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We have used Raman scattering to investigate the magnetic excitations and lattice dynamics in the prototypical spin-orbit Mott insulators Sr2IrO4 and Sr3Ir2O7. Both compounds exhibit pronounced two-magnon Raman scattering features with…

Strongly Correlated Electrons · Physics 2016-04-06 H. Gretarsson , N. H. Sung , M. Hoeppner , B. J. Kim , B. Keimer , M. Le Tacon

We reported two-magnon Raman scattering from La_{1.9}Sr_{0.1}CuO_4, which has a suppressed Tc=12 K, as the temperature is lowered below 37 K and an ordered spin phase is formed. The two-magnon Raman intensity increases with decreasing…

Superconductivity · Physics 2016-08-15 Y. Lin , J. Sichelschmidt , J. E. Eldridge , T. Wahlbrink , S. -W. Cheong

We present results of low-temperature two-magnon resonance Raman excitation profile measurements for single layer Sr_2CuO_2Cl_2 and bilayer YBa_2Cu_3O_{6 + \delta} antiferromagnets over the excitation region from 1.65 to 3.05 eV. These data…

Condensed Matter · Physics 2009-10-28 G. Blumberg , P. Abbamonte , M. V. Klein , L. L. Miller , W. C. Lee , D. M. Ginsberg

We investigated temperature dependent Raman spectra of the one-dimensional spin-ladder compound SrCu2O3. At low temperatures a two-magnon peak is identified at 3160+/-10 cm^(-1) and its temperature dependence analyzed in terms of a thermal…

Strongly Correlated Electrons · Physics 2008-01-09 A. Gössling , U. Kuhlmann , C. Thomsen , A. Löffert , C. Gross , W. Assmus

We report detailed neutron scattering studies on Ba$_2$Cu$_3$O$_4$Cl$_2$. The compound consists of two interpenetrating sublattices of Cu, labeled as Cu$_{\rm A}$ and Cu$_{\rm B}$, each of which forms a square-lattice Heisenberg…

Ba$_2$Cu$_3$O$_4$Cl$_2$ has two inter-penetrating square Cu sublattices, one with square root 2 times the in-plane spacing of the other. Isotropic magnetic interactions between the two sublattices are completely frustrated. Quantum…

Strongly Correlated Electrons · Physics 2009-11-11 M. K. Ramazanoglu , P. S. Clegg , S. Wakimoto , R. J. Birgeneau , S. Noro

Using Raman scattering, the quasi-two dimensional organic superconductor k-(BEDT-TTF)2Cu[N(CN)2]Br (T_c=11.8 K) and the related antiferromagnet k-(BEDT-TTF)2Cu[N(CN)2]Cl are studied. Raman scattering provides unique spectroscopic…

Strongly Correlated Electrons · Physics 2015-10-21 Natalia Drichko , Rudi Hackl , John A. Schlueter

We present an investigation of charge-compensated antiferromagnetic (Ca$_{x}$La$_{1-x}$)(Ba$_{1.75-x}$La$_{0.25+x}$)Cu$_{3}$O$_{y}$ single crystals using Raman scattering as well as muon spin rotation. In this system the parameter $x$…

We report the measurements of the pseudodielectric function, far-infrared reflectivity and Raman scattering spectra in Sr_{14}Cu_{24}O_{41} single crystal. We study the lattice and the spin dynamics of the Cu$_2$O$_3$ spin ladders and…

Strongly Correlated Electrons · Physics 2009-10-31 Z. V. Popović , M. J. Konstantinović , V. A. Ivanov , O. P. Khuong , R. Gajić , A. Vietkin , V. V. Moshchalkov

For CaCu$_{3}$Ti$_{4}$O$_{12}$ -- an insulator that exhibits a giant dielectric response above 100 K -- Cu$^{2+}$ antiferromagnetic spin ordering has been investigated by magnetic Raman scattering and magnetization measurements. Below the…

Strongly Correlated Electrons · Physics 2007-05-23 A. Koitzsch , G. Blumberg , A. Gozar , B. Dennis , A. P. Ramirez , S. Trebst , Shuichi Wakimoto

Using Raman spectroscopy, we investigate the lattice phonons, magnetic excitations, and magneto-elastic coupling in the distorted triangular-lattice Heisenberg antiferromagnet alpha-SrCr2O4, which develops helical magnetic order below 43 K.…

Raman experiments on the spin-Peierls compound CuGeO$_3$ and the substituted (Cu$_{1- x}$,Zn$_x$)GeO$_3$ and Cu(Ge$_{1-x}$,Ga$_x$)O$_3$ compounds were performed in order to investigate the response of specific magnetic excitations of the…

We present and analyze Raman spectra of the Mott insulator Ca$_2$RuO$_4$, whose quasi-two-dimensional antiferromagnetic order has been described as a condensate of low-lying spin-orbit excitons with angular momentum $J_{eff}=1$. In the…

We propose a theory of two-magnon Raman scattering from the insulating parent compounds of high-T$_c$ superconductors, which contains information not only on magnetism, but also on the electronic properties in these materials. We use spin…

Condensed Matter · Physics 2016-08-31 Andrey V. Chubukov , David M. Frenkel

We report the first observation of soft-x-ray scattering from spin fluctuations in a high-Tc parent compound. An antiferromagnetic charge transfer insulator, CaCuO2, was irradiated by Cu M-edge soft x-rays. Ultra-high resolution…

We use Raman scattering to study spin, charge, and lattice dynamics in various phases of Ca_{2-x}Sr_{x}RuO_{4}. With increasing substitution of Ca by Sr in the range 0 =< x < 0.2, we observe (1) evidence for an increase of the…

Strongly Correlated Electrons · Physics 2009-11-10 H. Rho , S. L. Cooper , S. Nakatsuji , H. Fukazawa , Y. Maeno

The ferrimagnetic spinels MnB2O4 (B = Mn,V) exhibit a similar series of closely spaced magnetic and structural phase transitions at low temperatures, reflecting both magnetic frustration and a strong coupling between the spin and lattice…

Strongly Correlated Electrons · Physics 2015-01-28 S. L. Gleason , T. Byrum , Y. Gim , A. Thaler , P. Abbamonte , G. J. MacDougall , L. W. Martin , H. D. Zhou , S. L. Cooper

We report inelastic light scattering studies on Ca(Fe0.97Co0.03)2As2 in a wide spectral range of 120-5200 cm-1 from 5K to 300K, covering the tetragonal to orthorhombic structural transition as well as magnetic transition at Tsm ~ 160K. The…

Superconductivity · Physics 2014-07-11 Pradeep Kumar , D. V. S. Muthu , L. Harnagea , S. Wurmehl , B. Büchner , A. K. Sood

We suggest, and demonstrate, a systematic approach to the study of cuprate superconductors, namely, progressive change of ion size in order to systematically alter the interaction strength and other key parameters. R(Ba,Sr)$_2$Cu$_3$O$_y$…

By means of resonant inelastic x-ray scattering at the Cu L$_3$ edge, we measured the spin wave dispersion along $\langle$100$\rangle$ and $\langle$110$\rangle$ in the undoped cuprate Ca$_2$CuO$_2$Cl$_2$. The data yields a reliable estimate…

Strongly Correlated Electrons · Physics 2017-04-12 B. W. Lebert , M. P. M. Dean , A. Nicolaou , J. Pelliciari , M. Dantz , T. Schmitt , R. Yu , M. Azuma , J-P. Castellan , H. Miao , A. Gauzzi , B. Baptiste , M. d'Astuto
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