Related papers: Dissipative Two-Electron Transfer
We develop a computationally inexpensive model to examine the dynamics of boson-assisted electron relaxation in solids, studying nonequilibrium dynamics in a metal, in a nodal superconductor with a stationary density of states, and in a…
We analyze the heat transfer between two metals separated by a vacuum gap in the extreme near-field regime. In this cross-over regime between conduction and radiation, heat exchanges are mediated by photon, phonon and electron tunneling. We…
We study two-mode bosonic engines undergoing an Otto cycle. The energy exchange between the two bosonic systems is provided by a tunable unitary bilinear interaction in the mode operators modeling frequency conversion, whereas the cyclic…
The advancement of fabrication and lithography techniques of semiconductors have made it possible to study bi-layer systems made of two electronic layers separated by distances of several hundred Angstroms. In this situation the electrons…
Driven-dissipative light-matter systems can exhibit collective nonequilibrium phenomena due to loss and gain processes on the one hand and effective photon-photon interactions on the other hand. As generic example we study a bosonic lattice…
We develop a mathematically rigorous theory for the quantum transfer processes in degenerate donor-acceptor dimers in contact with a thermal environment. We calculate explicitly the transfer rates and the acceptor population efficiency. The…
Ferromagnetic transition in double-exchange systems is studied by non-equilibrium relaxation technique combined with Monte Carlo calculations. Critical temperature and critical exponents are estimated from relaxation of the magnetic moment.…
We apply the hierarchical equations of motion technique to analyzing nonequilibrium heat transport in a spin-boson type model, whereby heat transfer through a central spin is mediated by an intermediate pair of coupled harmonic oscillators.…
The lowest-lying states of LiH have been widely used to develop and calibrate many different methods in quantum mechanics. In this paper we show that the electron-transfer processes occurring in these two states are a difficult test for…
We have reexamined the thermally induced Co(NH_3)_6^{2+/3+} [Co(II/III)] redox reaction using the first principles density-functional-theory method, semiclassical Marcus theory, and known charge transfer parameters. We confirm a previously…
We investigate full counting statistics of quantum heat transfer in a collective-qubit system, constructed by multi-qubits interacting with two thermal baths. The nonequilibrium polaron-transformed Redfield approach embedded with an…
We consider the dependence of the electron transfer in photosynthetic complexes on correlation properties of random fluctuations of the protein environment. The electron subsystem is modeled by a finite network of connected electron…
Ultrafast multistage electron transfer (ET) in molecular systems with multiple redox centers is fundamental to photochemical energy conversion, including processes in natural photosynthesis, molecular optoelectronics, and organic…
We present a computer simulation study of a disordered two-dimensional system of localized interacting electrons at thermal equilibrium. It is shown that the configuration of occupied sites within the Coulomb gap persistently changes at…
Stimulated emission and absorption are two fundamental processes of light-matter interaction, and the coefficients of the two processes should be equal in general. However, we will describe a generic method to realize significant difference…
We investigate theoretically the stochastic dynamics of Resonance Electronic Energy Transfer (RET), in a bi-dimensional overexcited ensemble of donor and acceptor molecules. We find that, after initial optical excitation of all the donors,…
Biological systems are known to communicate by diffusing chemical signals in the surrounding medium. However, most of the recent literature has neglected the electron transfer mechanism occurring amongst living cells, and its role in…
We present Quantum Monte Carlo simulations of the soft-core bosonic Hubbard model with a ring exchange term K. For values of K which exceed roughly half the on-site repulsion U, the density is a non-monotonic function of the chemical…
Time modulation opens new avenues for light, heat control, and energy harvesting, yet the impact of nonequilibrium dynamics of microscopic particles remains largely unexplored. We develop a microscopic theory to describe radiative heat…
Understanding non-equilibrium heat transport is crucial for controling heat flow in nano-scale systems. We study thermal energy transfer in a generalized non-equilibrium spin-boson model (NESB) with non-commutative system-bath coupling…