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Metal-organic frameworks (MOFs) are an incredibly diverse group of highly porous hybrid materials, which are interesting for a wide range of possible applications. For a reliable description of many of their properties accurate…

Materials Science · Physics 2024-11-26 Sandro Wieser , Egbert Zojer

Predicting and characterizing the crystal structure of materials is a key problem in materials research and development. We report the results of ab initio LDA/GGA computations for the following systems: AgAu, AgCd, AgMg, AgMo*, AgNa,…

Materials Science · Physics 2009-09-29 Stefano Curtarolo , Dane Morgan , Gerbrand Ceder

In this paper I propose a new model for representing the formation energies of multicomponent crystalline alloys as a function of atom types. In the cases when displacements of atoms from their equilibrium positions are not large, the…

Computational Physics · Physics 2017-08-02 Alexander Shapeev

Au-Fe alloys are of immense interest due to their biocompatibility, anomalous hall conductivity, and applications in various medical treatment. However, irrespective of the method of preparation, they often exhibit a high-level of disorder,…

Materials Science · Physics 2017-09-27 Jiban Kangsabanik , Rajiv K. Chouhan , D. D. Johnson , Aftab Alam

Prediction and characterization of crystal structures of alloys are a key problem in materials research. Using high-throughput ab initio calculations we explore the low-temperature phase diagrams for the following systems: {Bi-In, Bi-Mg,…

Materials Science · Physics 2007-05-23 Stefano Curtarolo , Aleksey N. Kolmogorov , Franklin Hadley Cocks

This work demonstrates that fine-tuning transforms foundational machine-learned interatomic potentials (MLIPs) to achieve consistent, near-ab initio accuracy across diverse architectures. Benchmarking five leading MLIP frameworks (MACE,…

Chemical Physics · Physics 2025-11-10 Jonas Hänseroth , Aaron Flötotto , Muhammad Nawaz Qaisrani , Christian Dreßler

Two intermetallic FeAl compounds with Al content of 70.68 and 72.17 at.pct were studied using M\"ossbauer spectroscopy (5 to 296 K) and X-ray diffraction (15 to 300 K). The compounds were found to crystallize in the orthorhombic Cmcm space…

Materials Science · Physics 2021-05-19 Stanisław M. Dubiel , Łukasz Gondek , Tilo Zienert , Jan Żukrowski

Machine learning interatomic potentials (MLIPs) can now reproduce the energy, forces and stresses of bulk materials with high accuracy compared to first-principles calculations. The description of imperfections, where coordination…

Materials Science · Physics 2026-03-06 Xinwei Wang , Irea Mosquera-Lois , Aron Walsh

The advent of machine learning in materials science opens the way for exciting and ambitious simulations of large systems and long time scales with the accuracy of ab-initio calculations. Recently, several pre-trained universal machine…

Materials Science · Physics 2024-06-28 Luis Casillas-Trujillo , Abhijith S. Parackal , Rickard Armiento , Björn Alling

Icosahedral quasicrystals spontaneously form from the melt in simulations of Al--Cu--Fe alloys. We model the interatomic interactions using oscillating pair potentials tuned to the specific alloy system based on a database of density…

Materials Science · Physics 2020-03-04 Marek Mihalkovic , Michael Widom

Force matching is an established technique to generate effective potentials for molecular dynamics simulations from first-principles data. This method has been implemented in the open source code potfit. Here, we present a review of the…

A reliable prediction of interatomic force constants in disordered alloys is an outstanding problem. This is due to the need for a proper treatment of multisite (atleast pair) correlation within a random environment. The situation becomes…

Materials Science · Physics 2014-04-14 Rajiv K. Chouhan , Aftab Alam , Subhradip Ghosh , Abhijit Mookerjee

Machine learning approaches have recently emerged as powerful tools to probe structure-property relationships in crystals and molecules. Specifically, Machine learning interatomic potentials (MLIP) can accurately reproduce first-principles…

Materials Science · Physics 2024-03-01 Sasaank Bandi , Chao Jiang , Chris A. Marianetti

We report the development of a forcefield capable of reproducing accurate lattice dynamics of metal-organic frameworks. Phonon spectra, thermodynamic and mechanical properties, such as free energies, heat capacities and bulk moduli, are…

Materials Science · Physics 2016-10-28 J. K. Bristow , J. M. Skelton , K. L. Svane , A. Walsh , J. D. Gale

Machine learning potentials (MLPs) are becoming powerful tools for performing accurate atomistic simulations and crystal structure optimizations. An approach to developing MLPs employs a systematic set of polynomial invariants including…

Computational Physics · Physics 2020-11-18 Atsuto Seko

In this letter, we apply the mixed-bond spin-1 Ising model to the study of the magnetic properties of Fe-Mn alloys in the $\alpha$ phase by employing the effective field theory (EFT). Here, we suggest a new approach to the ferromagnetic…

Disordered Systems and Neural Networks · Physics 2014-11-18 A. S. Freitas , Douglas F. de Albuquerque , I. P. Fittipaldi , N. O. Moreno

$Ab-initio$ probabilities of phonon-assisted intervalley scattering of electrons in the conduction bands of ternary chalcopyrite compounds $ZnSiP_2$ and $ZnGeP_2$ between the central $\Gamma$ minima and the lowest lateral minima (valleys)…

Materials Science · Physics 2019-10-08 V. G. Tyuterev

We study the structural, electronic, and magnetic properties of Co$_2$ZAl compounds employing a pseudopotential electronic bandstructure method. The stability of the compounds is established through the formation and cohesive energy…

Materials Science · Physics 2020-08-11 Sashi Nepal , Ramesh Dhakal , Iosif Galanakis

Using indium as a test case, we investigate the accuracy of the electron-phonon coupling calculated with state-of-the-art ab initio and many-body theory methods. The ab initio calculations -- where electrons are treated in the local-density…

Superconductivity · Physics 2016-08-31 Sven P. Rudin , R. Bauer , Amy Y. Liu , J. K. Freericks

The accurate calculation of phonons and vibrational spectra remains a significant challenge, requiring highly precise evaluations of interatomic forces. Traditional methods based on the quantum description of the electronic structure, while…

Computational Physics · Physics 2025-06-03 Bowen Han , Yongqiang Cheng