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We study the dynamics of initial nucleation processes of photoinduced structural change of molecular crystals. In order to describe the nonadiabatic transition in each molecule, we employ a model of localized electrons coupled with a fully…

Materials Science · Physics 2009-11-13 Kunio Ishida , Keiichiro Nasu

Nonlinear dynamics of photoinduced cooperative phenomena is studied by numerical calculations on a model of molecular crystals. We found that the photoinduced nucleation process is triggered only when certain amount of excitation energy is…

Computational Physics · Physics 2009-11-13 Kunio Ishida , Keiichiro Nasu

Transient quantum dynamics in an interacting fermion-phonon system are investigated. In particular, a charge order (CO) melting after a short optical-pulse irradiation and roles of the quantum phonons on the transient dynamics are focused…

Strongly Correlated Electrons · Physics 2017-09-13 Hiroshi Hashimoto , Sumio Ishihara

In this work we postulate that Schwinger's threshold for a dynamic electric field intensity to induce spatial nonlinearity is a special case and, more generally, it is the threshold field for both static and dynamic electric fields. Fields…

Quantum Physics · Physics 2020-09-17 Dale M. Grimes , Craig A. Grimes

Ultrafast photoinduced dynamics of electronic excitation in molecular dimers is drastically affected by the dynamic reorganization of inter- and intra- molecular nuclear configuration modeled by a quantized nuclear degree of freedom [Cina…

Mathematical Physics · Physics 2009-11-10 Dmitri S. Kilin , Yuri V. Pereversev , Oleg V. Prezhdo

Phase transitions induced by short optical pulses is a new mainstream in studies of cooperative electronic states. Its special realization in systems with neutral-ionic transformations stands out in a way that the optical pumping goes to…

Strongly Correlated Electrons · Physics 2015-01-27 Tianyou Yi , Natasha Kirova , Serguei Brazovskii

Controlling electrically-stimulated quantum light sources (QLS) is key for developing integrated and low-scale quantum devices. The mechanisms leading to quantum emission are complex, as a large number of electronic states of the system…

Mesoscale and Nanoscale Physics · Physics 2024-02-28 Katharina Kaiser , Anna Rosławska , Michelangelo Romeo , Fabrice Scheurer , Tomáš Neuman , Guillaume Schull

A single quantum dot deterministically coupled to a photonic crystal environment constitutes an indispensable elementary unit to both generate and manipulate single-photons in next-generation quantum photonic circuits. To date, the scaling…

Photons are the elementary quantum excitations of the electromagnetic field. Quantization is usually constructed on the basis of an expansion in eigenmodes, in the form of plane waves. Since they form a basis, other electromagnetic…

Quantum Physics · Physics 2022-12-07 M. Federico , V. Dorier , S. Guérin , H. R. Jauslin

The rates of protein folding with photon absorption or emission and the cross section of photon -protein inelastic scattering are calculated from the quantum folding theory by use of standard field-theoretical method. All these protein…

Biomolecules · Quantitative Biology 2011-05-13 Liaofu Luo

The processes of generation of phonons and electron excitations with quantum oriented particle in crystal are considered. Expressions are obtained for the probability of emission of phonons and plasmons with channeled particle. The theory…

Other Condensed Matter · Physics 2015-12-09 Evgeny Mazur

We develop a trajectory-based approach for excited-state molecular dynamics simulations of systems subject to an external periodic drive. We combine the exact-factorization formalism, allowing to treat electron-nuclear systems in…

Chemical Physics · Physics 2021-03-31 Marco Schirò , Florian G. Eich , Federica Agostini

There has been rapid development of systems that yield strong interactions between freely propagating photons in one dimension via controlled coupling to quantum emitters. This raises interesting possibilities such as quantum information…

The decay of photoexcited quantum systems (examples are photodissociation of molecules and autoionization of atoms) can be viewed as a half-collision process (an incoming photon excites the system which subsequently decays by dissociation…

Disordered Systems and Neural Networks · Physics 2009-11-10 T. Gorin , B. Mehlig , W. Ihra

In recent years, Born-Markov master equations based on tracing out the electromagnetic degrees of freedom have been extensively employed in the description of quantum optical phenomena originating from photon-mediated interactions in…

The generation of quantum entanglement between phonons in photoirradiated remote electron-phonon systems is numerically studied. Upon excitation by a visible/ultraviolet laser pulse, the entanglement of electrons is immediately generated…

Mesoscale and Nanoscale Physics · Physics 2021-10-13 Kunio Ishida , Hiroaki Matsueda

With advanced micro- and nano-photonic structures, the vacuum photon-photon coupling rate is anticipated to approach the intrinsic loss rate and lead to unconventional quantum effects. Here, we investigate the classical-to-quantum…

Quantum Physics · Physics 2022-04-11 Yue-Xun Huang , Ming Li , Ke Lin , Yan-Lei Zhang , Guang-Can Guo , Chang-Ling Zou

Electronic coherences are key to understanding and controlling photo-induced molecular transformations. We identify a crucial quantum-mechanical feature of electron-nuclear correlation, the projected nuclear quantum momenta, essential to…

Chemical Physics · Physics 2024-11-13 Evaristo Villaseco Arribas , Neepa T. Maitra

We study the influence of the phonon environment on the electron dynamics in a doped quantum dot molecule. A non-perturbative quantum kinetic theory based on correlation expansion is used in order to describe both diagonal and off-diagonal…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 A. Grodecka-Grad , J. Förstner

We study the dynamics of photonic quantum circuits consisting of nodes coupled by quantum channels. We are interested in the regime where time delay in communication between the nodes is significant. This includes the problem of quantum…

Quantum Physics · Physics 2016-03-07 Hannes Pichler , Peter Zoller
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