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We numerically study thermodynamic and structural properties of the one-component Gaussian core model (GCM) at very high densities. The solid-fluid phase boundary is carefully determined. We find that the density dependence of both the…

Soft Condensed Matter · Physics 2015-05-27 Atsushi Ikeda , Kunimasa Miyazaki

We investigated the equilibrium properties of a one-dimensional system of classical particles which interact in pairs through a bounded repulsive potential with a Gaussian shape. Notwithstanding the absence of a proper fluid-solid phase…

Soft Condensed Matter · Physics 2012-01-11 Cristina Speranza , Santi Prestipino , Paolo V. Giaquinta

We trace with unprecedented numerical accuracy the phase diagram of the Gaussian-core model, a classical system of point particles interacting via a Gaussian-shaped, purely repulsive potential. This model, which provides a reliable…

Soft Condensed Matter · Physics 2011-10-25 S. Prestipino , F. Saija , P. V. Giaquinta

We study the structural and thermodynamic properties of a model of point particles interacting by means of a Gaussian pair potential first introduced by Stillinger [Stillinger F H 1976 J. Chem. Phys. 65, 3968]. By employing integral…

Soft Condensed Matter · Physics 2009-10-31 A. Lang , C. N. Likos , M. Watzlawek , H. Lowen

We use molecular dynamics simulations to investigate dynamic heterogeneities and the potential energy landscape of the Gaussian core model (GCM). Despite the nearly Gaussian statistics of particles' displacements, the GCM exhibits giant…

Statistical Mechanics · Physics 2016-04-13 Daniele Coslovich , Atsushi Ikeda , Kunimasa Miyazaki

Pair potentials that are bounded at the origin provide an accurate description of the effective interaction for many systems of dissolved soft macromolecules (e.g., flexible dendrimers). Using numerical free-energy calculations, we…

Soft Condensed Matter · Physics 2014-10-29 C. Speranza , S. Prestipino , G. Malescio , P. V. Giaquinta

In the present work we investigate a gas-liquid transition in a two-component Gaussian core model, where particles of the same species repel and those of different species attract. Unlike a similar transition in a one-component system with…

Soft Condensed Matter · Physics 2018-02-14 Derek Frydel , Yan Levin

We numerically study crystal nucleation and glassy slow dynamics of the one-component Gaussian core model (GCM) at high densities. The nucleation rate at a fixed supersaturation is found to decrease as the density increases. At very high…

Soft Condensed Matter · Physics 2015-05-28 Atsushi Ikeda , Kunimasa Miyazaki

We redraw, using state-of-the-art methods for free-energy calculations, the phase diagrams of two reference models for the liquid state: the Gaussian and inverse-power-law repulsive potentials. Notwithstanding the different behavior of the…

Soft Condensed Matter · Physics 2011-10-26 S. Prestipino , F. Saija , P. V. Giaquinta

We present a simple density functional theory for the solid phases of systems of particles interacting via soft-core potentials. In particular, we apply the theory to particles interacting via repulsive point Yukawa and Gaussian pair…

Soft Condensed Matter · Physics 2007-05-23 A. J. Archer

We show that the Gaussian core model of particles interacting via a penetrable repulsive Gaussian potential, first considered by Stillinger (J. Chem. Phys. 65, 3968 (1976)), behaves like a weakly correlated ``mean field fluid'' over a…

Soft Condensed Matter · Physics 2009-10-31 A. A. Louis , P. G. Bolhuis , J. P. Hansen

The three-dimensional Gaussian core model (GCM) for soft-matter systems has repulsive interparticle interaction potential $\phi (r) = \varepsilon\, {\rm exp}\left[ -(r/\sigma)^{2} \right]$, with $r$ the distance between a pair of atoms, and…

Soft Condensed Matter · Physics 2021-01-18 George Ruppeiner , Peter Mausbach , Helge-Otmar May

A two-component system of penetrable particles interacting via a gaussian core potential is considered, which may serve as a crude model for binary polymer solutions. The pair structure and thermodynamic properties are calculated within the…

Soft Condensed Matter · Physics 2007-05-23 R. Finken , J. -P. Hansen , A. A. Louis

Isotropic pair potentials that are bounded at the origin have been proposed from time to time as models of the effective interaction between macromolecules of interest in the chemical physics of soft matter. We present a thorough study of…

Soft Condensed Matter · Physics 2014-03-05 S. Prestipino , C. Speranza , G. Malescio , P. V. Giaquinta

We numerically study dynamical properties of the one-component Gaussian Core Model in the supercooled states. We find that nucleation is suppressed as density increases. Concomitantly the system exhibits glassy slow dynamics characterized…

Soft Condensed Matter · Physics 2015-05-19 Atsushi Ikeda , Kunimasa Miyazaki

We study through integral equation theory and numerical simulations the structure and dynamics of fluids composed of ultrasoft, nearly Gaussian particles. Namely, we explore the fluid phase diagram of a model in which particles interact via…

Soft Condensed Matter · Physics 2013-03-14 Daniele Coslovich , Atsushi Ikeda

Hybrid particle-field molecular dynamics is a molecular simulation strategy wherein particles couple to a density field instead of through ordinary pair potentials. Traditionally considered a mean-field theory, a momentum and…

Computational Physics · Physics 2023-02-03 Morten Ledum , Samiran Sen , Sigbjørn Løland Bore , Michele Cascella

We report molecular dynamics simulation results for two-component fluid mixtures of Gaussian-core particles, focusing on how tracer diffusivities and static pair correlations depend on temperature, particle concentration, and composition.…

Soft Condensed Matter · Physics 2009-11-04 Mark J. Pond , William P. Krekelberg , Vincent K. Shen , Jeffrey R. Errington , Thomas M. Truskett

We study thermal equilibrium of classical pointlike counterions confined between symmetrically charged walls at distance $d$. At very large couplings when the counterion system is in its crystal phase, a harmonic expansion of particle…

Soft Condensed Matter · Physics 2019-01-21 L. Samaj , M. Trulsson , E. Trizac

We study the problem of learning Gaussian Mixture Models (GMMs) and ask: which structural properties govern their sample complexity? Prior work has largely tied this complexity to the minimum pairwise separation between components, but we…

Machine Learning · Computer Science 2025-08-06 Farzad Aryan
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