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The electronic property and magnetic susceptibility of Ce$_3$Pd$_3$Bi$_4$ were systemically investigated from 18 K to 290 K for varying values of cell-volume using dynamic mean-field theory coupled with density functional theory. By…

Strongly Correlated Electrons · Physics 2022-02-08 Chenchao Xu , Chao Cao , Jian-Xin Zhu

For diatomic molecules and chains bound anharmonically by interactions such a the Lennard Jones and Morse potentials, we obtain analytical expressions for thermodynamic observables including the mean bond length, thermally averaged internal…

Statistical Mechanics · Physics 2016-05-20 D. J. Priour , Christopher Watenpool

Combining classical electrodynamics and density functional theory (DFT) calculations, we develop a general and rigorous theoretical framework that describes the energetics of metal surfaces under high electric fields. We show that the…

Materials Science · Physics 2019-05-22 Andreas Kyritsakis , Ekaterina Baibuz , Ville Jansson , Flyura Djurabekova

We investigate the pressure-temperature ($p$-$T$) phase diagram of elemental lithium (Li) up to multiterapascal (TPa) pressures using ab-initio random structure search (AIRSS) and density functional theory (DFT). At zero temperature, beyond…

Materials Science · Physics 2024-03-21 Jack Whaley-Baldwin , Miguel Martinez-Canales , Chris J. Pickard

Correlated systems at both zero and nonzero temperature are treated here from a novel angle using a functional method. This functional method is an extension of the usual effective potential method. Here, however the effective action is…

Condensed Matter · Physics 2007-05-23 A. Rebei , W. N. G. Hitchon

By using the arc-melting method, we successfully synthesized the compound Sc$_{0.5}$Zr$_{0.5}$Co with the space group of $Pm$-$3m$. Both the resistivity and magnetic susceptibility measurements reveal a phase transition at about 86 K. This…

Materials Science · Physics 2020-07-06 Jin Si , Xinwei Fan , Enyu Wang , Xiyu Zhu , Qing Li , Hai-Hu Wen

We present a computational scheme for total energy calculations of disordered alloys with strong electronic correlations. It employs the coherent potential approximation combined with the dynamical mean-field theory and allows one to study…

Strongly Correlated Electrons · Physics 2015-10-02 A. S. Belozerov , A. I. Poteryaev , S. L. Skornyakov , V. I. Anisimov

The accurate prediction of solid-solid structural phase transitions at finite temperature is a challenging task, since the dynamics is so slow that direct simulations of the phase transitions by first-principles (FP) methods are typically…

Materials Science · Physics 2021-05-25 Peitao Liu , Carla Verdi , Ferenc Karsai , Georg Kresse

Effective pair interactions with a soft-repulsive component are a well-known feature of polymer solutions and colloidal suspensions, but they also provide a key to interpret the high-pressure behaviour of simple elements. We have computed…

Soft Condensed Matter · Physics 2009-09-08 Santi Prestipino , Franz Saija , Gianpietro Malescio

Inspired by the synthesis of XB3C3 (X= Sr, La) compounds in the bipartite sodalite clathrate structure, density functional theory (DFT) calculations are performed on members of this family containing up to two different metal atoms. A…

Superconductivity · Physics 2023-01-27 Nisha Geng , Katerina P. Hilleke , Li Zhu , Xiaoyu Wang , Timothy A. Strobel , Eva Zurek

The combination of density functional theory and single-site dynamical mean-field theory, using both Hartree and full continuous-time quantum Monte Carlo impurity solvers, is used to study the metal-insulator phase diagram of perovskite…

Strongly Correlated Electrons · Physics 2014-09-25 Hung T. Dang , Xinyuan Ai , Andrew J. Millis , Chris A. Marianetti

Ensemble Density Functional Theory (EDFT) is a generalization of ground-state Density Functional Theory (GS DFT), which is based on an exact formal theory of finite collections of a system's ground and excited states. EDFT in various forms…

Materials Science · Physics 2024-08-27 Remi J. Leano , Aurora Pribram-Jones , David A. Strubbe

Density Functional Theory (DFT) is one of the most widely used methods for "ab initio" calculations of the structure of atoms, molecules, crystals, surfaces, and their interactions. Unfortunately, the customary introduction to DFT is often…

Physics Education · Physics 2010-12-07 Nathan Argaman , Guy Makov

We propose a new method for accurately calculating electrical transport properties of a lightly-doped thermoelectric material from density functional theory (DFT) calculations, based on experimental data and density functional theory…

Materials Science · Physics 2014-01-14 Alireza Faghaninia , Cynthia S. Lo

The transition temperature between the low-temperature alpha phase of tin to beta tin is close to the room temperature (Tab =13C), and the difference in cohesive energy of the two phases at 0 K of about dEcoh=0.02 eV/atom is at the limit of…

Materials Science · Physics 2016-05-03 Fleur Legrain , Sergei Manzhos

The potential of zero free charge (PZFC) value is a crucial parameter in electrochemistry. However, the evaluations of PZFC have traditionally been difficult. To overcome this challenge, we applied a hybrid solvation method that…

Materials Science · Physics 2023-09-06 Jack Jon Hinsch , Jessica Jein White , Yun Wang

A brief introduction to conventional DFT of 3D freezing is given and some recent results are reviewed. The conventional DFT, however, can not be used in the 2D case, particularly, because it can not describe the hexatic phase --…

Statistical Mechanics · Physics 2007-05-23 Elena Tareyeva , Valentin Ryzhov

Combining density functional theory (DFT) and embedded dynamical mean-field theory (DMFT) methods, we study the metal-insulator transition in $R_2$Ir$_2$O$_7$ ($R$=Y, Eu, Sm, Nd, Pr, and Bi) and the topological nature of the insulating…

Strongly Correlated Electrons · Physics 2017-01-18 Hongbin Zhang , Kristjan Haule , David Vanderbilt

Phase field crystal (PFC) theory, extensively used for modelling the structure of solids, can be derived from dynamical density functional theory (DDFT) via a sequence of approximations. Standard derivations neglect a term of form…

Soft Condensed Matter · Physics 2019-09-04 Andrew J. Archer , Daniel J. Ratliff , Alastair M. Rucklidge , Priya Subramanian

Thermodynamic conventions suffer from describing dynamical distinctions, especially when the structural and energetic changes induced by localized rare events are insignificant. By using the ensemble theory in the trajectory space, we…

Statistical Mechanics · Physics 2023-03-30 Qi-Jun Ye , Xin-Zheng Li