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We have determined the electronic and atomic structure of N doped TiO2 using a combination of hard x-ray photoelectron spectroscopy (HAXPES) and first- principles density functional theory calculations. Our results reveal that N doping of…

Materials Science · Physics 2015-05-14 Abdul K. Rumaiz , J. C. Woicik , E. Cockayne , H. Y. Lin , G. Hassnain Jaffari , S. Ismat Shah

The formation energies of the oxygen vacancy and titanium interstitial in rutile TiO2 were calculated by the screened exchange (sX) hybrid density functional method, which gives a band gap of 3.1 eV, close to the experimental value. The O…

Atomic and Molecular Clusters · Physics 2015-06-05 Hsin-Yi Lee , Stewart J. Clark , John Robertson

Metal-insulator transition materials such as NbO2 have generated much excitement in recent years for their potential applications in computing and sensing. NbO2 has generated considerable debate over the nature of the phase transition, and…

We present density-functional theory calculations of Ru 3d and O 1s surface core-level shifts (SCLSs) at an oxygen-rich Ru(0001) surface, namely for the O(1x1)/Ru(0001) chemisorption phase and for two surface terminations of fully oxidized…

Materials Science · Physics 2009-11-07 Karsten Reuter , Matthias Scheffler

Cu$_2$O has appealing properties as an electrode for photo-electrochemical water splitting, yet its practical performance is severely limited by inefficient charge extraction at the interface. Using hybrid DFT calculations, we investigate…

Materials Science · Physics 2021-03-09 Chiara Ricca , Lisa Grad , Matthias Hengsberger , Jürg Osterwalder , Ulrich Aschauer

High value of magnetic moment 0.08 emu/g at room temperature for SnO_2 nanoparticles (NPs) was observed. Surface functionalization with octadecyltrichlorosilane (OTS) enhanced the saturation magnetic moment of NPs to an anomalously high…

Materials Science · Physics 2015-09-01 Venkataramana Bonu , Arindam Das , Manas Sardar , Sandip Dhara , Ashok Kumar Tyagi

Modifications of the electronic bands of thin FeSe films due to oxygen vacancies in the supporting SrTiO 3 (001) substrate - and the interplay with spin-orbit coupling, magnetism, and epitaxy - are investigated by first-principles supercell…

Materials Science · Physics 2017-01-11 M. X. Chen , Zhuozhi Ge , Y. Y. Li , D. F. Agterberg , L. Li , M. Weinert

Correlated band theory is employed to investigate the magnetic and electronic properties of different arrangements of oxygen di- and tri-vacancy clusters in SrTiO$_3$. Hole and electron doping of oxygen deficient SrTiO$_3$ yields various…

Materials Science · Physics 2016-03-30 Alejandro Lopez-Bezanilla , P. Ganesh , Peter B. Littlewood

We provide a first-principles description of the crystalline and oxygen-deficient Ta2O5 using refined computational methods and models. By performing calculations on a number of candidate structures, we determined the low-temperature phase…

Materials Science · Physics 2012-11-05 Yong Yang , Ho-Hyun Nahm , Osamu Sugino , Takahisa Ohno

The quasi two-dimensional electron gas (q-2DEG) at oxide interfaces provides a platform for investigating quantum phenomena in strongly correlated electronic systems. Here, we study the transport properties at the high-mobility…

Strongly Correlated Electrons · Physics 2017-06-30 K. Han , Z. Huang , S. W. Zeng , M. Yang , C. J. Li , W. X. Zhou , X. Renshaw Wang , T. Venkatesan , J. M. D. Coey , M. Goiran , W. Escoffier , Ariando

A high-frequency optical phonon mode of SrTiO3 (STO) was found to assist the high-temperature superconductivity observed recently at the interface between monolayer FeSe and STO substrate. However, the origin of this mode is not clear.…

Superconductivity · Physics 2015-07-02 Yun Xie , Hai-Yuan Cao , Yang Zhou , Shiyou Chen , Hongjun Xiang , Xin-Gao Gong

We discuss the applicability of the pseudopotential-like self-interaction correction (pSIC) to the study of defect energetics and electronic structure of In2O3. Our results predict that substitutional (at oxygen sites) and interstitial (at…

Materials Science · Physics 2016-06-24 Juan J. Meléndez , Małgorzata Wierzbowska

Point defects in diamond are of high interest as candidates for realizing solid state quantum bits, bioimaging agents, or ultrasensitive electric or magnetic field sensors. Various artificial diamond synthesis methods should introduce…

Materials Science · Physics 2016-09-14 Gergő Thiering , Adam Gali

The consideration of oxygen vacancies influence on the relaxors with perovskite structure was considered in the framework of Landau-Ginzburg-Devonshire phenomenological theory. The theory applicability for relaxors is based on the existence…

HfO$_2$-based ferroelectrics have emerged as promising materials for advanced nanoelectronics, with their robust polarization and silicon compatibility making them ideal for high-density, non-volatile memory applications. Oxygen vacancies,…

Materials Science · Physics 2026-01-06 Yudi Yang , Wooil Yang , Young-Woo Son , Shi Liu

We perform ab initio calculations, based on density functional theory, of substitutional and vacancy defects in the monoclinic hafnium oxide (m-HfO2) and alpha-quartz (SiO2). The neutral oxygen vacancies and substitutional Si and Hf defects…

Materials Science · Physics 2009-11-10 W. L. Scopel , Antonio J. R. da Silva , W. Orellana , A. Fazzio

Hydroxyapatite (HAp) is a widely used biomaterial for the preparation of bone and dental implants. Despite the relevance of HAp in medicine, exciting applications involving this material as a bio-compatible photocatalyst, depend on how well…

Materials Science · Physics 2019-03-05 Vladimir S. Bystrov , Leon A. Avakyan , Ekaterina V. Paramonova , José Coutinho

An unusual Fe-H bonding rather than conventional OH bonding is identified at Fe3O4 (001) surface. This abnormal behavior is associated with the oxygen vacancies which exist on the surface region but also penetrate deep into the bulk Fe3O4.…

Strongly Correlated Electrons · Physics 2016-11-23 Fangyang Liu , Chen Chen , Hangwen Guo , Mohammad Saghayezhian , Gaomin Wang , Lina Chen , Wei Chen , Jiandi Zhang , E. W. Plummer

The observation of metallic interface between band insulators LaAlO$_3$ and SrTiO$_3$ has led to massive efforts to understand the origin of the phenomenon as well as to search for other systems hosting such two dimensional electron gases…

The energies, widths, and shapes of features observed in the total energy distributions in field emission from W(100) and W(111) are compared with the results of a full-potential LAPW calculation of the surface density of states based on a…

Materials Science · Physics 2011-05-27 Z. A. Ibrahim , M. J. G. Lee
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