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We have investigated the electronic structure of the transition metal oxide Ca3Ru2O7 within density functional theory using the generalized gradient approximation while considering strong Coulomb correlations in the framework of the fully…

Strongly Correlated Electrons · Physics 2024-04-22 V. N. Antonov , D. A. Kukusta , L. V. Bekenov

We employ a combination of density functional theory and dynamical mean-field theory to investigate the electronic structure of the recently synthesized insulator BaCrO$_3$. Our calculations show that Hund's coupling is responsible for…

Strongly Correlated Electrons · Physics 2014-12-31 G. Giovannetti , M. Aichhorn , M. Capone

Direct analytical and numerical calculation show that two-electron atomic configuration can be unstable with respect to a static or dynamic shift of the electron shells. This enables to develop a so called non-rigid shell model for a…

Strongly Correlated Electrons · Physics 2007-05-23 Yu. D. Panov , A. S. Moskvin

A survey is presented of current investigations of the impact of band structure effects on various aspects of the interaction of charged particles with real solids. The role that interband transitions play in the decay mechanism of bulk…

Materials Science · Physics 2009-10-31 J. M. Pitarke , I. Campillo

We explore quantum correlations, in particular, quantum entanglement, among vibrational phonon modes as well as between electronic and vibrational degrees of freedom in molecular systems, described by Jahn-Teller mechanism. Specifically, to…

Quantum Physics · Physics 2022-02-23 Ali Pedram , Onur Pusuluk , Özgür E. Müstecaplıoğlu

Recently, it was established that a two-dimensional electron system can arise at the interface between two oxide insulators LaAlO3 and SrTiO3. This paradigmatic example exhibits metallic behaviour and magnetic properties between…

Strongly Correlated Electrons · Physics 2016-11-28 I. I. Piyanzina , Yu. V. Lysogorskiy , I. I. Varlamova , A. G. Kiiamov , T. Kopp , V. Eyert , O. V. Nedopekin , D. A. Tayurskii

Despite the recent interest in "organic spintronics", the dominant spin relaxation mechanism of electrons or holes in an organic compound semiconductor has not been conclusively identified. There have been sporadic suggestions that it might…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 Supriyo Bandyopadhyay

We have investigated the electron correlation effect on the electronic structures and transport properties of the iron-based superconductors using the density functional theory (DFT) and dynamical mean field theory (DMFT). By considering…

Strongly Correlated Electrons · Physics 2011-08-19 Hyo Seok Ji , Geunsik Lee , Ji Hoon Shim

Heterostructured material systems devoid of ferroic components are presumed not to display ordering associated with ferroelectricity. In heterostructures composed of transition metal oxides, however, the disruption introduced by an…

Strongly Correlated Electrons · Physics 2012-09-25 K. Rogdakis , J. W. Seo , Z. Viskadourakis , Y. Wang , L. F. N. Ah Qune , E. Choi , J. D. Burton , E. Y. Tsymbal , J. Lee , C. Panagopoulos

We introduce a theory that exposes the fundamental and previously overlooked connection between the correlation among electrons and the degree of quantum coherence of electronic states in matter. For arbitrary states, the effects only…

Quantum Physics · Physics 2016-04-21 Arnab Kar , Liping Chen , Ignacio Franco

Structural alpha relaxation in liquid orthoterphenyl is studied by means of coherent neutron time-of-flight and backscattering spectroscopy over a large temperature range. Not only amplitude and relaxation time but also the spectral line…

Statistical Mechanics · Physics 2011-04-05 A. Toelle , H. Schober , J. Wuttke , F. Fujara

Relaxor ferroelectrics have been a focus of intense attention due to their anomalous dielectric characteristics, diffuse phase transitions, and strong piezoelectricity. Understanding the structure and dynamics of relaxors has been one of…

Materials Science · Physics 2013-12-09 Hiroyuki Takenaka , Ilya Grinberg , Andrew M. Rappe

The bonding pattern of a covalent semiconductor is disrupted when a surface is cut while keeping a rigid (truncated bulk) geometry. The covalent bonds are partly reformed (with a sizeable energy gain) when reconstruction is allowed. We show…

Materials Science · Physics 2009-10-31 L. De Santis , R. Resta

We present a new theory for partitioning simulations of periodic and solid-state systems into physically sound atomic contributions at the level of Kohn-Sham density functional theory. Our theory is based on spatially localized linear…

Chemical Physics · Physics 2024-10-01 Luna Zamok , Janus J. Eriksen

A framework for developing new approximate electronic structure methods is presented, in which the correlation energy of a many-electron system in the ground state is computed as in the single-reference second-order many-body perturbation…

Chemical Physics · Physics 2011-06-15 Dimitri Laikov

In this paper we present an accurate numerical scheme for extracting inter-atomic exchange parameters ($J_{ij}$) of strongly correlated systems, based on first-principles full-potential electronic structure theory. The electronic structure…

Strongly Correlated Electrons · Physics 2015-03-11 Y. O. Kvashnin , O. Grånäs , I. Di Marco , M. I. Katsnelson , A. I. Lichtenstein , O. Eriksson

Relaxor ferroelectrics are complex oxide materials which are rather unique to study the effects of compositional disorder on phase transitions. Here, we study the effects of quenched cubic random electric fields on the lattice instabilities…

Materials Science · Physics 2017-06-14 J. R. Arce-Gamboa , G. G. Guzmán-Verri

We show that quantum correlations induced by electron-electron interactions in the presence of random impurity scattering can play an important role in the thermal stabilization of amorphous Hume-Rothery systems: When there is strong…

Materials Science · Physics 2009-10-31 Johann Kroha

A crucial factor determining charge transport in organic semiconductors is the electronic coupling between the molecular constituents, which is heavily influenced by the relative arrangement of the molecules. This renders quinacridone, with…

Materials Science · Physics 2019-10-16 Christian Winkler , Andreas Jeindl , Florian Mayer , Oliver T. Hofmann , Ralf Tonner , Egbert Zojer

Atomic properties such as field shift constants, magnetic dipole and electric quadrupole hyperfine structure constants, Land\'e $g_J$ factors, and electric quadrupole moments that are described by electronic operators with different ranks…

Atomic Physics · Physics 2018-03-14 Pradeep Kumar , Cheng-Bin Li , B. K. Sahoo
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