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The complex Kohn variational method is extended to compute light-driven electronic transitions between continuum wavefunctions in atomic and molecular systems. This development enables the study of multiphoton processes in the perturbative…

Atomic Physics · Physics 2018-08-15 Nicolas Douguet , Barry I. Schneider , Luca Argenti

The time-dependent Schr\"{o}dinger equation for the hydrogen atom and its interaction with coherent intense high-frequency short laser pulses is solved numerically exactly by propagating the single-electron wave packets. Thereby, the…

Atomic Physics · Physics 2013-09-11 Philipp V. Demekhin , David Hochstuhl , Lorenz S. Cederbaum

In this work we study the single ionization of hydrogen and helium by the impact of a punctual Coulomb projectile. To interpretate the cross section we introduce a series of Pad\'{e} approximant. The nodes of the denominator of the Pad\'{e}…

Atomic Physics · Physics 2020-11-23 J. E. Miraglia

Streaked photoelectron emission spectra access the correlated dynamics of photoelectrons and residual target electrons with attosecond temporal resolution. We calculated ab initio single-ionization spectra for photoemission from helium…

Atomic Physics · Physics 2024-09-06 Hongyu Shi , Uwe Thumm

We study resonant two-color two-photon ionization of Helium via the 1s3p 1P1 state. The first color is the 15th harmonic of a tunable titanium sapphire laser, while the second color is the fundamental laser radiation. Our method uses…

In this paper, we study a nonlinear two-dimensional two-particle quantum tunnel effect with dissipation in diatomic H-H system. We use an instanton technique based on the path integral approach, and present analytical solutions, in the…

Strongly Correlated Electrons · Physics 2007-05-23 A. K. Aringazin , M. B. Semenov

The double-slit interference in single-photon ionization of the diatomic molecular ion $\mathrm{H}_2^+$ is theoretically studied beyond the dipole approximation. Via simulating and comparing the interactions of the prealigned…

Atomic Physics · Physics 2021-11-24 Kunlong Liu , Yibo Hu , Qingbin Zhang , Peixiang Lu

The convergent close-coupling method is applied to the calculation of fully differential cross sections for ionization of atomic hydrogen by 15.6 eV electrons. We find that even at this low energy the method is able to yield predictive…

Atomic Physics · Physics 2009-10-31 Igor Bray

The extension of coherent $\omega$-$2\omega$ control schemes, recently implemented in free-electron lasers (FELs), to molecular systems offers new opportunities to control chemical dynamics on the electronic timescale, potentially allowing…

The absolute generalized cross sections and angular distribution parameters of photoelectrons for the two-photon above threshold $3p$-ionization of Ar were calculated in the exciting photon energy range from 15.76 to 36 eV. The correlation…

We present fully ab initio simulations of attosecond streaking for ionization of helium accompanied by shake-up of the second electron. This process represents a prototypical case for strongly correlated electron dynamics on the attosecond…

Atomic Physics · Physics 2013-05-24 Renate Pazourek , Stefan Nagele , Johannes Feist , Joachim Burgdörfer

Nonrelativistic collision of proton and antiproton with hydrogen atom described by solving time-dependent Schrodinger equation numerically. Coulomb wave function discrete variable method (CWDVR) had been used to calculate electron wave…

Atomic Physics · Physics 2019-07-02 Zorigt Gombosuren , Khenmedekh Lochin , Aldarmaa Chuluunbaatar

We study the role of electron-electron correlation in the ground-state of Ne, as well as in photoionization dynamics induced by an attosecond XUV pulse. For a selection of central photon energies around 100 eV, we find that while the…

Atomic Physics · Physics 2018-01-31 Juan J. Omiste , Lars Bojer Madsen

The probability of photoionization of a heavy hydrogen like ion is calculated within the relativistic perturbation theory. The Coulomb potential of a heavy nucleus is taken into account accurately by usage of the corresponding solutions of…

Atomic Physics · Physics 2023-05-26 O. Novak , M. Diachenko , R. Kholodov

We discuss the results of the calculation of the photoionization with de-excitation of excited He and helium-like ions Li$^{+}$ and B$^{3+}$ at high but non-relativistic photon energies $\omega $. Several lower $^{1}S$ and $^{3}S$ states…

Atomic Physics · Physics 2009-11-11 M. Ya. Amusia , R. Krivec , E. Z. Liverts , V. B. Mandelzweig

The helium atom, with one nucleus and two electrons, is a prototypical system to study quantum many-body dynamics. Doubly-excited states, or quantum states in which both electrons are excited by one photon, are showcase scenarios of…

Atomic Physics · Physics 2024-08-02 Patrick Rupprecht , Nicolette G. Puskar , Daniel M. Neumark , Stephen R. Leone

We study the photoionization and autoionization of Helium atom subject to ultrashort laser pulses by using a Feshbach formalism in the time domain. We solve the time-dependent Schr\"odinger equation in terms of a configuration interaction…

Atomic Physics · Physics 2013-02-21 C. M. Granados-Castro , J. L. Sanz-Vicario

Strong field photoelectron holography has been proposed as a means for interrogating the spatial and temporal information of electrons and ions in a dynamic system. After ionization, part of the electron wave packet may directly go to the…

Atomic Physics · Physics 2016-02-22 Xiaohong Song , Cheng Lin , Zhihao Sheng , Peng Liu , Zhangjin Chen , Weifeng Yang , Shilin Hu , C. D. Lin , Jing Chen

Fully relativistic calculations are presented for the double $K$-shell photoionization cross section for several neutral medium-$Z$ atoms, from magnesium ($Z = 10$) up to silver ($Z = 47$). The calculations take into account all multipoles…

Atomic Physics · Physics 2015-06-23 V. A. Yerokhin , A. Surzhykov , S. Fritzsche

We investigate the possibility to monitor the dynamics of autoionizing states in real time and control the yields of different ionization channels in helium by simulating XUV-pump IR-probe experiments focused on the N=2 threshold. The XUV…

Atomic Physics · Physics 2015-05-18 Luca Argenti , Eva Lindroth