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Quantum interference between multiple pathways in molecular photodissociation often results in angular momentum polarization of atomic products and this can give deep insight into fundamental physical processes. For dissociation of diatomic…

Chemical Physics · Physics 2022-04-26 Chaya Weeraratna , Arthur G. Suits , Oleg S. Vasyutinskii

Bifurcations of classical orbits introduce divergences into semiclassical spectra which have to be smoothed with the help of uniform approximations. We develop a technique to extract individual energy levels from semiclassical spectra…

Chaotic Dynamics · Physics 2009-11-07 T. Bartsch , J. Main , G. Wunner

We theoretically investigate the laser wavelength dependence of asymmetric dissociation of H$_2^+$. It is found that the electron localization in molecular dissociation is significantly manipulated by varying the wavelength of the driving…

Atomic and Molecular Clusters · Physics 2015-06-03 Kunlong Liu , Weiyi Hong , Qingbin Zhang , Peixiang Lu

In this paper decomposition of periodic orbits in bifurcation diagrams are derived in unidimensional dynamics system $x_{n+1}=f(x_{n};r)$, being $f$ an unimodal function. We proof a theorem which states the necessary and sufficient…

Double ionization of diatomic molecules by short linearly polarized laser pulses is analyzed. We consider the final stage of the ionization process, that is the decay of a highly excited two electron molecule, which is formed after…

Atomic Physics · Physics 2016-09-08 Jakub S. Prauzner-Bechcicki , Krzysztof Sacha , Bruno Eckhardt , Jakub Zakrzewski

This paper studies a class of $1\frac12$-degree-of-freedom Hamiltonian systems with a slowly varying phase that unfolds a Hamiltonian pitchfork bifurcation. The main result of the paper is that there exists an order of…

Dynamical Systems · Mathematics 2015-06-04 Kristian Uldall Kristiansen

We show that two-particle interferences can be used to probe the nuclear motion in a doubly-excited hydrogen molecule. The dissociation of molecular hydrogen by electron impact involves several decay channels, associated to different…

We address the influence of the orbital symmetry and of the molecular alignment with respect to the laser-field polarization on laser-induced nonsequential double ionization of diatomic molecules, in the length and velocity gauges. We work…

Atomic Physics · Physics 2009-11-13 C. Figueira de Morisson Faria , T. Shaaran , X. Liu , W. Yang

We are concerned with random ordinary differential equations (RODEs). Our main question of interest is how uncertainties in system parameters propagate through the possibly highly nonlinear dynamical system and affect the system's…

Dynamical Systems · Mathematics 2021-08-30 Christian Kuehn , Kerstin Lux

We study chemical oscillators in the presence of phase separation. By imposing timescale separation between slow reactions and fast diffusion, we define a dynamics at phase equilibrium for the relevant degrees of freedom. We demonstrate…

Soft Condensed Matter · Physics 2025-07-23 Jonathan Bauermann , Giacomo Bartolucci , Artemy Kolchinsky

An ab initio simulation of strong-field photodissociation of diatomic molecules was developed, inspired by recent dissociation experiments of F2-. The transition between electronic states was modeled, including the laser pulse and…

Atomic Physics · Physics 2020-06-26 Bar Ezra , Shimshon Kallush , Ronnie Kosloff

Shell structure of the single-particle spectrum for reflection-asymmetric deformed cavity is investigated. Remarkable shell structure emerges for certain combinations of quadrupole and octupole deformations. Semiclassical periodic-orbit…

Nuclear Theory · Physics 2009-10-30 A. Sugita , K. Arita , K. Matsuyanagi

The dynamics of non-polar diatomic molecules interacting with a far-detuned narrow-band laser field, that only may drive rotational transitions, is studied. The rotation of the molecule is considered both classically and quantum…

Quantum Physics · Physics 2009-11-10 A. Adelswaerd , S. Wallentowitz

We investigate the emergence of complex dynamics in a system of coupled dissipative kicked rotors and show that critical transitions can be understood via bifurcations of simple states. We study multistability and bifurcations in the single…

Chaotic Dynamics · Physics 2025-10-27 Jin Yan

Irradiation of a molecular system by an intense laser field can trigger dynamics of both electronic and nuclear subsystems. The lighter electrons usually move on much faster, attosecond time scale but the slow nuclear rearrangement damps…

Chemical Physics · Physics 2020-08-26 Nikolay V. Golubev , Tomislav Begušić , Jiří Vaníček

The effect of decaying oscillatory perturbations on autonomous Hamiltonian systems in the plane with a stable equilibrium is investigated. It is assumed that perturbations preserve the equilibrium and satisfy a resonance condition. The…

Dynamical Systems · Mathematics 2023-10-11 Oskar Sultanov

We present a quantitative semiclassical treatment of the effects of bifurcations on the spectral rigidity and the spectral form factor of a Hamiltonian quantum system defined by two coupled quartic oscillators, which on the classical level…

Chaotic Dynamics · Physics 2016-08-16 Marta Gutiérrez , Matthias Brack , Klaus Richter , Ayumu Sugita

The bifurcation period in low-mass X-ray binaries is the initial orbital pe- riod which separates the formation of converging systems (which evolve with decreasing orbital periods until the donor becomes degenerate) from the diverging…

Astrophysics · Physics 2011-02-11 Bo Ma , Xiang-Dong Li

Few-cycle pulses of intense 800 nm light are used to probe ionization and dissociation of carbon disulfide in the intensity and temporal regime where rescattering is expected to dominate the laser-molecule interaction. The wavepacket of the…

We examine the potential-energy curves and polarization of the dipole moments of two static polar molecules under the influence of an external dc electric field and their anisotropic dipole-dipole interaction. We model the molecules as…

Quantum Physics · Physics 2024-09-24 Felipe Isaule , Robert Bennett , Jörg B. Götte