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Related papers: Persistent Spin Dynamics in the $S=1/2$ V$_{15}$ M…

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Muon spin relaxation ($\mu$SR) and magnetic susceptibility measurements have been performed on the pure and diluted spin 1/2 kagom\'{e} system (Cu$_x$Zn$_{1-x}$)$_{3}$V$_{2}$O$_7$(OH)$_{2}$ 2H$_2$O. In the pure $x=1$ system we found a…

A single-molecule magnet placed in a magnetic field perpendicular to its anisotropy axis can be truncated to an effective two-level system, with easily tunable energy splitting. The quantum coherence of the molecular spin is largely…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 A. Morello , A. Millán , L. J. de Jongh

We present zero field muon spin lattice relaxation measurements of a Dysprosium triangle molecular magnet. The local magnetic fields sensed by the implanted muons indicate the coexistence of static and dynamic internal magnetic fields below…

Strongly Correlated Electrons · Physics 2015-05-20 Z. Salman , S. R. Giblin , Y. Lan , A. K. Powell , R. Scheuermann , R. Tingle , R. Sessoli

We address the cause of the unusual muon spin relaxation (muSR) results on molecular nanomagnets (MNMs). Through measurements on protonated and deuterated samples of the MNMs Cr7Mn (S=1) and Cr8 (S=0), we show that the muon spin for $S \neq…

The spin dynamics in [TbPc$_{2}$]$^{0}$ and [DyPc$_{2}$]$^{0}$ single molecule magnets have been investigated by means of muon and nuclear spin-lattice relaxation rate measurements. The correlation time for the spin fluctuations was found…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 F. Branzoli , M. Filibian , P. Carretta , S. Klytaskaya , M. Ruben

We report single-crystal 51V NMR studies on volborthite Cu3V2O7(OH)2 2H2O, which is regarded as a quasi-two-dimensional frustrated magnet with competing ferromagnetic and antiferromagnetic interactions. In the 1/3 magnetization plateau…

We report muon spin relaxation and inelastic neutron measurements on the Heusler system YbPd$_2$Sn. Localised anisotropic and quasi-elastic Yb magnetic fluctuations are observed below $T = 150$K. Both $\mu$SR and neutron data indicate a…

Strongly Correlated Electrons · Physics 2009-11-07 A. Amato , B. Roessli , P. Fischer , N. Bernhoeft , A. Stunault , C. Baines , A. Dönni , H. Sugawara

The spin dynamics of geometrically frustrated pyrochlore antiferromagnets Y2Mo2O7 and Tb2Mo2O7 have been investigated using muon spin relaxation. A dramatic slowing down of the moment fluctuations occurs as one approaches the spin freezing…

The spin-lattice relaxation rate $T_{1}^{-1}$ and NMR spectra of $^1$H in single crystal molecular magnets of Fe8 have been measured down to 15 mK. The relaxation rate $T_1^{-1}$ shows a strong temperature dependence down to 400 mK. The…

Condensed Matter · Physics 2009-11-07 Miki Ueda , Satoru Maegawa , Susumu Kitagawa

Employing the muon spin relaxation technique we evidence temperature independent magnetic fluctuations persisting down to the lowest temperatures in the samarium-based ($J=5/2$) kagome-lattice Langasite. A detailed bulk-magnetization…

Strongly Correlated Electrons · Physics 2012-11-01 A. Zorko , F. Bert , P. Mendels , A. Potočnik , A. Amato , C. Baines , K. Marty , P. Bordet , P. Lejay , E. Lhotel , V. Simonet , R. Ballou

The temporal magnetic correlations of the triangular lattice antiferromagnet NiGa$_2$S$_4$ are examined through thirteen decades ($10^{-13}-1$~sec) using ultra-high-resolution inelastic neutron scattering, muon spin relaxation, AC and…

Muon spin rotation (muSR) experiments reveal unconventional spin freezing and dynamics in the two-dimensional (2D) triangular lattice antiferromagnet NiGa2S4. Long-lived disordered Ni-spin freezing (correlation time > 10-6 s at 2 K) sets in…

Strongly Correlated Electrons · Physics 2009-11-13 D. E. MacLaughlin , Y. Nambu , S. Nakatsuji , R. H. Heffner , Lei Shu , O. O. Bernal , K. Ishida

We report muon spin relaxation (muSR) and magnetic susceptibility investigations of two Ti3+ chain compounds which each exhibit a spin gap at low temperature, NaTiSi2O6 and TiOCl. From these we conclude that the spin gap in NaTiSi2O6 is…

Strongly Correlated Electrons · Physics 2010-07-08 P. J. Baker , S. J. Blundell , F. L. Pratt , T. Lancaster , M. L. Brooks , W. Hayes , M. Isobe , Y. Ueda , M. Hoinkis , M. Sing , M. Klemm , S. Horn , R. Claessen

Low-temperature muon spin-lattice relaxation measurements in the non-Fermi-liquid heavy-fermion alloys UCu_{5-x}Pd_x, x = 1.0 and 1.5, indicate inhomogeneously distributed f-electron spin fluctuation rates, and exhibit a time-field scaling…

Strongly Correlated Electrons · Physics 2009-11-07 D. E. MacLaughlin , R. H. Heffner , O. O. Bernal , G. J. Nieuwenhuys , J. E. Sonier , M. S. Rose , R. Chau , M. B. Maple , B. Andraka

We report results of a muon spin relaxation study of slow magnetic fluctuations in the pseudogap phase of underdoped single-crystalline YBa$_{2}$Cu$_{3}$O$_{y}$, $y = 6.77$ and 6.83. The dependence of the dynamic muon spin relaxation rate…

We present an ultra-low temperature study (down to T = 20 mK) of the nuclear spin-lattice relaxation (SLR) in the 55Mn nuclei of the molecular magnet Mn12-ac. The nuclear spins act as local probes for the electronic spin fluctuations, due…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 A. Morello , O. N. Bakharev , H. B. Brom , L. J. de Jongh

We present a muon-spin relaxation investigation of the Ising chain magnet Ca_{3}Co_{2-x}Mn_{x}O_{6} (x~0.95). We find dynamic spin fluctuations persisting down to the lowest measured temperature of 1.6 K. The previously observed transition…

Strongly Correlated Electrons · Physics 2009-08-27 T. Lancaster , S. J. Blundell , P. J. Baker , H. J. Lewtas , W. Hayes , F. L. Pratt , H. T. Yi , S. -W. Cheong

We measure the spin-lattice relaxation of donor bound electrons in ultrapure, isotopically enriched, phosphorus-doped $^{28}$Si:P. The optical pump-probe experiments reveal at low temperatures extremely long spin relaxation times which…

Mesoscale and Nanoscale Physics · Physics 2021-04-13 Eduard Sauter , Nikolay V. Abrosimov , Jens Hübner , Michael Oestreich

Spin relaxation between the two lowest-lying spin-states has been studied in the S=4 single molecule magnet Ni$_4$ under steady state conditions of low amplitude and continuous microwave irradiation. The relaxation rate was determined as a…

Mesoscale and Nanoscale Physics · Physics 2008-07-22 G. de Loubens , D. A. Garanin , C. C. Beedle , D. N. Hendrickson , A. D. Kent

Nuclear spin-lattice relaxation times are measured on copper using magnetic resonance force microscopy performed at temperatures down to 42 mK. The low temperature is verified by comparison with the Korringa relation. Measuring spin-lattice…

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