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We report the enhancement of the optical second harmonic signal in non-centrosymmetric semiconductor CdS quantum dots, when they are placed in close contact with isolated silver nanoparticles. The intensity enhancement is about 1000. We…

Mesoscale and Nanoscale Physics · Physics 2012-02-15 Pablo M. Jais , Catalina von Bilderling , Andrea V. Bragas

Second-harmonic generation (SHG) is a fundamental nonlinear optical process widely used in photonics; however, it is strictly forbidden in the bulk of centrosymmetric materials due to their inversion symmetry. Nevertheless, applying an…

The motive of this work is to understand the complex spatial characteristics of finite-amplitude elastic wave propagation in periodic structures and leverage the unique opportunities offered by nonlinearity to activate complementary…

Pattern Formation and Solitons · Physics 2017-06-27 R. Ganesh , Stefano Gonella

The terahertz transmission properties of symmetrical and asymmetrical annular apertures arrays (AAAs) are investigated both experimentally and numerically. It is found that only odd order resonant modes are observed for the symmetrical…

Optics · Physics 2012-07-17 Dan Hu , Changqing Xie , Ming Liu , Yan Zhang

In this paper, we proposed and numerically demonstrated a giant enhancement up to 108 in both forward and backward propagation of the Second Harmonic Generation by combining the high-quality factor cavities of the Bound States in the…

Optics · Physics 2022-06-24 Juan José Robayo Yepes , Fadi Issam Baida , Abdoulaye Ndao

We illustrate that a Hermitian nonlinear optical system consisting of hybridized parametric amplification and second harmonic generation mimics non-Hermitian evolution dynamics. Oscillation damping, evolution to a static steady state, and…

Optics · Physics 2021-01-05 Noah Flemens , Nicolas Swenson , Jeffrey Moses

We describe an approach based on topology optimization that enables automatic discovery of wavelength-scale photonic structures for achieving high-efficiency second-harmonic generation (SHG). A key distinction from previous formulation and…

Second-order nonlinear optical response allows to detect different properties of the system associated with the inversion symmetry breaking. Here, we use a second harmonic generation effect to investigate the alignment of a…

Mesoscale and Nanoscale Physics · Physics 2020-07-03 E. A. Stepanov , S. V. Semin , C. R. Woods , M. Vandelli , A. V. Kimel , K. S. Novoselov , M. I. Katsnelson

High-harmonic generation is a light up-conversion process occurring in a strong laser field, leading to coherent bursts of extreme ultrashort broadband radiation [1]. As a new perspective, we propose that ultrafast strong-field electronic…

The discovery of second harmonic generation in 1961 marked the birth of nonlinear optics, unlocking a range of applications from frequency conversion to quantum light generation. Yet, phase matching in bulk nonlinear crystals remains a key…

The study of high-harmonic generation in confined quantum systems is vital to establishing a complete physical picture of harmonic generation from atoms and molecules to bulk solids. Based on a multilevel approach, we demonstrate how…

Mesoscale and Nanoscale Physics · Physics 2023-03-28 Xiao Zhang , Tao Zhu , Hongchuan Du , Hong-Gang Luo , Jeroen van den Brink , Rajyavardhan Ray

We report comparative experimental and theoretical studies of second and third harmonic generation from a 20nm-thick indium tin oxide layer in proximity of the epsilon-near-zero condition. Using a tunable OPA laser we record both spectral…

Theoretical investigation is conducted of high-order harmonic generation (HHG) in silicon thin films to elucidate the effect of light propagation in reflected and transmitted waves. The first-principles simulations are performed of the…

Materials Science · Physics 2023-01-23 Shunsuke Yamada , Tomohito Otobe , David Freeman , Anatoli Kheifets , Kazuhiro Yabana

We present experimental results on the observation of a bulk second-order nonlinear susceptibility derived from both free-space and integrated measurements in silicon nitride. Phase-matching is achieved through dispersion engineering of the…

Harmonic generation mechanisms are of great interest in nanoscience and nanotechnology, since they allow generating visible light by using near-infrared radiation, which is particularly suitable for its endless applications in…

Recent years have witnessed significant developments in the study of nonlinear properties of various optical materials at the nanoscale. However, in most cases experimental results on harmonic generation from nanostructured materials are…

Plasmonic gratings constitute a paradigmatic instance of the wide range of applications enabled by plasmonics. While subwavelength metal gratings find applications in optical biosensing and photovoltaics, atomically thin gratings achieved…

Optics · Physics 2018-10-25 P. A. Huidobro , Y. H. Chang , M. Kraft , J. B. Pendry

The existence of resonant enhanced transmission and collimation of light waves by subwavelength slits in metal films [for example, see T.W. Ebbesen et al., Nature (London) 391, 667 (1998) and H.J. Lezec et al., Science, 297, 820 (2002)]…

Optics · Physics 2013-05-29 S. V. Kukhlevsky , M. Mechler , L. Csapo , K. Janssens , O. Samek

Comparative analysis of second harmonic generation in ordinary and backward-wave settings is presented. Extraordinary properties of frequency doubling nonlinear optical reflectivity and pulse shaping through phase matching of ordinary and…

Optics · Physics 2016-02-02 Alexander K. Popov , Sergey A. Myslivets

We demonstrate a simple and scalable approach to increase conversion efficiencies of nonlinear metasurfaces by incorporating them into multipass cells and by letting the pump beam to interact with the metasurfaces multiple times. We…