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Evidence for another phase transition at 120 K in the metallic pyrochlore oxide Cd2Re2O7, following the structural transition at 200 K and followed by the superconducting transition at 1.0 K, is given through resistivity, magnetoresistance,…

Strongly Correlated Electrons · Physics 2009-11-07 Zenji Hiroi , Jun-Ichi Yamaura , Yuji Muraoka , Masafumi Hanawa

We report magnetic, optical and oxidation states of oxygen deficient TiO$_{2-\delta}$ nanoparticles (NPs) synthesized by environment-friendly green route using Phyllanthus niruri (PN) whole plant extract instead of leaf extract. Rietveld…

We report high resolution single crystal x-ray diffraction measurements of the frustrated pyrochlore magnet Tb2Ti2O7, collected using a novel low temperature pulsed magnet system. This instrument allows characterization of structural…

Strongly Correlated Electrons · Physics 2012-07-16 J. P. C. Ruff , Z. Islam , J. P. Clancy , K. A. Ross , H. Nojiri , Y. H. Matsuda , H. A. Dabkowska , A. D. Dabkowski , B. D. Gaulin

Despite a well-ordered pyrochlore crystal structure and strong magnetic interactions between the Dy$^{3+}$ or Ho$^{3+}$ ions, no long range magnetic order has been detected in the pyrochlore titanates Ho$_2$Ti$_2$O$_7$ and…

A new series of cubic double perovskites Ba$_2R_{2/3}$TeO$_6$ ($R$ = Y, La, Pr, Nd, Sm-Lu) was synthesized via solid state reaction. The $R^{3+}$ and Te$^{6+}$ ions are ordered on alternating octahedral sites, with the rare earth sites 2/3…

Materials Science · Physics 2019-03-14 Tai Kong , Robert J. Cava

In recent years, solid state magnetic cooling based on magnetocaloric effect (MCE) have drawn attention worldwide as a promising alternative potential candidate to the conventional gas compression-expansion cooling technique. In this…

Materials Science · Physics 2024-10-23 Vinod Kumar Dwivedi

We have investigated the effect of synthesis and growth conditions on the magnetic, structural, and compositional properties of pyrochlore oxide holmium titanate and demonstrate a method for growing high quality stoichiometric single…

Materials Science · Physics 2018-09-26 Alireza Ghasemi , Allen Scheie , Jonas Kindervater , Seyed M. Koohpayeh

The crystal structure of Rb$_2$Ru$_2$O$_7$.H$_2$O was determined by three-dimensional electron diffraction from the individual crystallites of a solid-state powder product. Rb$_2$Ru$_2$O$_7$.H$_2$O crystallizes in space group…

Materials Science · Physics 2026-01-21 Krystof Chrappova , Jeremiah P. Tidey , Christopher Bell , Simon R. Hall

In connection with numerous X-ray and neutron investigations of some high temperature superconductors (YBa$_2$Cu$_3$O$_{6+x}$ and related compounds) a non-trivial part of the structure factor, coming from partly disordered Cu-O-$\dots$-O-Cu…

Condensed Matter · Physics 2009-10-22 Gennadi Uimin

Pb_1.83Mg_0.29Nb_1.71O_6.39 (PMN) crystallizing in a cubic pyrochlore structure exhibits, as the first dielectrics with pyrochlore structure, typical feature of quantum paraelectrics - its permittivity continuously increases on cooling and…

Materials Science · Physics 2007-09-25 S. Kamba , D. Nuzhnyy , S. Denisov , S. Veljko , V. Bovtun , M. Savinov , J. Petzelt , M. Kalnberga , A. Sternberg

In situ growth of pyrochlore iridate thin films has been a long-standing challenge due to the low reactivity of Ir at low temperatures and the vaporization of volatile gas species such as IrO3(g) and IrO2(g) at high temperatures and high…

Angle-resolved photoemission measurements have been performed on Bi2Ir2O7 single crystals, a prototypical example of the pyrochlore iridates. The density of states, the Fermi surface, and the near Fermi level band dispersion in the plane…

Strongly Correlated Electrons · Physics 2013-11-14 Q. Wang , Y. Cao , X. G. Wan , J. D. Denlinger , T. F. Qi , O. B. Korneta , G. Cao , D. S. Dessau

A "supercooled" liquid develops when a fluid does not crystallize upon cooling below its ordering temperature. Instead, the microscopic relaxation times diverge so rapidly that, upon further cooling, equilibration eventually becomes…

Polarized and unpolarized neutron diffraction has been used to search for magnetic order in YBa$_2$Cu$_3$O$_{6+x}$ superconductors. Most of the measurements were made on a high quality crystal of YBa$_2$Cu$_3$O$_{6.6}$. It is shown that…

Superconductivity · Physics 2009-11-07 H. A. Mook , Pengcheng Dai , S. M. Hayden , A. Hiess , J. W. Lynn , S. -H. Lee , F. Dogan

A new pyrochlore ruthenium oxide, Hg2Ru2O7 was synthesized under a high pressure of 6 GPa. In contrast to the extensively studied Ru4+ oxides, this compound possesses a novel Ru5+ valence state, corresponding to a half-filled t_2g_3…

Breathing pyrochlores are a unique class of materials characterized by a three-dimensional lattice of corner-sharing tetrahedra. However, unlike conventional pyrochlores where all tetrahedra are identical in size, the breathing pyrochlore…

The chemical composition, crystal structure, and magnetic properties of a manganese zinc alloy with an ideal composition of YMn2Zn20, which comprises a pyrochlore lattice made of Mn atoms, are reported. The compound is stable only when In…

Materials Science · Physics 2015-06-04 Yoshihiko Okamoto , Takeshi Shimizu , Jun-ichi Yamaura , Zenji Hiroi

Dy$_{2}$Zr$_{2}$O$_{7}$ a disordered pyrochlore system, exhibits the spin ice freezing under the application of magnetic field. Our studies suggest the stabilization of pyrochlore phase in Dy$_{2-x}$La$_{x}$Zr$_{2}$O$_{7}$ with the…

Strongly Correlated Electrons · Physics 2021-10-12 Sheetal , C. S. Yadav

Bulk superconductor samples of YBa2Cu3-xCoxO7-{\delta} with x = 0, 0.01, 0.03, 0.05 are synthesized by solid-state reaction route. Both x-ray diffraction and electron microscopy have been employed to study the phase identification,…

Superconductivity · Physics 2011-07-07 Sushant Gupta , R. S. Yadav , N. P. Lalla , G. D. Verma , B. Das

The question of structural disorder and its effects on magnetism is relevant to a number of spin liquid candidate materials. Although commonly thought of as a route to spin glass behavior, here we describe a system in which the structural…

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