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We propose a scheme to transfer molecules from a slow beam into an optical trap using only a single photon absorption and emission cycle. The efficiency of such a scheme is numerically explored for BaF using realistic experimental…

A deformable body can rotate even with no angular momentum, simply by changing its shape. A good example is a falling cat, how it maneuvers in air to land on its feet. Here a first principles molecular level example of the phenomenon is…

Computational Physics · Physics 2020-09-17 Xubiao Peng , Jin Dai , Antti J. Niemi

Accurate computer simulations of the rotational dynamics of linear molecules solvated in He clusters indicate that the large-size (nano-droplet) regime is attained quickly for light rotors (HCN, CO) and slowly for heavy ones (OCS, N$_2$O,…

Other Condensed Matter · Physics 2009-11-11 S. Paolini , S. Fantoni , S. Moroni , S. Baroni

Recently, several femtosecond laser techniques have been developed that are capable of bringing gas molecules to extremely fast rotation in a very short time, while keeping their translational motion intact and relatively slow. We…

Chemical Physics · Physics 2015-03-11 Yuri Khodorkovsky , Uri Steinitz , Jean-Michel Hartmann , Ilya Sh. Averbukh

We study the coupled atom-molecular quantized ring vortices of 87Rb Bose-Einstein Condensates (BEC) trapped in a rotating three dimensional (3D) anisotropic cylindrical trap both in time independent and time-dependent Gross-Pitaevskii…

Quantum Gases · Physics 2020-04-22 Sreoshi Dutta , Krishna Rai Dastidar , Chanchal Chaudhuri

We report on the deceleration of a beam of SrF molecules from 290 to 120~m/s. Following supersonic expansion, the molecules in the $X^2\Sigma$ ($v=0$, $N=1$) low-field seeking states are trapped by the moving potential wells of a…

Atomic Physics · Physics 2019-07-17 S. C. Mathavan , A. Zapara , Q. Esajas , S. Hoekstra

Beams of neutral polar molecules in a low-field seeking quantum state can be slowed down using a Stark decelerator, and can subsequently be loaded and confined in electrostatic quadrupole traps. The efficiency of the trap loading process is…

With a Stark decelerator, beams of neutral polar molecules can be accelerated, guided at a constant velocity, or decelerated. The effectiveness of this process is determined by the 6D volume in phase space from which molecules are accepted…

Atomic and Molecular Clusters · Physics 2009-11-13 Ludwig Scharfenberg , Henrik Haak , Gerard Meijer , Sebastiaan Y. T. van de Meerakker

An alternating gradient electric guide provides a way to transport a wide variety of polar molecules, including those in high-field seeking states. We investigate the motion of polar molecules in such a guide by measuring the transmission…

Atomic Physics · Physics 2015-05-13 T. E. Wall , S. Armitage , J. J. Hudson , B. E. Sauer , J. M. Dyne , E. A. Hinds , M. R. Tarbutt

We present a comprehensive characterization of cold molecular beams from a cryogenic buffer-gas cell, providing an insight into the physics of buffer-gas cooling. Cold molecular beams are extracted from a cryogenic cell by electrostatic…

Chemical Physics · Physics 2018-12-04 X. Wu , T. Gantner , M. Zeppenfeld , S. Chervenkov , G. Rempe

The Stark effect provides a powerful method to shift the spectra of molecules, atoms and electronic transitions in general, becoming one of the simplest and most straightforward way to tune the frequency of quantum emitters by means of a…

Using an optical centrifuge to control molecular rotation in an extremely broad range of angular momenta, we study coherent rotational dynamics of nitrogen molecules in the presence of collisions. We cover the range of rotational quantum…

Chemical Physics · Physics 2015-06-19 Alexander A. Milner , Aleksey Korobenko , John W. Hepburn , Valery Milner

We present a robust, continuous molecular decelerator that employs high magnetic fields and few optical pumping steps. CaOH molecules are slowed, accumulating at low velocities in a range sufficient for loading both magnetic and…

Heavy polar molecules can be used to measure the electric dipole moment of the electron, which is a sensitive probe of physics beyond the Standard Model. The value is determined by measuring the precession of the molecule's spin in a plane…

Atomic Physics · Physics 2010-01-29 M. R. Tarbutt , J. J. Hudson , B. E. Sauer , E. A. Hinds

Photonic Molecules made of dielectric cylinders assembled as two-dimensional octagons and decagons have been studied. These structures exhibit resonance states that change their intensity depending on the incident radiation angle. While…

Optics · Physics 2018-11-14 Angel Andueza , Jesus Perez-Conde , Joaquin Sevilla

Stark deceleration has been utilized for slowing and trapping several species of neutral, ground-state polar molecules generated in a supersonic beam expansion. Due to the finite physical dimension of the electrode array and practical…

Atomic Physics · Physics 2009-11-10 Eric R. Hudson , J. R. Bochinski , H. J. Lewandowski , Brian C. Sawyer , Jun Ye

We report on the Stark deceleration of a pulsed molecular beam of NO radicals. Stark deceleration of this chemically important species has long been considered unfeasible due to its small electric dipole moment of 0.16 D. We prepared the NO…

Chemical Physics · Physics 2013-01-11 Xingan Wang , Moritz Kirste , Gerard Meijer , Sebastiaan Y. T. van de Meerakker

We report on our recent progress in the manipulation and cooling of a magnetically guided, high flux beam of $^{87}{\rm Rb}$ atoms. Typically $7\times 10^9$ atoms per second propagate in a magnetic guide providing a transverse gradient of…

Other Condensed Matter · Physics 2016-08-16 Thierry Lahaye , Z. Wang , G. Reinaudi , S. P. Rath , J. Dalibard , D. Guéry-Odelin

We here report on a quantitative study of Enantiomer-Specific State Transfer (ESST), performed in a pulsed, supersonic molecular beam. The chiral molecule 1-indanol is cooled to low rotational temperatures (1-2 K) and a selected rotational…

The rotational constant parametrizes the relative spacing between a molecule's rotational energy levels. It depends on the molecule's classical moments of inertia, which, in all studies, are expressed by treating the constituent nuclei as…

Atomic Physics · Physics 2024-02-20 Michail Athanasakis-Kaklamanakis , Gerda Neyens