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Controlling molecular reactivity by shaped laser pulses is a long-standing goal in chemistry. Here we suggest a direct optimal control approach which combines external pulse optimization with other control parameters arising in the upcoming…

Quantum Physics · Physics 2024-01-03 A. R. Ramos Ramos , E. W. Fischer , P. Saalfrank , O. Kühn

The superadiabatic quantum driving, producing a perfect adiabatic transfer on a given Hamitonian by introducing an additional Hamiltonian, is theoretically analysed for transfers within a three-level system. Our starting point is the…

Quantum Physics · Physics 2016-11-18 Luigi Giannelli , Ennio Arimondo

A method for the generation of ultrarelativistic electron beams with high spin polarization is put forward, where a tightly-focused linearly-polarized ultraintense laser pulse interacts with a nonprepolarized transverse-size-tailored solid…

Plasma Physics · Physics 2024-06-11 Xiaofei Shen , Zheng Gong , Karen Z. Hatsagortsyan , Christoph H. Keitel

Interaction of an ultrastrong short laser pulse with non-prepolarized near-critical density plasma is investigated in an ultrarelativistic regime, with an emphasis on the radiative spin polarization of ejected electrons. Our…

Plasma Physics · Physics 2021-10-29 Zheng Gong , Karen Z. Hatsagortsyan , Christoph H. Keitel

Here, we demonstrate the radiative polarization of high-energy electron beams in collisions with ultrashort pulsed bi-chromatic laser fields. Employing a Boltzmann kinetic approach for the electron distribution allows us to simulate the…

Plasma Physics · Physics 2019-12-06 Daniel Seipt , Dario Del Sorbo , Christopher P. Ridgers , Alec G. R. Thomas

Rapid development of ultrafast ultraintense laser technologies continues to create opportunities for studying strong-field physics under extreme conditions. However, accurate determination of the spatial and temporal characteristics of a…

Plasma Physics · Physics 2023-01-03 Zhi-Wei Lu , Xin-Di Hou , Feng Wan , Yousef I. Salamin , Chong Lv , Bo Zhang , Fei Wang , Zhong-Feng Xu , Jian-Xing Li

Several methods have been proposed in the literature to improve Free Electron Laser output by transforming the electron phase-space before entering the FEL interaction region. By utilising `beam by design' with novel undulators and other…

Accelerator Physics · Physics 2015-09-02 J. R. Henderson , L. T. Campbell , B. W. J. McNeil

A numerical study on ion acceleration in electrostatic shock waves is presented, with the aim of determining the best plasma configuration to achieve quasi-monoenergetic ion beams in laser-driven systems. It was recently shown that tailored…

Plasma Physics · Physics 2018-03-14 E. Boella , F. Fiúza , A. Stockem Novo , R. Fonseca , L. O. Silva

In adiabatic Cooper pair pumps, operated by means of gate voltage modulation only, the quantization of the pumped charge during a cycle is limited due to the quantum coherence of the macroscopic superconducting wave function. In this work…

Mesoscale and Nanoscale Physics · Physics 2010-09-08 Shabnam Safaei , Simone Montangero , Fabio Taddei , Rosario Fazio

We analyze the alignment of molecules generated by a pair of crossed ultra-short pump pulses of different polarizations by a technique based on the induced time-dependent gratings. Parallel polarizations yield an intensity grating, while…

Quantum Physics · Physics 2009-11-13 Arnaud Rouzee , Vincent Renard , Stephane Guerin , Olivier Faucher , Bruno Lavorel

Employing colliding-pulse injection has been shown to enable high-quality electron beams to be generated from laser-plasma accelerators. Here by leveraging test particle simulations, Hamiltonian analysis, and multidimensional…

Accelerator Physics · Physics 2023-10-09 Zheng Gong , Michael J. Quin , Simon Bohlen , Christoph H. Keitel , Kristjan Põder , Matteo Tamburini

Light-pulse atom interferometers rely on the wave nature of matter and its manipulation with coherent laser pulses. They are used for precise gravimetry and inertial sensing as well as for accurate measurements of fundamental constants.…

Quantum Physics · Physics 2015-12-02 Stephan Kleinert , Endre Kajari , Albert Roura , Wolfgang P. Schleich

An efficient mechanism of laser pulse focusing with the help of shaped underdense plasma target immersed in inhomogeneous magnetic field has been demonstrated. These studies have been carried out with the help of 2-D Particle-In-Cell (PIC)…

Plasma Physics · Physics 2025-07-01 Trishul Dhalia , Rohit Juneja , Amita Das

Altermagnets (AMs) constitute a novel class of spin-compensated materials in which the symmetry connecting opposite-spin sublattices involves a spatial rotation. Here, we uncover a set of unique non-linear, light-driven properties that set…

Materials Science · Physics 2025-09-16 Amir Eskandari-asl , Jorge I. Facio , Oleg Janson , Adolfo Avella , Jeroen van den Brink

We discuss a simple scheme for preparing atoms and molecules in an arbitrary preselected coherent superposition of quantum states. The technique, which we call fractional stimulated Raman adiabatic passage ({\it f-STIRAP}), is based upon…

Quantum Physics · Physics 2007-05-23 N. V. Vitanov , K. -A. Suominen , B. W. Shore

We theoretically demonstrate a scheme for tomographic reconstruction of asymmetric molecular orbitals based on high-order harmonic generation with a two-color multicycle laser field. It is shown that by adjusting the relative phase of the…

Atomic Physics · Physics 2013-12-30 Meiyan Qin , Xiaosong Zhu , Qingbin Zhang , Peixiang Lu

We demonstrate how the shape of femtosecond laser pulses can be tailored in order to obtain maximal ionization of atoms or molecules. For that purpose, we have overlayed a direct-optimization scheme on top of a fully unconstrained…

Computational Physics · Physics 2015-05-13 A. Castro , E. Rasanen , A. Rubio , E. K. U. Gross

Laser-driven ion acceleration provides ultra-short, high-charge, low-emittance beams, which are desirable for a wide range of high-impact applications. Yet after decades of research, a significant increase in maximum ion energy is still…

We apply the inverse geometric optimization technique to generate an optimal and robust stimulated Raman exact passage (STIREP) considering the loss of the upper state as a characterization parameter. Control fields temporal shapes that are…

Quantum Physics · Physics 2022-09-19 Xavier Laforgue , Ghassen Dridi , Stéphane Guérin

Recent studies have demonstrated the possibility of accelerating electrons to MeV energies in ambient air using tightly focused laser configurations. In this article, we explore possible strategies to control and optimize the resulting…