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Stochastic and mixed stochastic-deterministic density functional theory (DFT) are promising new approaches for the calculation of the equation-of-state and transport properties in materials under extreme conditions. In the intermediate warm…

Computational Physics · Physics 2023-09-27 Vidushi Sharma , Lee A. Collins , Alexander J. White

Examining phase stabilities and phase equilibria in strongly correlated materials asks for a next level in the many-body extensions to the local-density approximation (LDA) beyond mainly spectroscopic assessments. Here we put the…

Materials Science · Physics 2013-04-26 Daniel Grieger , Christoph Piefke , Oleg E. Peil , Frank Lechermann

We have formulated and implemented a fully charge-self-consistent density functional theory plus dynamical mean field theory methodology which enables an efficient calculation of the total energy of realistic correlated electron systems.…

Strongly Correlated Electrons · Physics 2015-06-22 Hyowon Park , Andrew J. Millis , Chris A. Marianetti

Quantitative prediction of electronic properties in correlated materials requires simulations without empirical truncations and parameters. We present a method to achieve this goal through a new ab initio formulation of dynamical mean-field…

Strongly Correlated Electrons · Physics 2021-04-08 Tianyu Zhu , Garnet Kin-Lic Chan

We present the results of numerical studies for selected materials with strongly correlated electrons using a combination of the local-density approximation and dynamical mean-field theory (DMFT). For the solution of the DMFT equations a…

Strongly Correlated Electrons · Physics 2011-02-11 Arno P. Kampf , Marcus Kollar , Jan Kunes , Michael Sentef , Dieter Vollhardt

We present an accurate implementation of total energy calculations into the local density approximation plus dynamical mean-field theory (LDA+DMFT) method. The electronic structure problem is solved through the full potential linear…

Strongly Correlated Electrons · Physics 2009-03-16 I. Di Marco , J. Minár , S. Chadov , M. I. Katsnelson , H. Ebert , A. I. Lichtenstein

We give a detailed description of a recently proposed first principles approach to the electronic structure of strongly correlated materials. The method combines the GW approximation with dynamical mean field theory. It is designed to…

Strongly Correlated Electrons · Physics 2007-05-23 Ferdi Aryasetiawan , Silke Biermann , Antoine Georges

These are introductory lectures to some aspects of the physics of strongly correlated electron systems. I first explain the main reasons for strong correlations in several classes of materials. The basic principles of dynamical mean-field…

Strongly Correlated Electrons · Physics 2009-09-29 Antoine Georges

We propose a self-consistent method for electronic structure calculations of correlated systems, which combines the local spin-density approximation (LSDA) and the dynamical mean field theory (DMFT). The LSDA part is based on the exact…

Strongly Correlated Electrons · Physics 2007-05-23 L. Chioncel , L. Vitos , I. A. Abrikosov , J. Kollar , M. I. Katsnelson , A. I. Lichtenstein

Strongly correlated materials exhibit complex electronic phenomena that are challenging to capture with traditional theoretical methods, yet understanding these systems is crucial for discovering new quantum materials. Addressing the…

Strongly Correlated Electrons · Physics 2024-11-22 Egor Agapov , Oriol Bertomeu , Andrés Carballo , Christian B. Mendl , Aaron Sander

The use of effective local Coulomb interactions that are dynamical, that is, frequency-dependent, is an efficient tool to describe the effect of long-range Coulomb interactions and screening thereof in solids. The dynamical character of the…

Strongly Correlated Electrons · Physics 2015-12-29 Silke Biermann , Ambroise van Roekeghem

We propose a dynamical mean field approach for calculating the electronic structure of strongly correlated materials from first principles. The scheme combines the GW method with dynamical mean field theory, which enables one to treat…

Strongly Correlated Electrons · Physics 2009-11-07 S. Biermann , F. Aryasetiawan , A. Georges

The electronic and magnetic properties of many strongly-correlated systems are controlled by a limited number of states, located near the Fermi level and well isolated from the rest of the spectrum. This opens a formal way for combining the…

Strongly Correlated Electrons · Physics 2010-07-15 I. V. Solovyev

We investigate the electronic structure of SrMnO$_3$ with Density Functional Theory (DFT) plus Dynamical Mean-Field Theory (DMFT). Within this scheme the selection of the correlated subspace and the construction of the corresponding Wannier…

Strongly Correlated Electrons · Physics 2018-06-20 Daniel Bauernfeind , Robert Triebl , Manuel Zingl , Markus Aichhorn , Hans Gerd Evertz

The combination of density functional theory with dynamical mean-field theory (DFT+DMFT) has become a powerful first-principles approach to tackle strongly correlated materials in condensed matter physics. The wide use of this approach…

Strongly Correlated Electrons · Physics 2022-05-10 Xin Qu , Peng Xu , Rusong Li , Gang Li , Lixin He , Xinguo Ren

Local density approximation (LDA) to the density functional theory (DFT) has continuous derivative of total energy as a number of electrons function and continuous exchange-correlation potential, while in exact DFT both should be…

Strongly Correlated Electrons · Physics 2010-06-28 V. I. Anisimov , A. V. Kozhevnikov , M. A. Korotin , A. V. Lukoyanov , D. A. Khafizullin

We have implemented the $GW$+dynamical mean field theory (DMFT) approach in the Vienna ab initio simulation package. Employing the interaction values obtained from the locally unscreened random phase approximation (RPA), we compare…

Strongly Correlated Electrons · Physics 2014-12-15 Ciro Taranto , Merzuk Kaltak , Nicolaus Parragh , Giorgio Sangiovanni , Georg Kresse , Alessandro Toschi , Karsten Held

The realistic description of correlated electron systems has taken an important step forward a few years ago as the combination of density functional methods and the dynamical mean-field theory was conceived. This framework allows access to…

Strongly Correlated Electrons · Physics 2011-06-15 M. Karolak , T. O. Wehling , F. Lechermann , A. I. Lichtenstein

We present a new scheme to include the van der Waals (vdW) interactions in approximated Density Functional Theory (DFT) by combining the Quantum Harmonic Oscillator model with the Maximally Localized Wannier Function technique. With respect…

Materials Science · Physics 2015-06-16 Pier Luigi Silvestrelli

The electronic spectrum, energy gap and local magnetic moment of paramagnetic NiO are computed by using the local density approximation plus dynamical mean-field theory (LDA+DMFT). To this end the noninteracting Hamiltonian obtained within…

Strongly Correlated Electrons · Physics 2007-05-23 X. Ren , I. Leonov , G. Keller , M. Kollar , I. Nekrasov , D. Vollhardt