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The electronic and lattice dynamical properties of compressed solid SiH$_{4}$ have been calculated in the pressure range up to 300 GPa with density functional theory. We find that structures having a layered network with eight-fold…

Superconductivity · Physics 2008-03-20 X. J. Chen , J. L. Wang , V. V. Struzhkin , H. K. Mao , R. J. Hemley , H. Q. Lin

Recently for the first time a stable compound of He and Na (Na2He) is predicted at high pressure. We explore the pressure dependent elastic, mechanical and thermodynamic properties of this newly discovered Na2He by using ab initio…

Materials Science · Physics 2018-01-08 Md. Zahidur Rahaman , Md. Lokman Ali , Md. Atikur Rahman

We study the structural stability and dynamical properties of Ar(H2)2 under pressure using first-principles and ab initio molecular dynamics techniques. At low temperatures, Ar(H2)2 is found to stabilize in the cubic C15 Laves structure…

Materials Science · Physics 2015-05-28 Claudio Cazorla , Daniel Errandonea

Following the idea that hydrogen-rich compounds might be high-T$_c$ superconductors at high pressures, and the very recent breakthrough in predicting and synthesizing hydrogen sulfide with record-high T$_c$ = 203 K, ab initio evolutionary…

Superconductivity · Physics 2017-04-19 M. M. Davari Esfahani , A. R. Oganov , H. Niu , J. Zhang

Mg$_2$IrH$_6$ is a metastable complex metal hydride with a predicted superconducting transition temperature as high as 170 K at ambient pressure. Following the synthesis of isomorphic, insulating Mg$_2$IrH$_5$ at low pressure,…

By means of first-principles calculations, we studied stable lattice structures and estimated superconducting transition temperature of CaSi$_2$ at high pressure. Our simulation showed stability of the AlB$_2$ structure in a pressure range…

Superconductivity · Physics 2009-11-13 A. Nakanishi , T. Ishikawa , H. Nagara , K. Kusakabe

Ab initio random structure searching with density functional theory was used to determine the zero-temperature structures of atomic metallic hydrogen from 500 GPa to 5 TPa. Including zero point motion in the harmonic approximation, we…

Materials Science · Physics 2015-05-20 Jeffrey M. McMahon , David M. Ceperley

AgSbTe2 is a well-known thermoelectric material with a high Seebeck coefficient and intrinsically low thermal conductivity, but its behavior under pressure remains largely unexplored. Here we report a systematic investigation of the…

We have performed ab initio calculations for new high-pressure phase of Ca-VI between 158-180 GPa. The study includes elastic parameters of mono- and poly-crystalline aggregates, electronic band structure, lattice dynamics and…

Superconductivity · Physics 2015-05-19 M. Aftabuzzaman , A. K. M. A. Islam

Alkali metals exhibit unexpected structures and electronic behavior at high pressures. Compression of metallic sodium (Na) to 200 GPa leads to the stability of a wide-band-gap insulator with the double hexagonal hP4 structure. Post-hP4…

Materials Science · Physics 2015-08-19 Yinwei Li , Yanchao Wang , Chris J. Pickard , Richard J. Needs , Yi Wang , Yanming Ma

By employing first-principles metadynamics simulations, we explore the 300 K structures of solid hydrogen over the pressure range 150-300 GPa. At 200 GPa, we find the ambient-pressure disordered hexagonal close-packed (hcp) phase transited…

Materials Science · Physics 2012-08-16 Hanyu Liu , Li Zhu , Wenwen Cui , Yanming Ma

High-pressure studies on elements play an essential role in superconductivity research, with implications for both fundamental science and applications. Here we report the experimental discovery of surprisingly low pressure driving a novel…

High pressure in-situ synchrotron X-ray diffraction experiments were performed on Ag2Te up to 42.6 GPa at room temperature and four phases were identified. Phase I ({\beta}-Ag2Te) transformed into phase II at 2.4 GPa, and phase III and…

Materials Science · Physics 2015-05-01 Zhao Zhao , Shibing Wang , Haijun Zhang , Wendy L. Mao

In the search for MgB2-like phonon-mediated superconductors we have carried out a systematic density functional theory study of the Ca-B system, isoelectronic to Mg-B, at ambient and gigapascal pressures. A remarkable variety of candidate…

Materials Science · Physics 2015-06-16 Sheena Shah , Aleksey N. Kolmogorov

The first-principle method of mathematical modeling was used to calculate the structural, electronic, phonon, and other characteristics of the normal metallic phase of hydrogen at a pressure of 500 GPa. It has been shown that metal hydrogen…

Superconductivity · Physics 2016-07-06 Nikolay Degtyarenko , Evgeny Mazur

Ab initio molecular dynamic method within the framework of density functional theory is applied to analyze the structural and electronic properties of crystalline molecular hydrogen at temperature 100\,K. Pressure, pair correlation function…

Materials Science · Physics 2022-01-12 I. Saitov

Based on ab initio calculations and metadynamics simulations, we predict that 2H-MoS$_2$, a layered insulator, will metallize under pressures in excess of 20-30 GPa. In the same pressure range, simulations and enthalpy optimization predict…

Materials Science · Physics 2015-06-12 Liliana Hromadová , Roman Martoňák , Erio Tosatti

We have studied solid hydrogen up to pressures of 300 GPa and temperatures of 350 K using density functional theory methods and have found "mixed structures" that are more stable than those predicted earlier. Mixed structures consist of…

Materials Science · Physics 2012-06-20 Chris J. Pickard , Miguel Martinez-Canales , Richard J. Needs

The crystal structure and electrical resistance of the structurally-layered EuFe2As2 have been studied up to 70 GPa and down to temperature of 10 K, using a synchrotron x-ray source and the designer diamond anvils. The room-temperature…

A systematic ab initio search for low enthalpy phases of disilane (Si_2H_6) at high pressures was performed based on the minima hopping method. We found a novel metallic phase of disilane with Cmcm symmetry, which is enthalpically more…

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