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We study the spectrum of vibrational modes in metal nanoparticles with a dielectric core. Vibrational modes are excited by the rapid heating of the particle lattice that takes place after laser excitation, and can be monitored by means of…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Arman S. Kirakosyan , Tigran V. Shahbazyan

The vibrational spectroscopy of semiconductor nanostructures can provide important information on their structure. In this work, experimental Raman and infrared spectra are compared with vibrational spectra of CdSe/CdS core/shell…

The discrete nature of the vibrational modes of an isolated nanometer-scale solid dramatically modifies its low-energy electron and phonon dynamics from that of a bulk crystal. However, nanocrystals are usually coupled--even if only…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Kelly R. Patton , Michael R. Geller

The coupling effects affecting the vibrations of two close nanostructures (e.g., two metal nanoplates or nanospheres separated by a thin dielectric layer) may considerably alter their vibrational eigenfrequencies, as demonstrated by several…

Applied Physics · Physics 2021-05-06 Jean Lermé , Jérémie Margueritat , Aurélien Crut

In this paper, we derive a series of exact analytical closed expressions to calculate the complex eigenfrequencies and the displacement for the corresponding eigenmodes of a viscoelastic (nano-)sphere in the presence of linear damping.…

Materials Science · Physics 2024-07-22 Markus Wenin , Andreas Windisch

The formation process of core-shell bimetallic nanoparticles synthesized by sputtering onto a substrate is observed in real time using an originally developed acoustic technique. The technique enables us to evaluate the structural change of…

Applied Physics · Physics 2022-03-04 Nobutomo Nakamura , Koji Matsuura , Akio Ishii , Hirotsugu Ogi

We discuss the rich vibrational dynamics of nanometer-scale semiconducting and insulating crystals as probed by localized electronic impurity states, with an emphasis on nanoparticles that are only weakly coupled to their environment. Two…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Michael R. Geller , W. M. Dennis , Vadim A. Markel , Kelly R. Patton , Daniel T. Simon , Ho-Soon Yang

We develop a theoretical framework, based on a multipole, quasi-static approach, for the prediction of the localized surface plasmon resonances in Fanoshells formed via geometrical symmetry-breaking in multilayer nanoshells consisting of a…

Optics · Physics 2022-01-12 Luke C. Ugwuoke , Tjaart P. J. Krüger

The acoustic vibrations of single monomers and dimers of gold nanoparticles were investigated by measuring for the first time their ultra-low frequency micro-Raman scattering. This experiment provides access not only to the frequency of the…

Vibrational spectra and normal modes of mechanically stable particle packings in three dimensions are analyzed over a range of compressions, from near the jamming transition, where the packings lose their rigidity, to far above it. At high…

Statistical Mechanics · Physics 2011-08-02 Leonardo E. Silbert , Andrea J. Liu , Sidney R. Nagel

The vibrational density of states of silicon nanoparticles in the range from 2.3 to 10.3 nm is studied with the help of molecular-dynamics simulations. From these simulations the vibrational density of states and frequencies of bulk-like…

Materials Science · Physics 2011-01-20 R. Meyer , D. Comtesse

We present a first-principles study on lattice vibrational modes of Si/Ge core-shell nanowires (NWs). In addition to quantum confinement, the internal strain induced by the lattice mismatch between core and shell contributes to significant…

Mesoscale and Nanoscale Physics · Physics 2012-07-04 Shouting Huang , Li Yang

The validity of the linear elasticity theory is examined at the nanometer scale by investigating the vibrational properties of silver and gold nanoparticles whose diameters range from about 1.5 to 4 nm. Comparing the vibration modes…

Materials Science · Physics 2022-03-18 Nicolas Combe , Lucien Saviot

Noble metal nanoparticles have been utilized for a vast amount of optical applications. For the applications that used metal nanoparticles as nanosensors and optical labeling, larger radiation damping is preferred (higher optical signal).…

Optics · Physics 2022-03-02 Yanhe Yang , Weihai Ni , Hao Xie , Jian You , Weixiang Ye

We report results of a systematic study of structural, vibrational and thermodynamical properties of 34-atom bimetallic nanoparticles from the AgnCu34-n family using model interaction potentials as derived from the embedded atom method and…

Materials Science · Physics 2009-11-13 Handan Yildirim , Abdelkader Kara , Talat. S Rahman

Multipolar plasmon oscillation frequencies and corresponding damping rates for nanospheres formed of the simplest free-electron metals are studied. The possibility of controlling plasmon features by choosing the size and dielectric…

Optics · Physics 2008-04-15 A. Derkachova , K. Kolwas

We study nonlinear resonance of coupled modes in nano-mechanical systems. To reveal the qualitative features of the dynamics, we consider the limiting cases, where the results can be obtained analytically. For 1:3 resonance, we find the…

Mesoscale and Nanoscale Physics · Physics 2017-02-03 O. Shoshani , S. W. Shaw , M. I. Dykman

Classical continuum elastic calculations show that the acoustic vibrational modes of an embedded nanoparticle can be lightly damped even when the longitudinal plane wave acoustic impedances $Z_o=\rho v_L$ of the nanoparticle and the matrix…

Materials Science · Physics 2007-05-23 Lucien Saviot , Daniel B. Murray

We use continuum elasticity theory to revise scaling laws for radial breathing-like and shear-like vibration modes in quasi-2D nanostructures including finite-width nanoribbons and finite-size thin circular discs. Such modes can be observed…

Mesoscale and Nanoscale Physics · Physics 2019-10-21 Dan Liu , Colin Daniels , Vincent Meunier , Arthur G. Every , David Tomanek

Acoustic vibrations of nanoparticles made of materials with anisotropic elasticity and nanoparticles with non-spherical shapes are theoretically investigated using a homogeneous continuum model. Cubic, hexagonal and tetragonal symmetries of…

Mesoscale and Nanoscale Physics · Physics 2009-06-02 Lucien Saviot , Daniel B. Murray
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