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Neutron powder diffraction and single crystal x-ray resonant magnetic scattering measurements suggest that Dy plays an active role in enhancing the ferroelectric polarization in multiferroic DyMnO3 above TNDy = 6.5 K. We observe the…

Strongly Correlated Electrons · Physics 2007-05-23 O. Prokhnenko , R. Feyerherm , E. Dudzik , S. Landsgesell , N. Aliouane , L. C. Chapon , D. N. Argyriou

Novel imaging spin-filter techniques, which are based on low energy electron diffraction, are currently of high scientific interest. To improve the spin-detection efficiency a variety of new materials have been introduced in recent years. A…

Computational Physics · Physics 2015-11-18 Stephan Borek , Jürgen Braun , Hubert Ebert , Ján Minár

We study the polarization induced via spin-orbit interaction by a magnetic cycloidal order in orthorhombic TbMnO3 using first-principle methods. The case of magnetic spiral lying in the b-c plane is analyzed, in which the pure electronic…

Materials Science · Physics 2009-12-16 Andrei Malashevich , David Vanderbilt

Magnetic ferroelectrics or multiferroics, which are currently extensively explored, may provide a good arena to realize a novel magnetoelectric function. Here we demonstrate the genuine electric control of the spiral magnetic structure in…

Strongly Correlated Electrons · Physics 2009-11-13 Y. Yamasaki , H. Sagayama , T. Goto , M. Matsuura , K. Hirota , T. Arima , Y. Tokura

By performing first-principles calculations, we systematically explore the effect of epitaxial strain on the structure and properties of multiferroic TbMnO3. We show that, although the unstrained bulk TbMnO3 displays a non-collinear…

Materials Science · Physics 2015-05-20 Yusheng Hou , Jihui Yang , Xingao Gong , Hongjung Xiang

We uncover a new pathway towards multiferroicity, showing how magnetism can drive ferroelectricity without relying on inversion symmetry breaking of the magnetic ordering. Our free-energy analysis demonstrates that any commensurate…

Materials Science · Physics 2009-11-11 Joseph J. Betouras , Gianluca Giovannetti , Jeroen van den Brink

By performing accurate ab-initio density functional theory calculations, we study the role of $4f$ electrons in stabilizing the magnetic-field-induced ferroelectric state of DyFeO$_{3}$. We confirm that the ferroelectric polarization is…

Materials Science · Physics 2015-05-14 Alessandro Stroppa , Martijn Marsman , Georg Kresse , Silvia Picozzi

We investigate the crystal structure in multiferroic tetragonal perovskite Sr$_{1/2}$Ba$_{1/2}$MnO$_3$ with high accuracy of the order of 10$^{-3}$ Angstrom for an atomic displacement. The large atomic displacement for Mn ion from the…

Materials Science · Physics 2020-07-15 D. Okuyama , K. Yamauchi , H. Sakai , Y. Taguchi , Y. Tokura , K. Sugimoto , T. J. Sato , T. Oguchi

We report on diffraction measurements on multiferroic TbMnO3 which demonstrate that the Tb- and Mn-magnetic orders are coupled below the ferroelectric transition TFE = 28 K. For T < TFE the magnetic propagation vectors (tau) for Tb and Mn…

Strongly Correlated Electrons · Physics 2009-11-13 O. Prokhnenko , R. Feyerherm , M. Mostovoy , N. Aliouane , E. Dudzik , A. U. B. Wolter , A. Maljuk , D. N. Argyriou

We provide compelling evidence to establish that, contrary to one's elementary guess, the tunneling spin polarization (TSP) of amorphous CoFeB is larger than that of highly textured fcc CoFeB. First principles atomic and electronic…

Local structural measurements have been performed on hexagonal HoMnO3 in order to ascertain the specific changes in bond distances which accompany magnetic ordering transitions. The transition from paramagnetic to the antiferromagetic…

Strongly Correlated Electrons · Physics 2015-05-14 T. A. Tyson , T. Wu , K. H. Ahn , S. Kim , S. -W. Cheong

We present a detailed study of the structural, electronic, magnetic and ferroelectric properties of prototypical \textit{proper} and \textit{improper} multiferroic (MF) systems such as BiFeO$_{3}$ and orthorhombic HoMnO$_{3}$, respectively,…

Materials Science · Physics 2017-03-15 A. Stroppa , S. Picozzi

Aiming at increasing the ferroelectric polarization in AFM-E ortho-\hmo, we investigate the in-plane strain effects on both the magnetic configuration and the polarization by means of density functional theory calculations and model…

CuFeO_2 is one of the multiferroic materials and is the first case that the electric polarization is not explained by the magnetostriction model or the spin-current model. We have studied this material using soft x-ray resonant diffraction…

In order to clarify the mechanism associated with pressure/magnetic-field-induced giant ferroelectric polarization in TbMnO3, this work investigated changes in magnetic ordering brought about by variations in temperature, magnetic field,…

Strongly Correlated Electrons · Physics 2019-03-05 Noriki Terada , Dmitry D. Khalyavin , Pascal Manuel , Toyotaka Osakabe , Akiko Kikkawa , Hideaki Kitazawa

Using first principle calculations under the framework of density functional theory we have investigated the electronic structure, magnetism and ferroelectric polarization in the triangular lattice antiferromagnet AgFeO2, and its comparison…

Materials Science · Physics 2018-01-03 Jayita Chakraborty , Indra Dasgupta

$Ab$ $initio$ calculations show the presence of a strong magnetoelectric interfacial coupling in CaMnO$_3$ ultra-thin film grown on a strained BaTiO$_3$ ferroelectric film. This heterostructure presents a polarization driven magnetic…

Materials Science · Physics 2025-04-23 S. Di Napoli , A. Román , A. M. Llois , M. H. Aguirre , L. B. Steren , M. A. Barral

Magnetically-driven ferroelectric atomic displacements of the order of 10$^{-3} Angstrom have been observed in orthorhombic (perovskite like) YMnO$_3$ by a single-crystal synchrotron x-ray diffraction. The refined polar structure shows the…

Strongly Correlated Electrons · Physics 2011-08-12 D. Okuyama , S. Ishiwata , Y. Takahashi , K. Yamauchi , S. Picozzi , K. Sugimoto , H. Sakai , M. Takata , R. Shimano , Y. Taguchi , T. Arima , Y. Tokura

Spin-polarized currents play a key role in spintronics. Recently, it has been found that antiferromagnets with a non-spin-degenerate band structure can efficiently spin-polarize electric currents, even though their net magnetization is…

Materials Science · Physics 2021-12-20 Gautam Gurung , Ding-Fu Shao , Evgeny Y. Tsymbal

Electric-field control of spin-dependent properties has become one of the most attractive phenomena in modern materials research due the promise of new device functionalities. One of the paradigms in this approach is to electrically toggle…

Materials Science · Physics 2015-06-19 Xiaohui Liu , J. D. Burton , Evgeny Y. Tsymbal