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We numerically study the ground state properties of endohedrally confined hydrogen (H) or helium (He) atom by a molecule of C$_{60}$. Our study is based on Diffusion Monte Carlo method. We calculate the effects of centered and small…

Other Condensed Matter · Physics 2009-11-13 M. Neek-Amal , G. Tayebirad , R. Asgari

In this paper the Diffusion Monte Carlo (DMC) method is applied to the confined hydrogen atom with different confinement geometries. This approach is validated using the much studied spherical and cylindrical confinements and then applied…

Chemical Physics · Physics 2019-03-20 Gaia Micca Longo , Savino Longo , Domenico Giordano

We calculate the energies of ground and three low lying excited states of confined helium atom centered in an impenetrable spherical box. We perform the calculation by employing variational method with two-parameter variational forms for…

Atomic Physics · Physics 2009-11-11 Arup Banerjee , C. Kamal , Avijit Chowdhury

We study the hydrogen atom confined to a spherical box with impenetrable walls but, unlike earlier pedagogical articles on the subject, we assume that the nucleus also moves. We obtain the ground-state energy approximately by means of…

Quantum Physics · Physics 2015-05-13 Francisco M. Fernandez

We calculate ground-state energies and densities of a helium atom confined in an impenetrable spherical box within density functional theory. These calculations are performed by variationally solving Kohn-Sham equation with the ground-state…

Atomic Physics · Physics 2010-06-24 Subhajit Waugh , Avijit Chowdhury , Arup Banerjee

The ground and excited state properties of small helium clusters, 4He_N, containing nanoscale (~3-10 Angstroms) planar aromatic molecules have been studied with quantum Monte Carlo methods. Ground state structures and energies are obtained…

Chemical Physics · Physics 2016-09-08 Patrick Huang , Heather D. Whitley , K. Birgitta Whaley

We calculate the ground--state energy and other physical properties of the hydrogen atom inside a spherical box with an impenetrable wall. We apply the variational method and perturbation theory and compare both approximate results. We show…

Quantum Physics · Physics 2015-05-19 Francisco M. Fernández , N. Aquino , A. Flores-Riveros

The variational Monte Carlo method is used to evaluate the ground-state energy of the confined hydrogen molecule, H_2. Accordingly, we considered the case of hydrogen molecule confined by a hard prolate spheroidal cavity when the nuclear…

Atomic and Molecular Clusters · Physics 2015-09-10 S. B. Doma , F. N. El-Gammal , A. A. Amer

The ground-state properties of two-dimensional liquid $^4$He at zero temperature are studied by means of a quadratic diffusion Monte Carlo method. As interatomic potential we use a revised version of the HFDHE2 Aziz potential which is…

Condensed Matter · Physics 2009-10-28 S. Giorgini , J. Boronat , J. Casulleras

The ground state energy of hydrogen molecular ion H2+ confined by a hard prolate spheroidal cavity is calculated. The case in which the nuclear positions are clamped at the foci is considered. Our calculations are based on using the…

Atomic and Molecular Clusters · Physics 2016-05-25 S. B. Doma , F. N. El-Gammal , A. A. Amer

The diffusion Monte Carlo method with symmetry-based state selection is used to calculate the quantum energy states of H$_2^+$ confined into potential barriers of atomic dimensions (a model for these ions in solids). Special solutions are…

Chemical Physics · Physics 2019-04-03 Gaia Micca Longo , Savino Longo , Domenico Giordano

A rich literature has been produced on the quantum states of atoms and molecules confined into infinite potential wells with a specified symmetry. Apart from their interest as basic quantum systems, confined atoms and molecules are useful…

Chemical Physics · Physics 2019-04-03 Savino Longo , Gaia Micca Longo , Domenico Giordano

The Pade approximant technique and the variational Monte Carlo method are applied to determine the ground-state energy of a finite number of charged bosons in two dimensions confined by a parabolic trap. The particles interact repulsively…

Condensed Matter · Physics 2009-10-31 A. Gonzalez , B. Partoens , A. Matulis , F. M. Peeters

A self-contained and tutorial presentation of the diffusion Monte Carlo method for determining the ground state energy and wave function of quantum systems is provided. First, the theoretical basis of the method is derived and then a…

Computational Physics · Physics 2009-10-30 Ioan Kosztin , Byron Faber , Klaus Schulten

We study one-dimensional (1D) and two-dimensional (2D) Helium atoms using a new time-dependent quantum Monte Carlo (TDQMC) method. The TDQMC method employs random walkers, with a separate guiding wave attached to each walker. The ground…

Atomic Physics · Physics 2025-02-07 I. P. Christov

We report ground state energies and structural properties for small helium clusters (4He) containing an H- impurity computed by means of variational and diffusion Monte Carlo methods. Except for 4He_2H- that has a noticeable contribution…

Atomic and Molecular Clusters · Physics 2009-10-31 M. Casalegno , M. Mella , G. Morosi , D. Bressanini

We have used diffusion Monte Carlo (DMC) simulations to calculate the energy barrier for H$_2$ dissociation on the Mg(0001) surface. The calculations employ pseudopotentials and systematically improvable B-spline basis sets to expand the…

Materials Science · Physics 2009-11-13 M. Pozzo , D. Alfe`

We report results for the ground-state energy and structural properties of small $^4$He-T$\downarrow$ clusters consisting of up to 4 T$\downarrow$ and 8 $^4$He atoms. These results have been obtained using very well-known $^4$He-$^4$He and…

Mesoscale and Nanoscale Physics · Physics 2016-08-14 P. Stipanović , L. Vranješ Markić , J. Boronat , B. Kežić

We have calculated the ground state electronic structure of He under pressure from 0 to 1500 GPa using both all-electron full-potential and pseudopotential methods based on the density functional theory (DFT). We find that throughout this…

Materials Science · Physics 2012-01-10 W. Xiao , Z. X. Tian , W. T. Geng

Computational codes based on the Diffusion Monte Carlo method can be used to determine the quantum state of two-electron systems confined by external potentials of various nature and geometry. In this work, we show how the application of…

Chemical Physics · Physics 2021-02-24 Gaia Micca Longo , Carla Maria Coppola , Domenico Giordano , Savino Longo
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