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Orbital degrees of freedom play a major role in the physics of many strongly correlated transition metal compounds. However, they are still very difficult to access experimentally, in particular by neutron scattering. We propose here how to…

Strongly Correlated Electrons · Physics 2015-04-28 Pasquale Marra

The study of elementary bosonic excitations is essential toward a complete description of quantum electronic solids. In this context, resonant inelastic X-ray scattering (RIXS) has recently risen to becoming a versatile probe of electronic…

Strongly Correlated Electrons · Physics 2019-01-23 M. Kang , J. Pelliciari , Y. Krockenberger , J. Li , D. E. McNally , E. Paris , R. Liang , W. N. Hardy , D. A. Bonn , H. Yamamoto , T. Schmitt , R. Comin

We present a computational study of $L$-edge resonant inelastic x-ray scattering (RIXS) in correlated 3$d$ transition-metal oxides using an $ab$ $initio$ method based on local density approximation + dynamical mean-field theory (DMFT). The…

Strongly Correlated Electrons · Physics 2020-03-25 Atsushi Hariki , Mathias Winder , Takayuki Uozumi , Jan Kuneš

We study the magnetic excitations in 5d transition-metal oxide Sr$_2$IrO$_4$ on the basis of the Heisenberg model with small anisotropic terms on a square lattice. We calculate the correlation functions by using the Green's functions in the…

Strongly Correlated Electrons · Physics 2015-06-18 Jun-ichi Igarashi , Tatsuya Nagao

Inelastic x-ray scattering (IXS) with very high (meV) energy resolution has become a valuable spectroscopic tool, complementing the well established coherent inelastic neutron scattering (INS) technique for phonon dispersion investigations.…

Strongly Correlated Electrons · Physics 2009-11-07 M. d'Astuto , P. K. Mang , P. Giura , A. Shukla , A. Mirone , M. Krisch , F. Sette , P. Ghigna , M. Braden , M. Greven

In a recent publication Larson \textit{et al.} reported remarkably clear $d$-$d$ excitations for NiO and CoO measured with x-ray energies well below the transition metal $K$ edge. In this letter we demonstrate that we can obtain an accurate…

Strongly Correlated Electrons · Physics 2008-01-09 M. W. Haverkort , A. Tanaka , L. H. Tjeng , G. A. Sawatzky

We report a comprehensive resonant inelastic x-ray scattering (RIXS) study of various iridate materials focusing on core-level excitations and transitions between crystal-field split d-levels. The 2p core hole created at the Ir $L_3$…

Strongly Correlated Electrons · Physics 2018-05-10 Young-June Kim , J. P. Clancy , H. Gretarsson , G. Cao , Yogesh Singh , Jungho Kim , M. H. Upton , D. Casa , T. Gog

The capability to probe the dispersion of elementary spin, charge, orbital, and lattice excitations has positioned resonant inelastic x-ray scattering (RIXS) at the forefront of photon science. Here we develop the scattering theory for RIXS…

Superconductivity · Physics 2015-04-10 Pasquale Marra , Steffen Sykora , Krzysztof Wohlfeld , Jeroen van den Brink

The state-resolved differential cross sections for both the 1s2 1S0 - 1s2s 1S0 monopolar transition and the 1s2 1S0 - 1s2p 1P1 dipolar transition of atomic helium have been measured over a large momentum transfer region by the…

Atomic Physics · Physics 2015-05-13 B. P. Xie , L. F. Zhu , K. Yang , B. Zhou , N. Hiraoka , Y. Q. Cai , Y. Yao , C. Q. Wu , E. L. Wang , D. L. Feng

Inelastic X-ray scattering (IXS) is an important tool for studies of equilibrium dynamics in condensed matter. A new spectrometer recently proposed for ultra-high-resolution IXS (UHRIX) has achieved 0.6~meV and 0.25~nm$^{-1}$ spectral and…

An application of resonant inelastic x-ray scattering technique for studying of optical scale excitations in electron-correlated materials is discussed. Examples are given including data obtained for 3d transition metal, lanthanide, and…

Strongly Correlated Electrons · Physics 2007-05-23 Sergei M. Butorin

We explore the use of optimized operators, designed to interpolate only a single meson eigenstate, in three-point correlation functions with a vector-current insertion. These operators are constructed as linear combinations in a large basis…

High Energy Physics - Lattice · Physics 2015-01-30 Christian J. Shultz , Jozef J. Dudek , Robert G. Edwards

The resonant inelastic x-ray scattering (RIXS) was measured in an insulating SrCuO$_{2}$ with changing the incident photon energy ($h\nu$) near the Cu $1s$ absorption edge (K-edge). Complex structures and their dependences on the momentum…

We report a high resolution resonant inelastic x-ray scattering investigation of the bilayer manganites La$_{2-2x}$Sr$_{1+2x}$Mn$_2$O$_7$ with $x = 0.36$ and $0.5$. The momentum dependence along the crystallographic $(110)$ direction for…

Strongly Correlated Electrons · Physics 2011-07-07 F. Weber , S. Rosenkranz , J. -P. Castellan , R. Osborn , J. F. Mitchell , H. Zheng , D. Casa , J. H. Kim , T. Gog

Resonant inelastic X-ray scattering (RIXS) detects various types of high- and low-energy elementary excitations in correlated solids, and this tool will play an increasingly important role in investigations of time-dependent phenomena in…

Strongly Correlated Electrons · Physics 2021-12-21 Philipp Werner , Steven Johnston , Martin Eckstein

Non-resonant inelastic x ray scattering (NIXS) experiments have been performed to probe the 5d-5f electronic transitions at the uranium O(4,5) absorption edges in uranium dioxide. For small values of the scattering vector q, the spectra are…

Strongly Correlated Electrons · Physics 2013-12-19 R. Caciuffo , G. van der Laan , L. Simonelli , T. Vitova , C. Mazzoli , M. A. Denecke , G. H. Lander

Time-resolved measurements of materials provide a wealth of information on quasiparticle dynamics, and have been the focus of optical studies for decades. In this paper, we develop a theory for explicitly evaluating time-resolved resonant…

Strongly Correlated Electrons · Physics 2019-03-27 Yuan Chen , Yao Wang , Chunjing Jia , Brian Moritz , Andrij M. Shvaika , James K. Freericks , Thomas P. Devereaux

Phase transitions driven by ultrashort laser pulses have attracted interest both for understanding the fundamental physics of phase transitions and for potential new data storage or device applications. In many cases these transitions…

We study the resonant inelastic x-ray scattering (RIXS) features of vector chiral ordered kagome antiferromagnets. Utilizing a group theoretical formalism that respects lattice site symmetry, we calculated the $L$ -edge magnon contribution…

Strongly Correlated Electrons · Physics 2024-01-05 Zijian Xiong , Trinanjan Datta , Dao-Xin Yao

X-ray absorption spectroscopy (XAS) is an explicit probe of the unoccupied electronic structure of materials and an invaluable tool for fingerprinting various electronic properties and phenomena. Computational methods capable of simulating…

Materials Science · Physics 2023-02-07 Subhayan Roychoudhury , David Prendergast