Toshio Ono , Akira Matsuo , Koichi Kindo

Strain applied to a condensed-matter system can be used to engineer its excitation spectrum via artificial gauge fields, or it may tune the system through transitions between different phases. Here we demonstrate that strain tuning of the…

Strongly Correlated Electrons · Physics 2022-03-28 Mary Madelynn Nayga , Matthias Vojta

We report a detailed study of the magnetic properties, critical analysis of magnetization, and magnetocaloric effect of a spin-$2$ kagome lattice YCa$_3$(MnO)$_3$(BO$_3$)$_4$. The experiments are complemented by the density functional band…

Materials Science · Physics 2025-07-29 A. Choudhary , A. Magar , S. Ghosh , S. Kanungo , R. Nath

We present a $^{35}$Cl NMR study for spin $S=1/2$ perfect kagome antiferromagnet Ca-kapellasite (CaCu$_{3}$(OH)$_{6}$Cl$_{2}\cdot$0.6H$_{2}$O) with a magnetic transition at $T^{\ast}=7.2$ K. The static magnetic structure in the ground state…

Strongly Correlated Electrons · Physics 2020-07-01 Y. Ihara , K. Arashima , H. Yoshida , M. Hirata , T. Sasaki

We prepared a powder sample of edwardsite Cd2Cu3(SO4)2(OH)6 4H2O, which is a new candidate compound for the spin-1/2 kagome antiferromagnet, and studied its magnetic properties by magnetic susceptibility and heat capacity measurements.…

Materials Science · Physics 2015-06-15 Hajime Ishikawa , Yoshihiko Okamoto , Zenji Hiroi

Hexagonal antiferromagnets Cs$_2$Cu$_3$MF$_{12}$ (M = Zr, Hf and Sn) have uniform Kagome lattices of Cu$^{2+}$ with S = 1/2, whereas Rb$_2$Cu$_3$SnF$_{12}$ has a 2a by 2a enlarged cell as compared with the uniform Kagome lattice. The…

Strongly Correlated Electrons · Physics 2013-05-29 T. Ono , K. Morita , M. Yano , H. Tanaka , K. Fujii , H. Uekusa , Y. Narumi , K. Kindo

The kagome lattice antiferromagnets Mn$_3$X(= Sn, Ge) have a noncollinear 120$^\circ$ ordered ground state, which engenders a strong anomalous Hall response. It has been shown that this response is linked to the magnetic order and can be…

Mesoscale and Nanoscale Physics · Physics 2022-11-16 Sayak Dasgupta , Oleg A. Tretiakov

We report thermodynamic measurements of the S=1/2 kagome lattice antiferromagnet ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$, a promising candidate system with a spin-liquid ground state. Using single crystal samples, the magnetic susceptibility both…

Strongly Correlated Electrons · Physics 2012-04-16 Tianheng Han , Shaoyan Chu , Young S. Lee

Spin-frustrated systems are one avenue for inducing macroscopic quantum states in materials. However, experimental realization of this goal has been difficult because of the lack of simple materials and, if available, the separation of the…

Strongly Correlated Electrons · Physics 2010-04-07 S. Chu , T. M. McQueen , R. Chisnell , D. E. Freedman , P. Müller , Y. S. Lee , D. G. Nocera

Quantum spin liquids represent exotic states of spin systems characterized by long-range entanglement and emergent fractionalized quasiparticles. It is generally believed that disorder is hostile to quantum spin liquids. In our study, we…

Strongly Correlated Electrons · Physics 2024-08-30 Aini Xu , Qinxin Shen , Bo Liu , Zhenyuan Zeng , Lankun Han , Liqin Yan , Jun Luo , Jie Yang , Rui Zhou , Shiliang Li

This study examines the effect of distorted triangular magnetic interactions in the Kagome lattice. Using a Holstein-Primakoff expansion, we determine the analytical solutions for classical energies and the spin-wave modes for various…

Strongly Correlated Electrons · Physics 2021-02-09 A. A. Coker , A. Saxena , J. T. Haraldsen

Non-collinear Kagome antiferromagnets (AFMs) Mn3X (X = Sn, Ga, Ge, Ir, Pt) can generate an anomalous Hall effect (AHE) despite vanishing net magnetization, enabled by broken time-reversal and inversion symmetries. However, strong in-plane…

Single-crystal growth, magnetic properties, and magnetocaloric effect of the $S = 3/2$ kagome ferromagnet Li$_9$Cr$_3$(P$_2$O$_7$)$_3$(PO$_4$)$_2$ (trigonal, space group: $P\bar{3}c1$) are reported. Magnetization data suggest dominant…