Related papers: Attoscience
We report on new routes to generating a train of attosecond pulses. The methods are extremely simple and robust; we need to place only a few thin dispersive materials in the optical path. We numerically demonstrate the generation of a train…
The generation of ultra-strong attosecond pulses through laser-plasma interactions offers the opportunity to surpass the intensity of any known laboratory radiation source, giving rise to new experimental possibilities, such as quantum…
We present the first direct experimental confirmation of attosecond pulse generation in the hard X-ray regime with a free-electron laser. Our experiment is based on measurements of a nonlinear optical phenomenon known as amplified…
The motion of electrons in or near solids, liquids and gases can be tracked by forcing their ejection with attosecond x-ray pulses, derived from femtosecond lasers. The momentum of these emitted electrons carries the imprint of the…
We demonstrate control over attosecond pulse generation and shaping by numerically optimizing the synthesis of few-cycle to sub-cycle driver waveforms. The optical waveform synthesis takes place in an ultrabroad spectral band covering the…
The discovery of pulsars in 1968 heralded an era where the temporal characteristics of detectors had to be reassessed. Up to this point detector integration times would normally be measured in minutes rather seconds and definitely not on…
This tutorial presents an introduction to the interaction of light and matter on the attosecond timescale. Our aim is to detail the theoretical description of ultra-short time-delays, and to relate these to the phase of extreme ultraviolet…
Femtosecond electron microscopy produces real-space images of matter in a series of ultrafast snapshots. Pulses of electrons self-disperse under space-charge broadening, so without compression, the ideal operation mode is a single electron…
Coherent control over electron dynamics in atoms and molecules using high-intensity circularly-polarized laser pulses gives rise to current loops, resulting in the emission of magnetic fields. We propose and demonstrate with ab-initio…
Relativistic surface high harmonics have been considered a unique source for the generation of intense isolated attosecond pulses in the extreme ultra-violet (XUV) and X-ray spectral range. However, its experimental realization is still a…
Attosecond pulses from X-ray free-electron laser (XFEL) have opened new opportunities for probing ultrafast electronic dynamics on the Angstrom--attosecond spatiotemporal scale. Most attosecond XFEL concepts rely on generating an ultrashort…
We propose utilizing a polarization-tailored high-power laser pulse to extract and accelerate electrons from the edge of a solid foil target to produce isolated attosecond electron bunches. The laser pulse consists of two…
Attosecond science is based on steering of electrons with the electric field of well-controlled femtosecond laser pulses. It has led to, for example, the generation of XUV light pulses with a duration in the sub-100-attosecond regime, to…
Time-resolved electronic processes on the attosecond scale have recently become experimentally accessible through the development of laser-based pump-probe interrogation techniques such as the attosecond streak camera, the reconstruction of…
We review the main research directions ongoing in the development of high-harmonic generation-based extreme ultraviolet sources for the synthesization and application of trains and isolated attosecond pulses to time-resolved spectroscopy. A…
The precise temporal characterization of laser pulses is crucial for ultrashort applications in biology, chemistry, and physics. Especially in femto- and attosecond science, diverse laser pulse sources in different spectral regimes from the…
The advent of ultrahigh-power femtosecond lasers creates a need for optical components suitable to handle ultrahigh light intensities. Due to the unavoidable laser-induced ionization of matter, these components will have to be based on a…
In the last few decades the development of ultrafast lasers has revolutionized our ability to gain insight into light-matter interactions. The appearance of few-cycle light sources available from the visible to the mid-infrared spectral…
Real-time optics and spectroscopy simulations ideally provide results at update rates of 120 Hz or more without any noticeable delay between changing input parameters and the calculated results. Such calculations require models of…
Photoionization from energetically distinct electronic states may have a relative time delay of tens of attoseconds. Here we demonstrate that pulses of optical vortices allow measuring such attoseconds delays from magnetic sublevels, even…