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We report a neutron diffraction study of the multiferroic mechanism in (ND4)2FeCl5D2O, a molecular compound that exhibits magnetically induced ferroelectricity. This material exhibits two successive magnetic transitions on cooling: a…

Within the BaFe2As2 crystal lattice, we partially substitute thallium for barium and report the effects of interlayer coupling in Ba1-xTlxFe2As2 crystals. We demonstrate the unusual effects of magneto-elastic coupling and charge doping in…

Superconductivity · Physics 2016-11-11 A. S. Sefat , L. Li , H. B. Cao , M. A. McGuire , B. Sales , R. Custelcean , D. S. Parker

An intriguingly complex phase diagram of Na-doped SrFe2As2 is uncovered using high-resolution thermal-expansion, magnetization and heat-capacity measurements. The detailed temperature dependence of the orthorhombic distortion and the…

Superconductivity · Physics 2019-10-01 L. Wang , M. He , D. D. Scherer , F. Hardy , P. Schweiss , T. Wolf , M. Merz , B. M. Andersen , C. Meingast

The magnetic and dielectric properties under high magnetic fields are studied in the single crystal of Cu3Mo2O9. This multiferroic compound has distorted tetrahedral spin chains. The effects of the quasi-one dimensionality and the…

Strongly Correlated Electrons · Physics 2013-11-13 H. Kuroe , K. Aoki , R. Kino , T. Sato , H. Kuwahara , T. Sekine , T Kihara , M. Akaki , Y. Kohama , M. Tokunaga , A. Matsuo , K. Kindo , M. Hase , K. Takehana , H. Kitazawa , K. Oka , T. Ito , H. Eisaki

Raman scattering studies of the frustrated spin chain system LiCu$_{2}$O$_{2}$ are reported. Two transitions into a magnetically ordered phase (taken place at temperatures $\sim$ 9 K and $\sim$ 24 K) have been confirmed from the analysis of…

Strongly Correlated Electrons · Physics 2009-11-10 K. -Y. Choi , S. A. Zvyagin , G. Cao , P. Lemmens

The magnetic susceptibility between 1.5 and 800 K, the infrared reflectivity at room temperature and the temperature dependence of the dielectric constant at mm-wavelengths are reported for single crystalline BiFeO3. A well developed…

Strongly Correlated Electrons · Physics 2010-07-22 Jun Lu , M Schmidt , P Lunkenheimer , A Pimenov , A A Mukhin , V D Travkin , A Loidl

We investigated the magnetic phase diagram of single crystals of SrNdFeO$_{4}$ by measuring the magnetic properties, the specific heat and the dielectric permittivity. The system has two magnetically active ions, Fe$^{3+}$ and Nd$^{3+}$.…

Materials Science · Physics 2015-06-05 J. M. Hwang , E. S. Choi , H. D. Zhou , Y. Xin , J. Lu , P. Schlottmann

In the present study, we investigated magnetodielectric, magnetoelectric (ME), and angular-dependent polarization in single-crystal Fe4Nb2O9. The magnetodielectric effects in epsilon(x) (x//[100]), epsilon(y) (y//[120]), and epsilon(z)…

Materials Science · Physics 2021-09-29 Jing Zhang , Na Su , Xinrun Mi , Maocai Pi , Haidong Zhou , Jinguang Cheng , Yisheng Chai

Spinel compounds AB$_{2}$X$_{4}$ consist of both tetrahedral (AX$_{4}$) and octahedral (BX$_{6}$) environments with the former forming a diamond lattice and the latter a geometrically frustrated pyrochlore lattice. Exploring the fascinating…

Chemical Physics · Physics 2023-03-29 Qiang Zhang , Wei Tian , Roshan K. Nepal , Ashfia Huq , Stephen Nagler , J. F. DiTusa , Rongying Jin

This work reports an experimental investigation of the magneto-elastic coupling and polarization character of magnetic phases of the orthorhombic Eu1-xYxMnO3 system at low temperatures. The temperature dependence of the polarization…

We have found a remarkable increase (up to 60 %) of the dielectric constant with the onset of magnetic order at 42 K in the metastable orthorhombic structures of YMnO3 and HoMnO3 that proves the existence of a strong magneto-dielectric…

Strongly Correlated Electrons · Physics 2009-11-10 B. Lorenz , Y. Q. Wang , Y. Y. Sun , C. W. Chu

Rare-earth-based permanent-magnet materials rich in iron have relatively low ferromagnetic ordering temperatures. This is believed to be due to the presence of antiferromagnetic exchange interactions, besides the ferromagnetic interactions…

Materials Science · Physics 2009-11-11 Y. Janssen , S. Chang , A. Kreyssig , A. Kracher , Y. Mozharivskyj , S. Misra , P. C. Canfield

We report temperature dependent magnetization and neutron diffraction measurements on the corundum related magnetoelectric antiferromagnet Mn$_{4}$Ta$_{2}$O$_{9}$. Measurements performed on a single crystalline specimen reveal that the…

Strongly Correlated Electrons · Physics 2021-01-20 Soumendra Nath Panja , Pascal Manuel , Sunil Nair

Structural, magnetic and magnetocaloric properties of Mn2-xCrxSb compounds have been studied. In these compounds a first order magnetic phase transition from the ferrimagnetic to the antiferromagnetic state occurs with decreasing…

Materials Science · Physics 2014-10-01 L. Caron , X. F. Miao , J. C. P Klaasse , S. Gama , E. Brück

The compounds, PrCo9Si4 and NdCo9Si4, have been recently reported to exhibit first-order ferromagnetic transitions near 24 K. We have subjected this compound for further characterization by magnetization, heat-capacity and electrical…

Materials Science · Physics 2009-11-13 Niharika Mohapatra , E. V. Sampathkumaran

The magnetic structures and the magnetic phase transitions in the Mn-doped orthoferrite TbFeO$_3$ studied using neutron powder diffraction are reported. Magnetic phase transitions are identified at $T^\mathrm{Fe/Mn}_N \approx$ 295~K where a…

Strongly Correlated Electrons · Physics 2016-02-17 Harikrishnan S. Nair , Tapan Chatterji , C. M. N. Kumar , T. Hansen , Hariharan Nhalil , Suja Elizabeth , A. M. Strydom

In multiferroic BiFeO$_3$ a cycloidal antiferromagnetic structure is coupled to a large electric polarization at room temperature, giving rise to magnetoelectric functionality that may be exploited in novel multiferroic-based devices. In…

Strongly Correlated Electrons · Physics 2017-03-08 R. D. Johnson , P. A. McClarty , D. D. Khalyavin , P. Manuel , P. Svedlindh , C. S. Knee

Structural, impedance, ferroelectric and magnetic properties were examined in multiferroic Bi_{2}Fe_{4(1-x)}Co_{4x}O_{9} (0$\leq$x$\leq$0.02) ceramics synthesized via solid-state reaction method. X-ray diffraction analysis and Rietveld…

Materials Science · Physics 2016-05-06 S. R. Mohapatra , B. Sahu , M. Chandrasekhar , P. Kumar , S. D. Kaushik , S. Rath , A. K. Singh

Altermagnetism is a novel magnetic phase combining characteristics of both antiferromagnetism and ferromagnetic ordering. Despite growing theoretical interest in altermagnetic materials, reports of experimentally verified high Neel…

We have measured the dielectric constant and the pyroelectric current of orthorhombic (space group $Pbam$) NdCrTiO$_5$ polycrystalline samples. The dielectric constant and the pyroelectric current show features associated with ferroelectric…

Materials Science · Physics 2015-05-30 J. Hwang , E. S. Choi , H. D. Zhou , J. Lu , P. Schlottmann