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The ordering of cations in the B sublattice remains a challenging issue in double perovskites. In this work, a combined experimental and theoretical approach was employed to investigate the Co/Nb distribution in Ca$_2$CoNbO$_6$ and its…

Using density functional calculations we explore the properties of as-yet-unsynthesized $3d - 5d$ ordered double perovskites ($A_2BB'$O$_6$) with highly polarizable Bi$^{3+}$ ions on the $A$ site. We find that the Bi$_2$NiReO$_6$ and…

Materials Science · Physics 2015-03-13 Marjana Ležaić , Nicola A. Spaldin

Here we show that the B-site cation (Fe/Mo) ordering in the double-perovskite magnetoresistor, Sr2FeMoO6, is controlled by either kinetics or thermal equilibrium depending on the temperature range. In order to enhance the ordering, long…

Strongly Correlated Electrons · Physics 2007-05-23 T. Shimada , J. Nakamura , T. Motohashi , H. Yamauchi , M. Karppinen

Here, the first-principles predictions on the structural stability, magnetic behavior and electronic structure of B-site ordered double perovskite Nd$_{2}$FeCrO$_{6}$ have been reported. Initially, the ground state of the parent single…

Materials Science · Physics 2022-01-10 M. D. I. Bhuyan , Rana Hossain , Ferdous Ara , M. A. Basith

We report investigations of the structural, magnetic, electrical transport and thermal properties of five compositions of the metallic perovskite GdRh$_3$C$_{1-x}$B$_x$ ($0.00 \le x \le 1.00$). Our results show that all the five…

Strongly Correlated Electrons · Physics 2020-09-09 Abhishek Pandey , A. K. Singh , Shovan Dan , K. Ghosh , I. Das , S. Tripathi , U. Kumar , R. Ranganathan , D. C. Johnston , Chandan Mazumdar

We present theoretical study of ordering phenomena in binary $C_{1-x}B_{x}$, $C_{1-x}N_{x}$ and ternary $B_{x}C_{1-x-y}N_{y}$ alloys forming two-dimensional, graphene-like systems. For calculating energy of big systems (20 000 atoms in the…

Mesoscale and Nanoscale Physics · Physics 2017-01-11 Agnieszka Jamróz , Jacek A. Majewski

The usual classical behaviour of S = 3/2, B-site ordered double perovskites generally results in simple, commensurate magnetic ground states. In contrast, heat capacity and neutron powder diffraction measurements for the S = 3/2 systems…

Strongly Correlated Electrons · Physics 2015-06-11 A. A. Aczel , D. E. Bugaris , L. Li , J. -Q. Yan , C. de la Cruz , H. -C. zur Loye , S. E. Nagler

We show that the magnetism of double perovskite AFe_{1/2}M_{1/2}O_3 systems may be described by the Heisenberg model on the simple cubic lattice, where only half of sites are occupied by localized magnetic moments. The nearest-neighbor…

Materials Science · Physics 2015-01-16 R. O. Kuzian , I. V. Kondakova , A. -M. Dare , V. V. Laguta

Perovskite-like oxides $AB'_{1/2}B''_{1/2}$O$_3$ may experience different ordering degrees of $B$-cations, that can be varied by suitable synthesis conditions or post-synthesis treatment. In this work the earlier proposed statistical model…

Materials Science · Physics 2020-03-20 N. V. Ter-Oganessian , V. P. Sakhnenko

Vacancy-ordered double perovskites (A$_2$BX$_6$), being one of the environmentally friendly and stable alternatives to lead halide perovskites, have garnered considerable research attention in the scientific community. However, their…

Materials Science · Physics 2023-05-02 Preeti Bhumla , Manjari Jain , Sajjan Sheoran , Saswata Bhattacharya

Multiferroics are a unique class of materials where magnetic and ferroelectric orders coexist. The research on multiferroics contributes significantly to the fundamental understanding of the strong correlations between different material…

Materials Science · Physics 2021-11-03 A. C. Garcia-Castro , Yanjun Ma , Zachary Romestan , Eric Bousquet , Cheng Cen , Aldo H. Romero

Detailed magnetic properties of the compound Sr2YbRuO6 are presented here. The compound belongs to the family of double perovskites forming a monoclinic structure. Magnetization meas-urements reveal clear evidence for two components of…

Strongly Correlated Electrons · Physics 2008-09-29 Ravi P. Singh , C. V. Tomy

We construct and analyze a microscopic model for insulating rock salt ordered double perovskites, with the chemical formula A$_2$BB'O$_6$, where the B' atom has a 4d$^1$ or 5d$^1$ electronic configuration and forms a face centered cubic…

Strongly Correlated Electrons · Physics 2018-10-08 Gang Chen , Rodrigo Pereira , Leon Balents

We studied structural and magnetic properties of a series of insulating double perovskite compounds, La$_{2-x}$Sr$_{x}$CuRuO$_{6}$ (0 $\le$ x $\le$ 1), representing doping via \textit{A}-site substitution. The end members…

Strongly Correlated Electrons · Physics 2012-09-19 P. Anil Kumar , R. Mathieu , R. Vijayaraghavan , Subham Majumdar , Olof Karis , P. Nordblad , Biplab Sanyal , Olle Eriksson , D. D. Sarma

Double perovskite compounds containing 5d transition metal elements have been extensively studied as platforms for multipolar order phenomena stemming from spin-orbit-entangled 5d electrons. In this study, we examine the interplay between…

Strongly Correlated Electrons · Physics 2025-04-02 Koki Shibuya , Daigorou Hirai , Koshi Takenaka

We present a neutron powder diffraction study of the monoclinic double perovskite systems Nd2NaB'O6 (B' = Ru, Os), with magnetic atoms occupying both the A and B' sites. Our measurements reveal coupled spin ordering between the Nd and B'…

Strongly Correlated Electrons · Physics 2013-07-25 A. A. Aczel , D. E. Bugaris , J. Yeon , C. de la Cruz , H. -C. zur Loye , S. E. Nagler

Double-perovskite oxides that contain both 3d and 5d transition metal elements have attracted growing interest as they provide a model system to study the interplay of strong electron interaction and large spin-orbit coupling (SOC). Here,…

Strongly Correlated Electrons · Physics 2016-09-01 W. K. Zhu , J. -C. Tung , W. Tong , L. Ling , M. Starr , J. M. Wang , W. C. Yang , Y. Losovyj , H. D. Zhou , Y. Q. Wang , P. -H. Lee , Y. -K. Wang , Chi-Ken Lu , S. X. Zhang

Recent experimental and theoretical work has shown that the double perovskite NaLaMnWO$_6$ exhibits antiferromagnetic ordering owing to the Mn $d$ states, and computational studies further predict it to exhibit a spontaneous electric…

Materials Science · Physics 2015-11-18 Joshua Young , Alessandro Stroppa , Silvia Picozzi , James M. Rondinelli

We report the comprehensive experimental results identifying the magnetic spin ordering and the magnetization dynamics of a double perovskite Pr2CoFeO6 by employing the (dc and ac) magnetization, powder neutron diffraction (NPD) and X-ray…

We use a group theoretical approach to enumerate the possible couplings between magnetism and ferroelectric polarisation in the parent $Pm\bar{3}m$ perovskite structure. We show that third order magnetoelectric coupling terms must always…

Materials Science · Physics 2018-05-18 Mark S. Senn , Nicholas C. Bristowe