English
Related papers

Related papers: Resonant electron heating and molecular phonon coo…

200 papers

We study hot-electron cooling by acoustic and optical phonons in monolayer MoS$_2$. The cooling power $P$ ($P_e = P/n$) is investigated as a function of electron temperature $T_e$ (0-500 $\mathrm{K}$) and carrier density $n$…

Mesoscale and Nanoscale Physics · Physics 2014-11-04 Kristen Kaasbjerg , K. S. Bhargavi , S. S. Kubakaddi

Our objective is to study resonant tunneling of an electron in the presence of inelastic scattering by optical phonons. Using a recently developed technique, based on exact mapping of a many-body problem onto a one-body problem, we compute…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 K. Haule , J. Bonca

We propose and analyze a new way of using $\pi$ stacking to design molecular junctions that either enhance or suppress a phononic heat current, but at the same time remain conductors for an electric current. Such functionality is highly…

Mesoscale and Nanoscale Physics · Physics 2015-02-10 Gediminas Kiršanskas , Qian Li , Karsten Flensberg , Gemma C. Solomon , Martin Leijnse

A framework for estimating heating and expected temperature rise in current carrying molecular junctions is described. Our approach is based on applying the Redfield approximation to a tight binding model for the molecular bridge…

Condensed Matter · Physics 2009-11-07 Dvira Segal , Abraham Nitzan

Measurements of the thermal conductance of single-molecule junctions have recently been reported for the first time. It is presently unclear, how much the heat transport can be controlled through molecule-internal effects. The search for…

Mesoscale and Nanoscale Physics · Physics 2025-10-01 Matthias Blaschke , Fabian Pauly

We study the dependence of the heat transfer between two semi-infinite solids on the dielectric properties of the bodies. We show that the heat transfer at short separation between the solids may increase by many order of magnitude when the…

Materials Science · Physics 2009-11-11 A. I. Volokitin , B. N. J. Persson

We present {\it ab initio} density-functional calculations of molecular solids formed from C$_{28}$-derived closed-shell fullerenes. Solid C$_{28}$H$_4$ is found to bind weakly and exhibits many of the electronic structure features of solid…

Superconductivity · Physics 2009-11-10 Nichols A. Romero , Jeongnim Kim , Richard M. Martin

Due to their structured density of states, molecular junctions provide rich resources to filter and control the flow of electrons and phonons. Here we compute the out of equilibrium current-voltage characteristics and dissipated heat of…

Mesoscale and Nanoscale Physics · Physics 2023-11-01 Fatemeh Tabatabaei , Samy Merabia , Bernd Gotsmann , Mika Prunnila , Thomas A. Niehaus

Measuring thermodynamic quantities can be easy or not, depending on the system that is being studied. For a macroscopic object, measuring temperatures can be as simple as measuring how much a column of mercury rises when in contact with the…

Quantum Physics · Physics 2015-09-15 O. P. de Sá Neto , M. C. de Oliveira , G. J. Milburn

The plasmonic tip of a scanning tunnelling microscope (STM) is functionalized with a single fluorescent molecule and is scanned on a plasmonic substrate. The tunneling current flowing through the tip-molecule-substrate junction generates a…

The electron transport through a three-terminal single-molecular transistor (SMT) is theoretically studied. We find that the differential conductance of the third and weakly coupled terminal versus its voltage matches well with the spectral…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Juntao Song , Qing-feng Sun , Jinhua Gao , X. C. Xie

Electronic cooling in hybrid normal metal-insulator-superconductor junctions is a promising technology for the manipulation of thermal loads in solid state nanosystems. One of the main bottlenecks for efficient electronic cooling is the…

We study the electrical conductance $G$ and the thermopower $S$ of single-molecule junctions, and reveal signatures of different transport mechanisms: off-resonant tunneling, on-resonant coherent (ballistic) motion, and multi-step hopping.…

Mesoscale and Nanoscale Physics · Physics 2017-04-12 Roman Korol , Michael Kilgour , Dvira Segal

We present a detailed study of the non-linear thermoelectric properties of a molecular junction, represented by a dissipative Anderson-Holstein model. A single orbital level with strong Coulomb interaction is coupled to a localized…

Mesoscale and Nanoscale Physics · Physics 2013-01-10 M. Leijnse , M. R. Wegewijs , K. Flensberg

We show that the vibrations of a nanomechanical resonator can be cooled to near its quantum ground state by tunnelling injection of electrons from an STM tip. The interplay between two mechanisms for coupling the electronic and mechanical…

Mesoscale and Nanoscale Physics · Physics 2011-05-12 F. Santandrea , L. Y. Gorelik , R. I. Shekhter , M. Jonson

Heating and heat conduction in molecular junctions are considered within a general NEGF formalism. We obtain a unified description of heating in current carrying molecular junctions as well as the electron and phonon contributions to the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Michael Galperin , Mark A. Ratner , Abraham Nitzan

Electron spin resonance with a scanning tunneling microscope (ESR-STM) combines the high energy resolution of spin resonance spectroscopy with the atomic scale control and spatial resolution of STM. Here we describe the upgrade of a…

Instrumentation and Detectors · Physics 2019-01-30 Fabian D. Natterer , François Patthey , Tobias Bilgeri , Patrick R. Forrester , Nicolas Weiss , Harald Brune

The electrical conductance of molecular junctions may strongly depend on the temperature, and weakly on molecular length, under two distinct mechanisms: phase-coherent resonant conduction, with charges proceeding via delocalized molecular…

Mesoscale and Nanoscale Physics · Physics 2017-12-25 Hyehwang Kim , Dvira Segal

Single-walled carbon nanotubes (SWCNTs) in their pristine form have high thermal conductivity whose further improvement has attracted a lot of interest. Some theoretical studies have suggested that the thermal conductivity of a $(10,10)$…

Materials Science · Physics 2020-02-11 Haikuan Dong , Zheyong Fan , Ping Qian , Tapio Ala-Nissila , Yanjing Su

We theoretically study the heat flux between electrons and phonons in a thin metallic film embedded in a suspended dielectric slab (called a \textit{membrane}, in accordance with the established nomenclature), forming a layered structure.…

Mesoscale and Nanoscale Physics · Physics 2023-07-12 D. V. Anghel , M. Dolineanu , J. Bergli , I. J. Maasilta