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We present and test an approximate method for the semiclassical calculation of vibrational spectra. The approach is based on the mixed time-averaging semiclassical initial value representation method, which is simplified to a form that…

Chemical Physics · Physics 2018-03-22 Max Buchholz , Frank Grossmann , Michele Ceotto

We analyze the evolution of a quantum Brownian particle starting from an initial state that contains correlations between this system and its environment. Using a path integral approach, we obtain a master equation for the reduced density…

Quantum Physics · Physics 2009-10-30 Luciana Dávila Romero , Juan Pablo Paz

We present a numerical path-integral iteration scheme for the low dimensional reduced density matrix of a time-dependent quantum dissipative system. Our approach simultaneously accounts for the combined action of a microscopically modelled…

Quantum Physics · Physics 2016-10-12 A. M. Barth , A. Vagov , V. M. Axt

In this master thesis, a new approximation scheme to non-relativistic potential scattering is developed and discussed. The starting points are two exact path integral representations of the T-matrix, which permit the application of the…

Nuclear Theory · Physics 2010-01-15 Julien Carron

A multilevel approach to sample the potential energy surface in a path integral formalism is proposed. The purpose is to reduce the required number of ab initio evaluations of energy and forces in ab initio path integral molecular dynamics…

Computational Physics · Physics 2014-12-22 Hua Y. Geng

We present methods that can provide an exponential savings in the resources required to perform dynamic parameter estimation using quantum systems. The key idea is to merge classical compressive sensing techniques with quantum control…

Quantum Physics · Physics 2015-06-16 Easwar Magesan , Alexandre Cooper , Paola Cappellaro

Discretizations of the Feynman-Kac path integral representation of the quantum mechanical density matrix are investigated. Each infinite-dimensional path integral is approximated by a Riemann integral over a finite-dimensional function…

Statistical Mechanics · Physics 2007-05-23 Stephen D. Bond , Brian B. Laird , Benedict J. Leimkuhler

We present a new approach to calculate real-time quantum dynamics in complex systems. The formalism is based on the partitioning of a system's environment into "core" and "reservoir" modes, with the former to be treated quantum mechanically…

Statistical Mechanics · Physics 2015-05-30 Timothy C. Berkelbach , David R. Reichman , Thomas E. Markland

We study a model of dephasing (decoherence) in a two-state quantum system (qubit) coupled to a bath of harmonic oscillators. An exact analytic solution for the reduced dynamics of a two-state system in this model has been obtained…

Quantum Physics · Physics 2015-05-28 V. G. Morozov , S. Mathey , G. Röpke

The mixed states are important in quantum optics since they frequently appear in the decoherence problems. When one of the components of the system is prepared in the mixed state and the evolution operator of this system is not available,…

Quantum Physics · Physics 2011-02-24 Faisal A. A. El-Orany

A quantum-mechanical Gaussian wave-packet approach to the theoretical description of nuclear motions in a condensed-phase environment is developed. General expressions for the time-dependent reduced density matrix are given for a harmonic…

Chemical Physics · Physics 2009-10-31 L. Muhlbacher , A. Lucke , R. Egger

The Feynman-Vernon path integral formalism is used to derive the density matrix of a quantum oscillator that is linearly coupled to an environmental reservoir. Although low-temperature reservoirs thermalize the oscillator to the usual…

General Physics · Physics 2014-12-15 George E. Cragg

A system of trapped ions under the action of off--resonant standing--waves can be used to simulate a variety of quantum spin models. In this work, we describe theoretically quantum phases that can be observed in the simplest realization of…

Quantum Physics · Physics 2009-11-11 X. -L. Deng , D. Porras , J. I. Cirac

We present a new formulation for the emergence of classical dynamics in a quantum world by considering a path integral approach that also incorporates continuous measurements. Our program is conceptually different from the decoherence…

Quantum Physics · Physics 2025-05-23 Harsh Arora , Bishal Kumar Das , Baladitya Suri , Vaibhav Madhok

Quantum process tomography conventionally uses a multitude of initial quantum states and then performs state tomography on the process output. Here we propose and study an alternative approach which requires only a single (or few) known…

Quantum Physics · Physics 2023-11-09 Irene López Gutiérrez , Felix Dietrich , Christian B. Mendl

The paper addresses the problem of relaxation of open quantum systems. Using the path integral methods we found an analytical expression for time-dependent density matrix of two coupled quantum oscillators interacting with different baths…

Quantum Physics · Physics 2014-12-16 Illarion Dorofeyev

We introduce an improved semiclassical dynamics approach to quantum vibrational spectroscopy. In this method, a harmonic-based phase space sampling is preliminarily driven toward non-harmonic quantization by slowly switching on the actual…

Chemical Physics · Physics 2019-12-09 Riccardo Conte , Lorenzo Parma , Chiara Aieta , Alessandro Rognoni , Michele Ceotto

The concept of time-coarsened density matrix for open systems has frequently featured in equilibrium and non-equilibrium statistical mechanics, without being probed as to the detailed consequences of the time averaging procedure. In this…

Statistical Mechanics · Physics 2018-09-11 Robert Englman , Asher Yahalom

We present an approach that allows quantifying decoherence processes in an open quantum system subject to external time-dependent control. Interactions with the environment are modeled by a standard bosonic heat bath. We develop two…

Mesoscale and Nanoscale Physics · Physics 2010-10-12 Dmitry Solenov , Vladimir Privman

Warm dense matter (WDM) is an active field of research, with applications ranging from astrophysics to inertial confinement fusion. Ionization degree and continuum lowering are important quantities to understand how materials behave under…

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