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We present a kinetic energy tensor that unifies a scalar kinetic energy density commonly used in meta-Generalized Gradient Approximation functionals and the vorticity density that appears in paramagnetic current-density-functional theory.…

Chemical Physics · Physics 2018-11-14 Sangita Sen , Erik I. Tellgren

The paper is concerned with the sparse approximation of functions having hybrid regularity borrowed from the theory of solutions to electronic Schr\"odinger equations due to Yserentant [43]. We use hyperbolic wavelets to introduce…

Numerical Analysis · Mathematics 2022-03-21 Glenn Byrenheid , Janina Hübner , Markus Weimar

Large atomic-orbital (AO) basis sets of at least triple and preferably quadruple-zeta (QZ) size are required to adequately converge Kohn-Sham density functional theory (DFT) calculations towards the complete basis set limit. However,…

Chemical Physics · Physics 2025-12-02 Anthony O. Lara , Justin J. Talbot , Zhe Wang , Martin Head-Gordon

Electronic-structure functionals that include screening effects, such as Hubbard or Koopmans' functionals, require to describe the response of a system to the fractional addition or removal of an electron from an orbital or a manifold.…

Computational Physics · Physics 2018-10-02 Nicola Colonna , Ngoc Linh Nguyen , Andrea Ferretti , Nicola Marzari

To explore the applicability of orbital-free density functional theory (OF-DFT) in nuclear physics, we perform a systematic benchmark of 36 one-point kinetic energy density functionals, which are originally developed for electron systems in…

Nuclear Theory · Physics 2026-05-20 Tian Shuai Shang , Jian Li , Haozhao Liang , Xinhui Wu , Cheng Ma , Wenhui Mi , Xuecheng Shao , Yanchao Wang

Locality of compact one-electron orbitals expanded strictly in terms of local subsets of basis functions can be exploited in density functional theory (DFT) to achieve linear growth of computation time with systems size, crucial in…

Computational Physics · Physics 2021-10-01 Yifei Shi , Jessica Karaguesian , Rustam Z. Khaliullin

We introduce affordable computational strategies for calculating orbital and pair-orbital energies in atomic and molecular systems. Our methods are based on the pair Coupled Cluster Doubles (pCCD) ansatz and its orbital-optimized variant.…

Chemical Physics · Physics 2025-02-06 Seyedehdelaram Jahani , Somayeh Ahmadkhani , Katharina Boguslawski , Paweł Tecmer

Knowledge of the properties of the exchange-correlation functional in the form $\frac 1\lambda v_{xc}([\rho _\lambda ],\frac{{\bf r}}\lambda )$, where $\rho _\lambda ({\bf r})=$ $\lambda ^3\rho (\lambda {\bf r}),$ is important when…

Condensed Matter · Physics 2009-10-28 Daniel Joubert , Mel Levy

The Bertrand theorem concluded that; the Kepler potential, and the isotropic harmonic oscillator potential are the only systems under which all the orbits are closed. It was never stressed enough in the physical or mathematical literature…

Classical Physics · Physics 2019-04-03 Munir Al-Hashimi

The Hartree-Fock-Rothaan equations are solved for He-like ions using the iterative self-consistent method. New complete and orthonormal sets of exponential-type orbitals are employed as the basis. These orbitals satisfy the orthonormality…

Quantum Physics · Physics 2025-06-26 A. Bagci , P. E. Hoggan

We introduce a method for solving a self consistent electronic calculation within localized atomic orbitals, that allows us to converge to the complete basis set (CBS) limit in a stable, controlled, and systematic way. We compare our…

Strongly Correlated Electrons · Physics 2015-05-19 S. Azadi , C. Cavazzoni , S. Sorella

We study orbit-finite systems of linear equations, in the setting of sets with atoms. Our principal contribution is a decision procedure for solvability of such systems. The procedure works for every field (and even commutative ring) under…

Computation and Language · Computer Science 2024-02-28 Arka Ghosh , Piotr Hofman , Sławomir Lasota

A method for the calculation of elastic constants in the NVT ensamble, using molecular dynamics (MD) simulation with a realistic many-body embedded-atom-model (EAM) potential, is studied in detail. It is shown that in such NVT MD…

Materials Science · Physics 2021-06-30 Menahem Krief , Yinon Ashkenazy

We present a novel theory and implementation for computing coupled electronic and quantal nuclear subsystems on a single potential energy surface, moving beyond the standard Born-Oppenheimer (BO) separation of nuclei and electrons. We…

Chemical Physics · Physics 2021-11-15 Ziyong Chen , Jun Yang

We calculate the one-loop effective potential at finite temperature for a system of massless scalar fields with quartic interaction $\lambda\phi^4$ in the framework of the boundary effective theory (BET) formalism. The calculation relies on…

High Energy Physics - Phenomenology · Physics 2011-06-30 A. Bessa , C. A. A. de Carvalho , E. S. Fraga , F. Gelis

We introduce an orbital-optimized double-hybrid (DH) scheme using the optimized-effective-potential (OEP) method. The orbitals are optimized using a local potential corresponding to the complete exchange-correlation energy expression…

Exact relations are derived for the Fermi Hubbard spectral weight function for infinite U at zero temperature in the thermodynamic limit for any dimension,any lattice structure and general hopping matrix. These relations involve moments of…

Strongly Correlated Electrons · Physics 2018-12-11 Donald M. Esterling

The universal functional of Hohenberg-Kohn is given as a coupling-constant integral over the density as a functional of the potential. Conditions are derived under which potential-functional approximations are variational. Construction via…

Other Condensed Matter · Physics 2011-06-13 Attila Cangi , Donghyung Lee , Peter Elliott , Kieron Burke , E. K. U. Gross

Background: Calculating microscopic effective interactions (optical potentials) for elastic nucleon-nucleus scattering has already in the past led to a large body of work. For first-order calculations a nucleon-nucleon (\textit{NN})…

Nuclear Theory · Physics 2020-09-16 M. Burrows , R. B. Baker , Ch. Elster , S. P. Weppner , K. D. Launey , P. Maris , G. Popa

Solving the many-electron problem, even approximately, is one of the most challenging and simultaneously most important problems in contemporary condensed matter physics with various connections to other fields. The standard approach is to…

Strongly Correlated Electrons · Physics 2026-04-10 Jonas B. Profe , Jakša Vučičević , P. Peter Stavropoulos , Malte Rösner , Roser Valentí , Lennart Klebl